The Infrared Atmospheric Sounding Interferometer (IASI) forms the main infrared sounding component of the European Organisation for the Exploitation of Meteorological Satellites's (EUMETSAT's) Meteorological Operation (MetOp)-A satellite (Klaes et al. 2007), which was launched in October 2006. This article presents the results of the first 4 yr of the operational IASI mission. The performance of the instrument is shown to be exceptional in terms of calibration and stability. The quality of the data has allowed the rapid use of the observations in operational numerical weather prediction (NWP) and the development of new products for atmospheric chemistry and climate studies, some of which were unexpected before launch. The assimilation of IASI observations in NWP models provides a significant forecast impact; in most cases the impact has been shown to be at least as large as for any previous instrument. In atmospheric chemistry, global distributions of gases, such as ozone and carbon monoxide, can be produced in near–real time, and short-lived species, such as ammonia or methanol, can be mapped, allowing the identification of new sources. The data have also shown the ability to track the location and chemistry of gaseous plumes and particles associated with volcanic eruptions and fires, providing valuable data for air quality monitoring and aircraft safety. IASI also contributes to the establishment of robust long-term data records of several essential climate variables. The suite of products being developed from IASI continues to expand as the data are investigated, and further impacts are expected from increased use of the data in NWP and climate studies in the coming years. The instrument has set a high standard for future operational hyperspectral infrared sounders and has demonstrated that such instruments have a vital role in the global observing system.

The Joint Polar Satellite System (JPSS) Cross‐track Infrared Microwave Sounder Suite (CrIMSS) is an advanced operational satellite sounding system concept comprised of the Cross‐track Infrared Sounder and the Advanced Technology Microwave Sounder. These are synergistically designed to retrieve key environmental data records (EDR), namely atmospheric vertical temperature, moisture, and pressure profiles. CrIMSS will serve as the low‐Earth orbit satellite sounding system, starting with the Suomi National Polar‐orbiting Partnership (S‐NPP) satellite and spanning the JPSS‐1 and JPSS‐2 satellites. This paper organizes the general paradigm for validation of atmospheric profile EDR retrieved from satellite nadir sounder systems (e.g., CrIMSS) as a synthesis of complementary methods and statistical assessment metrics. The validation methodology is ordered hierarchically to include global numerical model comparisons, satellite EDR intercomparisons, radiosonde matchup assessments (conventional, dedicated, and reference), and intensive campaign “dissections.” We develop and recommend the proper approach for computing profile statistics relative to correlative data derived from high‐resolution in situ data (viz., radiosondes) reduced to forward model layers. The standard statistical metrics used for EDR product assessments on “coarse layers” are defined along with an overview of water vapor weighting schemes and the use of averaging kernels. We then overview the application of the methodology to CrIMSS within the context of the JPSS calibration/validation program, with focus given to summarizing the core data sets to be used for validation of S‐NPP sounder EDR products.

We perform a demonstration experiment using the National Oceanic Atmospheric Administration Unique Cross-track Infrared Sounder (CrIS)/Advanced Technology Microwave Sounder Processing System to assess the improvement on trace gas retrievals upon switching to high spectral resolution CrIS radiance measurements (0.625 cm^-1). The focus of this study is carbon monoxide retrievals. The experimental high spectral resolution CO retrievals show a remarkable improvement, of almost up to one order of magnitude in the degree of freedom of the signal, with respect to the low-resolution mode. Furthermore, high-resolution CO retrievals show similar skill with respect to existing CO operational products from the Atmospheric InfraRed Sounder, Atmospheric Sounder Interferometer, and Measurements of Pollution In The Troposphere instruments, both in terms of spatial variability and degrees of freedom. The results of this research provide evidence to support the need for high spectral resolution CrIS measurements. This is a fundamental prerequisite in guaranteeing continuity to the CO afternoon orbit monitoring as part of a multisatellite uniformly integrated long-term data record of atmospheric trace gases.

Mid-upper tropospheric methane (CH₄), as an operational product at NOAA's (National Oceanic and Atmospheric Administration) Comprehensive Large Array-data Stewardship System (CLASS), has been retrieved from the Infrared Atmospheric Sounding Interferometer (IASI) since 2008. This paper provides a description of the retrieval method and the validation using 596 CH₄ vertical profiles from aircraft measurements by the HIAPER Pole-to-Pole Observations (HIPPO) program over the Pacific Ocean. The number of degrees of freedom for the CH₄ retrieval is mostly less than 1.5, and it decreases under cloudy conditions. The retrievals show greatest sensitivity between 100–600 hPa in the tropics and 200–750 hPa in the mid- to high latitude. Validation is accomplished using aircraft measurements (convolved by applying the monthly mean averaging kernels) collocated with all the retrieved profiles within 200 km and on the same day, and the results show that, on average, a larger error of CH₄ occurs at 300–500 hPa. The bias in the trapezoid of 374–477 hPa is −1.74% with a residual standard deviation of 1.20%, and at layer 596–753 hPa the bias is −0.69% with a residual standard deviation of 1.07%. The retrieval error is relatively larger in the high northern latitude regions and/or under cloudy conditions. The main reasons for this negative bias include the uncertainty in the spectroscopy near the methane Q branch and/or the empirical bias correction, plus residual cloud contamination in the cloud-cleared radiances. It is expected for NOAA to generate the CH₄ product for 20 + years using a similar algorithm from three similar thermal infrared sensors: Atmospheric Infrared Sounder (AIRS), IASI and the Cross-track Infrared Sounder (CrIS). Such a unique product will provide a supplementary to the current ground-based observation network, particularly in the Arctic, for monitoring the CH₄ cycle, its transport and trend associated with climate change.

Several recent studies have observed systematic differences between measurements in the 183.31 GHz water vapor line by space-borne sounders and calculations using radiative transfer models, with inputs from either radiosondes (radiosonde observations, RAOBs) or short-range forecasts by numerical weather prediction (NWP) models. This paper discusses all the relevant categories of observation-based or model-based data, quantifies their uncertainties and separates biases that could be common to all causes from those attributable to a particular cause. Reference observations from radiosondes, Global Navigation Satellite System (GNSS) receivers, differential absorption lidar (DIAL) and Raman lidar are thus overviewed. Biases arising from their calibration procedures, NWP models and data assimilation, instrument biases and radiative transfer models (both the models themselves and the underlying spectroscopy) are presented and discussed. Although presently no single process in the comparisons seems capable of explaining the observed structure of bias, recommendations are made in order to better understand the causes.