In spite of the still increasing number of engineered nanomaterial (ENM) applications, large knowledge gaps exist with respect to their environmental fate, especially after release into air. This review aims to summarize the current knowledge of emissions and behavior of airborne engineered nanomaterials. The whole ENM lifecycle is considered from the perspective of possible releases into the atmosphere. Although in general, emissions during use phase and end-of-life seem to play a minor role compared to entry into soil and water, accidental and continuous emissions into air can occur especially during production and some use cases such as spray application. Implications of ENMs on the atmosphere as e.g., photo-catalytic properties or the production of reactive oxygen species are reviewed as well as the influence of physical processes and chemical reactions on the ENMs. Experimental studies and different modeling approaches regarding atmospheric transformation and removal are summarized. Some information exists especially for ENMs, but many issues can only be addressed by using data from ultrafine particles as a substitute and research on the specific implications of ENMs in the atmosphere is still needed.
30 April 1992 in Journal of Geophysical Research: Atmospheres
In the land use planning framework in the neighbourhood of industrial facilities, the current approach to predicting the consequences of massive toxic gas releases is generally based on Gaussian or integral models. For many years, CFD models have been more and more used in this context, in accordance with the development of high-performance computing (HPC). The present paper focuses on harmonising input data for atmospheric transport and dispersion (AT&D) modelling between the widely used approaches. First, a synthesis of the practice’s harmonisation for atmospheric dispersion modelling within the framework of risk assessment is presented. Then, these practices are applied to a large-scale INERIS ammonia experimental release. For illustration purposes, the impact of the proposed harmonisation will be evaluated using different approaches: the SLAB model, the FDS model, and the Code_Saturne model. The two main focuses of this paper are the adaptation of the source term dealing with a massive release and the wind flow modelling performance using an experimental signal for CFD model inflow. Finally, comparisons between the modelling and experimental results enable checking the consistency of these approaches and reinforce the importance of the input data harmonisation for each AT&D modelling approach.
1 January 2018 in International Journal of Environment and Pollution