We developed polymer-dispersed liquid crystals (PDLCs) that effectively scatter light both in the visible and near-infrared ranges simultaneously. Such PDLCs are characterized by an optimal size distribution of nematic liquid crystal droplets within 0.4 − 3 µm, which is achieved due to the specially selected copolymer, the elaborated liquid crystal material as well as the proper cooling mode from the isotropic phase. These PDLC films provide electrically controlled light scattering modulation in the spectral range 300 − 2300 nm with the response time around 10 ms.
We study the electro-optic properties of subwavelength-pitch deformed-helix ferroelectric liquid crystals (DHFLC) illuminated with unpolarized light. In the experimental setup based on the Mach-Zehnder interferometer, it was observed that the reference and the sample beams being both unpolarized produce the interference pattern which is insensitive to rotation of in-plane optical axes of the DHFLC cell. We find that the field-induced shift of the interference fringes can be described in terms of the electrically dependent Pancharatnam relative phase determined by the averaged phase shift, whereas the visibility of the fringes is solely dictated by the phase retardation.
In this paper, we report a study on Si nanopatterns, fabricated as a one-dimensional (1D) Si nanograting with a sub-wavelength (≈200 nm) period. Unpolarized light normally incident on the nanopatterned Si becomes partially polarized and chiral over the entire visible range of 380–740 nm. The degree and the state of polarization of light were measured using polarimetric and ellipsometric techniques. The analysis showed that the reflected light is partially linearly polarized and at the same time a slight chirality (Ŝ3≠0) is observed. Although the polarization of the reflected light is related to the 1D nanograting anisotropy, the chiral transformation of the light could be related to a micrometer-scale chiral substructure on the Si nanopatterned surface. This structure results from the dynamic polarization rotation of the femtosecond laser pulses in their filaments in liquid carbon disulfide near the Si surface during the interferential plasmonic self-organization of the surface nanorelief. These results could underline a key enabling process for the fabrication of polarization-sensitive metasurface-based sensors or devices within the common complementary metal-oxide semiconductor (CMOS)-compatible technology.
In our investigation into the effects of the degree of polarization in modulation of partially polarized light, we assume general settings of the interferometry of partially polarized light waves and perform theoretical analysis of the geometric phases: the Uhlmann phase and the interferometric phase. We introduce the relative Uhlmann phase determined by the Uhlmann holonomies of interfering beams and show that the interferometric phase generalized to the case of nonunitary evolution can, similar to the Uhlmann phase, be cast into the holonomy defined form. By using the technique based on a two-arm Mach-Zehnder interferometer, two different dynamical regimes of light modulation are experimentally studied: (a) modulation of the input light by the rotating quarter-wave plate (QWP), and (b) modulation of the testing beam by a birefringent plate with electrically controlled anisotropy represented by the deformed-helix ferroelectric liquid-crystal (DHFLC) cell. In the setup with the rotating QWP, the interferometric phase is found to be equal to the relative Uhlmann phase. Experimental and theoretical results being in excellent agreement show both that this phase is an oscillating function of the QWP angle and increases with the degree of polarization. For modulation by the DHFLC cell, the data derived from our electro-optic measurements are fitted using the theory of the orientational Kerr effect in FLCs. This theory in combination with the results of fitting is used to evaluate electric field dependencies of the interferometric and the Uhlmann phases.
We disclose the method to obtain polarization insensitive phase-only modulation that preserves both the state and the degree of polarization of light modulated using a medium with controlled birefringence. We find that, in the double-pass configuration involving reflection from the Faraday rotator mirror, such a medium acts as the phase-only modulator. The experimental data measured in the Michelson-interferometer-based setup for deformed-helix ferroelectric liquid crystal cells are found to be in good agreement with the theoretical results. For such cells, we experimentally demonstrate high-frequency (4 kHz modulation rate) phase-only light modulation governed by the average phase shift and solve the problem of optical axes switching.
1 September 2018 in Journal of Physics: Conference Series
We study modulation of partially polarized light governed by the orientational Kerr effect in subwavelength-pitch deformed-helix ferroelectric liquid crystals. In our experimental setup based on the Mach-Zehnder interferometer, it is found that the electric field induced shift of the interference fringes crucially depends on the degree of polarization of the incident light. We show that the experimental data can be theoretically described in terms of the electrically dependent Pancharatnam relative phase. The electric field dependence of both the Pancharatnam and geometric phases is evaluated by comparing the experimental and theoretical results.