Previous research studies of traffic networks are mainly based on planar networks and less considered the influence of multilayer networks, which illustrate and represent different appropriate urban traffic modes. Development of rail and road networks is inseparable from the development of a prosperous urban area; thus, research on multilayer networks has scientific potential and fulfils a real need. In this paper, a framework of complex network based integrated multilayer urban growth and optimisation model (CNIMUGOM) is proposed, to analyse the complex relationships between the traffic network structure, the population growth, and the urban land‐use. The innovation of this paper is the combination of the traffic complex multilayer networks and the “Four Step Model” (which stands for trip generation, trip distribution, model split, and traffic assignment steps). With the multiobjective, multilayer network coevolution and optimisation model, a more efficient traffic network layout was generated based on different land‐use, population density, and travel speed scenarios. Then, this paper has proved that the proposed CNIMUGOM can save the traffic network construction investment, reduce the travel cost, make the urban traffic network more efficient, and decrease the total traffic flow amount. This research has connected the recent complex multilayer network related study and traditional urban economic model based study. The findings of the study afford to improve the current land‐use and traffic integrated models and can provide traffic network planning suggestions for urban agglomeration development.