For laser ablation micropropulsion technology with metal as the target to increase the total impulse, the effective utilization and supply of a working medium is a crucial aspect. In this research, the ablation characteristics and propulsion performance of the typical metal targets, copper and aluminum, ablated via nanosecond laser ablation are analyzed. Due to the low melting point of aluminum, the protrusion characteristics in the remelted area are more prominent. Its surface morphology has characteristics for height extremum and roughness that are higher than those of copper. Affected by the anisotropy of the rough surface, the absorbed energy decreases with increasing roughness. The impulse coupling coefficient of the metal decreases and stabilizes at about 6 μN·W⁻¹. The specific pulse of aluminum obtains a minimum value of 603.6 s at 6000 pulses and improves with increasing pulses. The propulsion parameters of copper alters slightly under various working conditions, with a maximum specific impulse of 685 s.