Recent research focuses on replacing metal current collectors with metallized polymer foils. However, this introduces significant challenges during cell production, as manufacturing steps must be adapted. Currently, copper is used as the current collector on the anode side and aluminum on the cathode side. These current collectors are then joined within the cell with an arrester tab. This step, known as contacting, is carried out industrially in pouch cells using ultrasonic welding or laser beam welding. However, since the polymer foil is electrically insulating, the current contacting procedures cannot be directly transferred to the metal–polymer current collectors. In this work, ultrasonic welding, laser beam welding, and a mechanical contacting method are considered, and the challenges arising from the material properties are highlighted. The properties of the joints are discussed as a function of the number of foils and the coating thickness of the metallization. It is demonstrated that successful contacting by ultrasonic welding and mechanical clamping is possible, as both mechanical strength and electrical conductivity are ensured by the joint. Laser beam welding was unsuccessful. Additionally, the electrical resistance is one to two orders of magnitude higher than that of pure aluminum and copper foils, which necessitates further optimization. Furthermore, ultrasonic welding is limited to welding 16 foils or fewer. This does not match industrial requirements. Consequently, novel approaches for contacting metal–polymer current collectors are required.

The transition to high-energy-density lithium metal batteries (LMBs) is essential for advancing electric vehicle (EV) technologies beyond the limitations of conventional lithium-ion batteries. A key challenge in scaling LMB production is the precise, contamination-free separation of lithium metal (LiM) anodes, hindered by lithium’s strong adhesion to mechanical cutting tools. This study investigates high-speed, contactless laser cutting as a scalable alternative for shaping double-coated LiM anodes. The effects of pulse duration, pulse energy, repetition frequency, and scanning speed were systematically evaluated using a nanosecond pulsed laser system on 30 µm LiM foils laminated on both sides of an 8 µm copper current collector. A maximum single-pass cutting speed of 3.0 m/s was achieved at a line energy of 0.06667 J/mm, with successful kerf formation requiring both a minimum pulse energy (>0.4 mJ) and peak power (>2.4 kW). Cut edge analysis showed that shorter pulse durations (72 ns) significantly reduced kerf width, the heat-affected zone (HAZ), and bulge height, indicating a shift to vapor-dominated ablation, though with increased spatter due to recoil pressure. Optimal edge quality was achieved with moderate pulse durations (261–508 ns), balancing energy delivery and thermal control. These findings define critical laser parameter thresholds and process windows for the high-speed, high-fidelity cutting of double-coated LiM battery anodes, supporting the industrial adoption of nanosecond laser systems in scalable LMB electrode manufacturing.