Chang-Qi Ma

Dr. Chang-Qi Ma


Research Focus & Metrics

Academic Career Length

15Years (2012-Present)

(Calculated once Scilit publication data is synced: current year − year of first publication + 1)

Representative Publications

View All Publications
22 January 2020 in Nature Energy
Verified
Journal Article
Open access
PDF file
MKMark V. Khenkin
Mark V. Khenkin
EKEugene A. Katz
Eugene A. Katz
AAAntonio Abate
Antonio Abate
GBGiorgio Bardizza
Giorgio Bardizza
JBJoseph J. Berry
Joseph J. Berry
MLMonica Lira-Cantu
Monica Lira-Cantu
Improving the long-term stability of perovskite solar cells is critical to the deployment of this technology. Despite the great emphasis laid on stability-related investigations, publications lack consistency in experimental procedures and parameters reported. It is therefore challenging to reproduce and compare results and thereby develop a deep understanding of degradation mechanisms. Here, we report a consensus between researchers in the field on procedures for testing perovskite solar cell stability, which are based on the International Summit on Organic Photovoltaic Stability (ISOS) protocols. We propose additional procedures to account for properties specific to PSCs such as ion redistribution under electric fields, reversible degradation and to distinguish ambient-induced degradation from other stress factors. These protocols are not intended as a replacement of the existing qualification standards, but rather they aim to unify the stability assessment and to understand failure modes. Finally, we identify key procedural information which we suggest reporting in publications to improve reproducibility and enable large data set analysis.

8 June 2023 in Nature
Verified
Journal Article
Closed access
PDF file
RLRenxing Lin
Renxing Lin
YWYurui Wang
Yurui Wang
QLQianwen Lu
Qianwen Lu
BTBeibei Tang
Beibei Tang
JLJiayi Li
Jiayi Li
HTHairen Tan
Hairen Tan

9 June 2022 in Nature Energy
Verified
Journal Article
Closed access
PDF file
LLLudong Li
Ludong Li
YWYurui Wang
Yurui Wang
XWXiaoyu Wang
Xiaoyu Wang
RLRenxing Lin
Renxing Lin
XLXin Luo
Xin Luo
HTHairen Tan
Hairen Tan

20 April 2022 in Energy & Environmental Science
Verified
Journal Article
Closed access
PDF file
CHChengliang He
Chengliang He
YPYouwen Pan
Youwen Pan
YOYanni Ouyang
Yanni Ouyang
QSQing Shen
Qing Shen
YGYuan Gao
Yuan Gao
HCHongzheng Chen
Hongzheng Chen
A novel electron acceptor, BTP-H2, demonstrates a high efficiency of 18.5% with a high V oc of 0.932 V. It also enables the ternary device to yield an efficiency of 19.2%, ranking the highest among single-junction organic photovoltaics.

26 May 2022 in Science China Chemistry
Verified
Journal Article
Closed access
PDF file
YLYahui Liu
Yahui Liu
BLBowen Liu
Bowen Liu
CMChang-Qi Ma
Chang-Qi Ma
FHFei Huang
Fei Huang
GFGuitao Feng
Guitao Feng
ZBZhishan Bo
Zhishan Bo

21 April 2023 in Nature Communications
Verified
Journal Article
Open access
PDF file
LTLingfei Tang
Lingfei Tang
BCBowen Chen
Bowen Chen
ZZZhonghan Zhang
Zhonghan Zhang
CMChang-Qi Ma
Chang-Qi Ma
JCJunchao Chen
Junchao Chen
LCLiwei Chen
Liwei Chen
Solid polymer electrolytes (SPEs), which are favorable to form intimate interfacial contacts with electrodes, are promising electrolyte of choice for long-cycling lithium metal batteries (LMBs). However, typical SPEs with easily oxidized oxygen-bearing polar groups exhibit narrow electrochemical stability window (ESW), making it impractical to increase specific capacity and energy density of SPE based LMBs with charging cut-off voltage of 4.5 V or higher. Here, we apply a polyfluorinated crosslinker to enhance oxidation resistance of SPEs. The crosslinked network facilitates transmission of the inductive electron-withdrawing effect of polyfluorinated segments. As a result, polyfluorinated crosslinked SPE exhibits a wide ESW, and the Li|SPE|LiNi0.5Co0.2Mn0.3O2 cell with a cutoff voltage of 4.5 V delivers a high discharge specific capacity of ~164.19 mAh g−1 at 0.5 C and capacity retention of ~90% after 200 cycles. This work opens a direction in developing SPEs for long-cycling high-voltage LMBs by using polyfluorinated crosslinking strategy.