This study evaluates radon exhalation rates and assesses the potential radiological risks of external exposure to primordial radionuclides in building materials employed in the Ica region of Peru, particularly those with high uranium content. The radon exhalation rates are currently measured using a combination of a closed chamber and an active monitor. We proposed a novel method that effectively ensured a hermetic seal for the closed chamber and guaranteed that the efficient maintenance of secular equilibrium. The obtained results ranged from below the detection limit (BDL) to a maximum of 52.3 mBq · kg−1h−1. Gamma spectrometry was employed to measure the concentrations of radionuclides by utilizing a 3′ × 3′ NaI detector. The analysis of cement samples revealed a strong positive correlation between the activity concentration of radium and the radon exhalation rate. The activity concentrations for radionuclides varied, with values ranging from BDL to 60.6 mBq · kg−1h−1 for 226Ra, BDL to 22.3 mBq · kg−1h−1 for 232Th, and BDL to 1074 mBq · kg−1h−1 for 40K. These findings contribute valuable insight to decision-making processes in the Peruvian construction industry, particularly regarding material safety and radiological risk management.
Mining generates significant amounts of waste that can represent a source of contamination for areas close to the extraction area, generating a negative impact both on the environment and the health of people. This study aims to evaluate the radiological risk derived from exposure to natural radionuclides contained in tailings from Peruvian gold mines and to establish whether the tailings can be used as raw materials in building materials. The mine tailings come from a mining project in the northern highlands of Peru. Radon exhalation was measured using Rad7 in a closed chamber and activity concentration of 226Ra, 232Th, and 40K radioisotopes by gamma spectrometry using NaI 3” × 3” detector. Maximum activity concentrations measured for 226Ra and 232Th were 15.38 Bq kg−1 and 11.9 Bq kg−1, respectively; meanwhile, activity concentration for 40K ranged from 182.7 Bq kg−1 to 770.8 Bq kg−1. All activity concentrations were below the worldwide average except for 40K. The radon exhalation rate varied from 2.8 to 7.2 mBq kg−1 h−1. The gamma index (Iγ), and radiological parameters, including the Radium equivalent activity (Raeq), and the external hazard index (Hex), being below the recommended levels by UNSCEAR, ensure the safe use of these mines tailing to produce a geopolymer cement.
Radon is the main source of natural radioactivity, and its measurement is considered extremely important in radioprotection, given its relationship with the occurrence of lung cancer. In the last two years, measurements of this radioactive gas were carried out in Lima considering a grid of 5 km and the population density to determine the number of measurements to be carried out. Cellulose nitrate nuclear track detectors exposed in bare mode and diffusion chamber mode were used to estimate Rn concentrations. In diffusion chamber mode, non-commercial monitors and commercial monitors were used. The monitoring results are presented for 43 districts of the Lima Province whose population is approximately ten million inhabitants occupying a total area of 2655.15 km. Measurements were made obtaining an average concentration of 49 Bq·m using bare detectors and 66 Bq·m using non-commercial diffusion chambers. Average concentrations obtained by both detector exposure modes were below the maximum concentration recommended by the WHO. A radon (Rn) map was also obtained as a visual representation of the Rn levels in the Lima province using inverse distance weighting (IDW) interpolation.
Lima City is situated on alluvial fan deposits of rivers flowing through geological formations that contain different levels of uranium. In this paper, a study is made on the average spatial and temporal behavior of radon gas in soils of Lima City. Radon concentration was determined using the LR-115 type 2 track detector during 36 periods, of 14 days each, in twenty holes distributed in the fifteen districts of Lima City. Radon concentration in soil pores ranged from 0.1 to 64.3 kBq/m3 with an average value of 5.6 kBq/m3. The average radon concentration in soil gas was about two times lower in winter than in the other seasons. High radon values during October/November 2017 were related to the earthquakes perceived in Lima City in that period. The highest radon concentrations were found in areas of alluvial deposits whose parental material has been removed from the Quilmaná and Huarangal volcanics by the Chillón and Huaycoloro Rivers. Soil gas radon concentrations were even higher in areas closer to volcanic and less distant from rivers. During the period of maximum flooding of the Chillón, Rímac and Lurín rivers, due to the natural phenomenon “El Niño Costero”, anomalous high soil radon concentrations were observed in most of the measurement sites located near rivers. These high radon values were associated with ground vibrations caused by rock and debris avalanches in rivers and creeks.