The advent of the path to a single cycle X-ray laser pulse via thin film compression and the relativistic compression enables laser wakefield acceleration in solid materials. We study the collective interaction of the X-ray laser pulse with the solid-state plasma, including ultrafast polariton effects, giving rise to TeV/cm wakefields with highly increased critical density. Our particle-in-cell computational analysis delineates wakefield effects and polariton dynamics. We show that a good quality wakefield can be excited even in the presence of the lattice force and the electron acceleration process is not influenced by polaritons. The applications and implications of the ultrafast wakefield and ultrafast plasmonics are discussed.

Thin-film compression (TFC) and the focusability of high-power laser pulses after self-phase modulation in thin films at transport intensities ($\sim 1\mathrm{TW}/{\mathrm{cm}}^2$) for petawatt laser systems is demonstrated. High-energy ($\sim 296\mathrm{mJ}$) laser pulses are compressed from $\sim 55\mathrm{fs}$ to $\sim 31\mathrm{fs}$. Additionally, the focusability of high-power ($\sim 45–55\mathrm{TW}$) flat-top laser pulses after spectral broadening in thin films is found to be largely maintained, showing only modest decreases in the energy contained in the central part of the focal spot. In light of these findings, TFC offers a method for moving toward single-cycle pulse durations at significantly higher energies than those found at present, and if beam instabilities can be mitigated, maybe even higher intensities.

Intense few-cycle laser pulses have a breadth of applications in high energy density science, including particle acceleration and x-ray generation. Multi-amplifier laser system pulses have durations of tens of femtoseconds or longer. To achieve high intensities at the single-cycle limit, a robust and efficient post-compression scheme is required. We demonstrate a staged compression technique using self-phase modulation in thin dielectric media, in which few-cycle pulses can be produced. The few-cycle pulse is then used to generate extreme ultravoilet light via high harmonic generation at strong field intensities and to generate MeV electron beams via laser solid interactions at relativistic intensities.

Significance: Three-photon excitation microscopy has double-to-triple the penetration depth in biological tissue over two-photon imaging and thus has the potential to revolutionize the visualization of biological processes in vivo. However, unlike the plug-and-play operation and performance of lasers used in two-photon imaging, three-photon microscopy presents new technological challenges that require a closer look at the fidelity of laser pulses. Aim: We implemented state-of-the-art pulse measurements and developed innovative techniques for examining the performance of lasers used in three-photon microscopy. We then demonstrated how these techniques can be used to provide precise measurements of pulse shape, pulse energy, and pulse-to-pulse intensity variability, all of which ultimately impact imaging. Approach: We built inexpensive tools, e.g., a second harmonic generation frequency-resolved optical gating (SHG-FROG) device and a deep-memory diode imaging (DMDI) apparatus to examine laser pulse fidelity. Results: First, SHG-FROG revealed very large third-order dispersion (TOD). This extent of phase distortion prevents the efficient temporal compression of laser pulses to their theoretical limit. Furthermore, TOD cannot be quantified when using a conventional method of obtaining the laser pulse duration, e.g., when using an autocorrelator. Finally, DMDI showed the effectiveness of detecting pulse-to-pulse intensity fluctuations on timescales relevant to three-photon imaging, which were otherwise not captured using conventional instruments and statistics. Conclusions: The distortion of individual laser pulses caused by TOD poses significant challenges to three-photon imaging by preventing effective compression of laser pulses and decreasing the efficiency of nonlinear excitation. Moreover, an acceptably low pulse-to-pulse amplitude variability should not be assumed. Particularly for low repetition rate laser sources used in three-photon microscopy, pulse-to-pulse variability also degrades image quality. If three-photon imaging is to become mainstream, our diagnostics may be used by laser manufacturers to improve system design and by end-users to validate the performance of their current and future imaging systems.

The thin-film post-compression technique has the ability to reduce the pulse duration in PW-class lasers, increasing the peak power. Here, the nonlinear response of an increasingly available optical thermoplastic demonstrates enhanced spectral broadening, with corresponding shorter pulse duration compared to fused silica glass. The thermoplastic can be used close to its damage threshold when refreshed using a roller mechanism, and the total amount of material can be varied by folding the film. As a proof-of-principle demonstration scalable to 10-PW, a roller mechanism capable of up to 6 passes through a sub-millimeter thermoplastic film is used in vacuum to produce two-fold post-compression of the pulse. The compact design makes it an ideal method to further boost ultrahigh laser pulse intensities with benefits to many areas, including driving high energy acceleration.

Experimental evidence has accumulated to indicate that wakefield acceleration (WFA) accompanies intense and sometimes coherent emission of radiation such as from betatron radiation. The investigation of this issue has additional impetus nowadays because we are learning (1) there is an additional acceleration process of the ponderomotive acceleration; (2) WFA may become relevant in much higher density regimes; (3) WFA has been proposed as the mechanism for extreme high energy cosmic ray acceleration and gamma ray bursts for active galactic nuclei. These require us to closely examine the radiative mechanisms in WFA anew. We report studies of radiation from wakefield (self-injected betatron) and ponderomotive (laser field) mechanisms in scalings of the frequency and intensity of the driver, as well as the plasma density.