We study in this work the two-dimensional dynamics of an experimental system of disk-shaped rotors, fluidized by turbulent upflow. Contrary to previous knowledge, our experiments show the same particle chiral geometry can produce flows with different chiralities. In particular, we unveil a conspicuous complex chiral flow which displays multiple persistent vortices with either sign, located randomly in the system. This peculiar phase mediates a continuous transition, which takes place as the kinetic energy input increases, from a flow with positive chirality (one vortex rotating in the same direction as particles spin) to a flow with negative chirality (one vortex in opposite sense to particle spin). We find that these surprising transitions are determined by the specific state of the statistical correlations between particle-spin and translational velocity. We discuss how these correlations are determined in turn by the combined action of a series of mechanisms (for instance, heat dissipation at the boundaries, particle activity, average kinetic energy...), several of which are unveiled here.
Diffusion is a fundamental aspect of transport processes in biological systems, and thus, in the development of life itself. And yet, the diffusive dynamics of active fluids with directed rotation, known as chiral fluids, has not been analyzed in detail so far. Here, we describe the diffusive regimes of a two-dimensional chiral fluid, composed in this case of a set of identical disk-shaped rotors. We found strong experimental evidence of odd diffusion. This odd diffusion emerges in the form of a two-dimensional tensor with an antisymmetric part. In particular, we show that chiral diffusion is complex, featuring transitions between super, quasi-normal, and sub diffusion, and very slowly aging. Moreover, we show that the diffusion tensor elements, including off-diagonal elements; i.e., odd diffusion coefficient, change sign according to flow vorticity. Therefore, the chiral fluid has a self regulated diffusion, controlled by its vorticity.
The structural properties of the Jagla fluid are studied by Monte Carlo (MC) simulations, numerical solutions of integral equation theories, and the (semi-analytical) rational-function approximation (RFA) method. In the latter case, the results are obtained from the assumption (supported by our MC simulations) that the Jagla potential and a potential with a hard core plus an appropriate piecewise constant function lead to practically the same cavity function. The predictions obtained for the radial distribution function, , from this approach are compared against MC simulations and integral equations for the Jagla model, and also for the limiting cases of the triangle-well potential and the ramp potential, with a general good agreement. The analytical form of the RFA in Laplace space allows us to describe the asymptotic behavior of in a clean way and compare it with MC simulations for representative states with oscillatory or monotonic decay. The RFA predictions for the Fisher-Widom and Widom lines of the Jagla fluid are obtained.
We study in this work the dynamics of a collection of identical hollow spheres (ping-pong balls) that rest on a horizontal metallic grid. Fluidization is achieved by means of a turbulent air current coming from below. The upflow is adjusted so that the particles do not levitate over the grid, resulting in quasi-two-dimensional dynamics. We show that the behavior of diffusion and correlations in this system is particularly rich. Noticeably as well (and related to the complex dynamical behavior), a variety of phases appear, with important peculiarities with respect to analogous setups. We observe gas, liquid, glass, and hexagonal crystal phases. Most notably, we show that the melting of the hexagonal crystal occurs in coexistence with a liquid phase. This strikingly differs from the corresponding transition in a purely two-dimensional systems of air-fluidized disks, for which no phase coexistence has been reported in the literature.
In this paper, we present a molecular dynamics study of the glass transition for a soft-core primitive model for ionic liquids, in which cations are fully flexible chains of tangent soft spherical monomers, being the positively charged monomer at one of the ends of the chain, and anions as charged soft spheres. We have monitored transport coefficients such as the self-diffusion coefficients and the shear viscosity, as well as correlation functions such as the mean-square displacement, the self-intermediate scattering function, and probes of heterogeneous dynamics such as the van Hove distribution function and the four-points susceptibility. The analysis of these properties indicates that, for a given pressure, the glass transition shows a weak temperature dependence on the cation length, occurring first for short-chain than for long-chain ionic liquids.