By exciting high-temperature K3C60 with mid-infrared pulses, a large increase in carrier mobility is obtained, accompanied by the opening of a gap in the optical conductivity; these same signatures are observed at equilibrium when cooling K3C60 below the superconducting transition temperature of 20 kelvin, which could be an indication of light-induced high-temperature superconductivity. The use of light to control the properties of condensed-matter materials is a promising area of research, with the long-term prospect that it might lead to the development of quantum devices driven by light. In particular, it was shown recently that nonlinear excitation of certain phonons in bilayer copper oxides induces superconducting-like optical properties at temperatures far above the material's superconducting transition temperature (Tc). This effect was accompanied by the disruption of competing charge-density-wave correlations, explaining some, but not all, of the experimental results. Andrea Cavalleri and colleagues now report that by exciting metallic K3C60 with mid-infrared optical pulses, they can induce a large increase in carrier mobility, accompanied by the opening of a gap in the optical conductivity. Strikingly, these same signatures are observed at equilibrium when K3C60 cools below its Tc of 20 K. The non-equilibrium control of emergent phenomena in solids is an important research frontier, encompassing effects such as the optical enhancement of superconductivity1. Nonlinear excitation2,3 of certain phonons in bilayer copper oxides was recently shown to induce superconducting-like optical properties at temperatures far greater than the superconducting transition temperature, Tc (refs 4, 5, 6). This effect was accompanied by the disruption of competing charge-density-wave correlations7,8, which explained some but not all of the experimental results. Here we report a similar phenomenon in a very different compound, K3C60. By exciting metallic K3C60 with mid-infrared optical pulses, we induce a large increase in carrier mobility, accompanied by the opening of a gap in the optical conductivity. These same signatures are observed at equilibrium when cooling metallic K3C60 below Tc (20 kelvin). Although optical techniques alone cannot unequivocally identify non-equilibrium high-temperature superconductivity, we propose this as a possible explanation of our results.
We propose an experimental scheme to verify the quantum nonequilibrium fluctuation relations using current technology. Specifically, we show that the characteristic function of the work distribution for a nonequilibrium quench of a general quantum system can be extracted by Ramsey interferometry of a single probe qubit. Our scheme paves the way for the full characterization of nonequilibrium processes in a variety of quantum systems, ranging from single particles to many-body atomic systems and spin chains. We demonstrate our idea using a time-dependent quench of the motional state of a trapped ion, where the internal pseudospin provides a convenient probe qubit.
Autonomous engines operating at the nanoscale can be prone to deleterious fluctuations in the heat and particle currents. Thermodynamic uncertainty relations (TURs) express a fundamental lower bound which translates a trade-off relation between precision and entropy production. Importantly, recent studies have shown that they can be violated in the quantum regime, thus motivating the search for analogous quantum counterparts. In this paper, we show that the geometry of quantum nonequilibrium steady states alone directly implies the existence of TUR, but with a looser bound, which is not violated by the above recent findings. The geometrical nature of this result makes it extremely general, establishing a fundamental limit for the thermodynamics of precision. Our proof is based on the McLennan-Zubarev ensemble, which provides an exact description of nonequilibrium steady states. We first prove that the entropy production of this ensemble can be expressed as a quantum relative entropy. The TURs are then shown to be a direct consequence of the Cramer-Rao bound, a fundamental result from parameter estimation theory. By combining techniques from many-body physics and information sciences, our approach also helps to shed light on the delicate relationship between quantum effects and current fluctuations in autonomous machines, where new general bound on the power output are found and discussed.
We investigate the effects of a nearly uniform Bose-Einstein condensate (BEC) on the properties of immersed trapped impurity atoms. Using a weak-coupling expansion in the BEC-impurity interaction strength, we derive a model describing polarons, i.e., impurities dressed by a coherent state of Bogoliubov phonons, and apply it to ultracold bosonic atoms in an optical lattice. We show that, with increasing BEC temperature, the transport properties of the impurities change from coherent to diffusive. Furthermore, stable polaron clusters are formed via a phonon-mediated off-site attraction.