The procedures for analyzing pharmaceuticals and personal care products (PPCPs) are typically tedious and expensive and thus, it is necessary to synthesize all available information from previously conducted research. An extensive collection of PPCP data from the published literature was compiled to determine the occurrence, pathways, and the effectiveness of current treatment technologies for the removal of PPCPs in water and wastewater. Approximately 90% of the compiled published papers originated from Asia, Europe, and the North American regions. The incomplete removal of PPCPs in different water and wastewater treatment processes was widely reported, thus resulting in the occurrence of PPCP compounds in various environmental compartments. Caffeine, carbamazepine, diclofenac, ibuprofen, triclosan, and triclocarban were among the most commonly reported compounds detected in water and solid matrices. Trace concentrations of PPCPs were also detected on plants and animal tissues, indicating the bioaccumulative properties of some PPCP compounds. A significant lack of studies regarding the presence of PPCPs in animal and plant samples was identified in the review. Furthermore, there were still knowledge gaps on the ecotoxicity, sub-lethal effects, and effective treatment processes for PPCPs. The knowledge gaps identified in this study can be used to devise a more effective research paradigm and guidelines for PPCP management.
Twenty-three rainfall events were monitored to determine the characteristics of the stormwater runoff entering a rain garden facility and evaluate its performance in terms of pollutant removal and volume reduction. Data gathered during the five-year monitoring period were utilized to develop a deep learning-based model that can predict the concentrations of Total Suspended Solids (TSS), Chemical Oxygen Demand (COD), Total Nitrogen (TN), and Total Phosphorus (TP). Findings revealed that the rain garden was capable of effectively reducing solids, organics, nutrients, and heavy metals from stormwater runoff during the five-year period when hydrologic and climate conditions have changed. Volume reduction was also high but can decrease over time due to the accumulation of solids in the facility which reduced the infiltration capacity and increased ponding and overflows especially during heavy rainfalls. A preliminary development of a water quality prediction model based on long short-term memory (LSTM) architecture was also developed to be able to potentially reduce the labor and costs associated with on-site monitoring in the future. The LSTM model predicted pollutant concentrations that are close to the actual values with a mean square error of 0.36 during calibration and a less than 10% difference from the measured values during validation. The study showed the potential of using deep learning architecture for the prediction of stormwater quality parameters entering rain gardens. While this study is still in the preliminary stage, it can potentially be improved for use in performance monitoring, decision-making regarding maintenance, and design of similar technologies in the future.
Stormwater treatment wetlands are widely recognized as efficient and cost-effective solutions to growing stormwater problems. This study presented a new approach to evaluating the current status and trends in stormwater treatment wetlands research. The annual scientific productivity of different states was identified using a bibliometric analysis approach. The number of publications related to stormwater treatment wetlands has exhibited an increasing trend since the earliest record of publication. USA and China were among the states that had the most number of stormwater treatment wetlands-related publications and international collaborations. In terms of the population-to-publication ratio, Australia, Canada, and South Korea were found to have a higher level of scientific productivity. Analysis of frequently used keywords and terms in scientific publications revealed that the efficiency of stormwater treatment wetlands and the processes involved in the removal of nutrients and trace elements were adequately investigated; however, inquiries on the removal of organic micropollutants and emerging pollutants, such as pharmaceuticals and personal care products, microplastics, and industrial compounds, among others, are still lacking. Through the comprehensive review of related scientific works, the design, components, and primary factors affecting the performance of stormwater treatment wetlands were also identified. Future works that address the aforementioned knowledge gaps are recommended to optimize the benefits of stormwater treatment wetlands.
Evaluating the functionality of small and decentralized low-impact development (LID) technologies often requires extensive labor, time, and costs for water quality analysis. In order to reduce these in an infiltration trench in South Korea, monitoring data gathered over a period of 8 years were used to determine its long-term performance, establish a stormwater quality estimation model, and develop a comprehensive evaluation tool. Our findings show that the infiltration trench can treat up to 90% of the stormwater runoff from a paved road but would require annual maintenance to minimize the reduction in infiltration capacity. The facility was able to remove an average of 83% of total suspended solids (TSS), 75% of biochemical oxygen demand (BOD), 80% of chemical oxygen demand (COD), 76% of total nitrogen (TN), and 79% of total phosphorus (TP), with the highest removal efficiencies observed after maintenance was conducted. Rainfall depth and air quality parameters (i.e., PM2.5 and PM10) were found to be positively correlated with TSS, COD, TN, and TP. These parameters were then used to develop a model for the estimation of influent stormwater quality, which can help in estimating the effluent water quality based on the average removal efficiencies. Furthermore, a comprehensive evaluation tool considering indicators such as treatment efficiency, cultural benefits, and facility and operating conditions was established through the analytic hierarchy process (AHP). Aside from determining the facility’s overall efficiency, this can also serve as a diagnostic tool to identify whether maintenance is needed or not. While atmospheric and hydrological characteristics differ in different regions, and the results may vary if applied in other facilities, this study can serve as a guide to the effective and efficient evaluation of similar stormwater management facilities in South Korea.
With the increasing effect of urbanization becoming more apparent through flooding and decline in downstream water quality especially from heavy rainfalls, stormwater runoff management solutions have focused on treatment and infiltration. However, there are areas with low infiltration soils or are experiencing more dry days and even drought. In this study, experiments were conducted to compare the applicability of high infiltration and low infiltration soils as a base layer in gravel-filled infiltration systems with emphasis on runoff capture and suspended solids removal. Findings showed that infiltration rates increased with the water depth above the gravel-soil interface indicating the available depth for water storage affects this parameter. Runoff capture in high infiltration systems are more affected by rainfall depth and inflow rates as compared to low infiltration systems. Based on runoff capture and pollutant removal analysis, a media depth of 0.4 − 1 m and maximum infiltration rate of 200 mm/h were recommended. Moreover, it was revealed that low infiltration systems are more susceptible to horizontal flow and that the length of the structure may be more critical than depth in this condition.
A laboratory study was undertaken to pursue the filter performance of a micro-filter module employing highly porous fibre media under a high filtration rate (≥1,500 m/day), faster than that of any conventional filter process. The effects of filtration rate, head loss, raw water turbidity, and filter aid chemicals on filter performance were analysed. In spite of the extremely high filtration rate, the filter achieved an attractive efficiency, reducing the raw water turbidity by over 80%. As with other filter systems, the filter aid used ((polyaluminium chloride (PAC)) greatly affected the performance of this particular fibre filter. Long-term repetitive runs were additionally carried out to confirm the reproducibility of the filter performance. Also, a comparison was carried out with other high-rate filter systems which are either being tested for use in experimental studies, or are already commercially available. This study reveals that the filter performance under a high filtration speed is still attractive especially as PAC is used. Due to the high porosity of the fibre, the filter had small head loss even though the filtration rate was high. These results ascertain that it is possible to operate the filters with high filtration rate achieving reliable treatment performance.