The emissions of greenhouse gases, especially CO2, have been identified as the main contributor for global warming and climate change. Carbon capture and storage (CCS) is considered to be the most promising strategy to mitigate the anthropogenic CO2 emissions. This review aims to provide the latest developments of CO2 storage from the perspective of improving safety and economics. The mechanisms and strategies of CO2 storage, focusing on their characteristics and current status, are discussed firstly. In the second section, the strategies for assessing and ensuring the security of CO2 storage operations, including the risks assessment approach and monitoring technology associated with CO2 storage, are outlined. In addition, the engineering methods to accelerate CO2 dissolution and mineral carbonation for fixing the mobile CO2 are also compared within the second section. The third part focuses on the strategies for improving economics of CO2 storage operations, namely enhanced industrial production with CO2 storage to generate additional profit, and co-injection of CO2 with impurities to reduce the cost. Moreover, the role of multiple CCS technologies and their distribution on the mitigation of CO2 emissions in the future are summarized. This review demonstrates that CO2 storage in depleted oil and gas reservoirs could play an important role in reducing CO2 emission in the near future and CO2 storage in saline aquifers may make the biggest contribution due to its huge storage capacity. Comparing the various available strategies, CO2-enhanced oil recovery (CO2-EOR) operations are supposed to play the most important role for CO2 mitigation in the next few years, followed by CO2-enhanced gas recovery (CO2-EGR). The direct mineralization of flue gas by coal fly ash and the pH swing mineralization would be the most promising technology for the mineral sequestration of CO2. Furthermore, by accelerating the deployment of CCS projects on large scale, the government can also play its role in reducing the CO2 emissions.
Underground gas storage reservoirs (UGSRs) are used to keep the natural gas supply smooth. Native natural gas is commonly used as cushion gas to maintain the reservoir pressure and cannot be extracted in the depleted gas reservoir transformed UGSR, which leads to wasting huge amounts of this natural energy resource. CO2 is an alternative gas to avoid this particular issue. However, the mixing of CO2 and CH4 in the UGSR challenges the application of CO2 as cushion gas. In this work, the Donghae gas reservoir is used to investigate the suitability of using CO2 as cushion gas in depleted gas reservoir transformed UGSR. The impact of the geological and engineering parameters, including the CO2 fraction for cushion gas, reservoir temperature, reservoir permeability, residual water and production rate, on the reservoir pressure, gas mixing behavior, and CO2 production are analyzed detailly based on the 15 years cyclic gas injection and production. The results showed that the maximum accepted CO2 concentration for cushion gas is 9% under the condition of production and injection for 120 d and 180 d in a production cycle at a rate of 4.05 kg/s and 2.7 kg/s, respectively. The typical curve of the mixing zone thickness can be divided into four stages, which include the increasing stage, the smooth stage, the suddenly increasing stage, and the periodic change stage. In the periodic change stage, the mixed zone increases with the increasing of CO2 fraction, temperature, production rate, and the decreasing of permeability and water saturation. The CO2 fraction in cushion gas, reservoir permeability, and production rate have a significant effect on the breakthrough of CO2 in the production well, while the effect of water saturation and temperature is limited.
5 April 2022 in Journal of Natural Gas Science and Engineering
In this study, polyampholyte inhibitor DAM was synthesized from three monomers, namely, diallyl dimethyl ammonium chloride, methyl allyl alcohol and 2-acrylamido-2-methyl propane sulfonic acid, by aqueous solution polymerization.
11 September 2015 in Particulate Science and Technology
Lost circulation of drilling fluid occurs frequently when drilling in fractured formations. Granular lost circulation material (LCM) is still widely used as a cure to combat the circulation loss of drilling fluid. The placement styles of granular LCM in the fractured thief zone are discussed in this paper. A series of experimental tests to examine the placement style have been carried out using a new developed test equipment. The effects of the material type, particle size distribution (PSD), and concentration of the granular LCMs on the plugging behavior have been investigated. The experimental results proved that t the rigid granules work as an ideal bridging material determining the plugging depth, and the powder material is more suitable as filling material controlling the total fluid loss. The PSD of granular LCM dominates the placement style and efficiency in fractured thief zone, and there exists an optimum concentration for maximum effect of granular LCM additives.