We report on the observation of an approximately linear reduction in the maximum operating temperature with an increasing emission frequency for terahertz quantum-cascade lasers between 4.2 and 5.4 THz. These lasers are based on the same design type, but vary in period length and barrier height for the cascade structure. The sample emitting at the highest frequency around 5.4 THz can be operated in pulsed mode up to 56 K. We identify an additional relaxation channel for electrons by longitudinal optical phonon scattering from the upper to the lower laser level and increasing optical losses toward higher frequencies as major processes, leading to the observed temperature behavior.

We report on a fast self-mixing approach for real-time, coherent terahertz imaging based on a quantum-cascade laser and a scanning mirror. Due to a fast deflection of the terahertz beam, images with frame rates up to several Hz are obtained, eventually limited by the mechanical inertia of the employed scanning mirror. A phase modulation technique allows for the separation of the amplitude and phase information without the necessity of parameter fitting routines. We further demonstrate the potential for transmission imaging.

We have realized GaAs/AlAs quantum-cascade lasers operating at 4.75 THz exhibiting more than three times higher wall plug efficiencies than GaAs/Al0.25Ga0.75As lasers with an almost identical design. At the same time, the threshold current density at 10 K is reduced from about 350 A/cm2 for the GaAs/Al0.25Ga0.75As laser to about 120 A/cm2 for the GaAs/AlAs laser. Substituting AlAs for Al0.25Ga0.75As barriers leads to a larger energy separation between the subbands reducing the probability for leakage currents through parasitic states and for reabsorption of the laser light. The higher barriers allow for a shift of the quasi-continuum of states to much higher energies. The use of a binary barrier material may also reduce detrimental effects due to the expected composition fluctuations in ternary alloys.

GaAs-based terahertz quantum-cascade lasers (QCLs) are continuously tuned in their emission frequency by illuminating the rear facet with a near-infrared, high-power diode laser. For QCLs emitting around 3.1 THz, the maximum tuning range amounts to 2.8 GHz for continuous-wave operation at a heat sink temperature of 55 K, while in pulsed mode 9.1 and 8.0 GHz are achieved at 35 and 55 K, respectively.

We demonstrate the feasibility of high-resolution terahertz gas spectroscopy based on the external optical feedback effect in a quantum-cascade laser. Tuning the frequency of the quantum-cascade laser across a molecular absorption line of CH₃OH leads to a reduction of the optical feedback, which can be detected by monitoring the voltage across the quantum-cascade laser. This method provides a high spectral resolution of $\nu /\Delta \nu ={10}^6$ and a sensitivity comparable to that obtained with a cryogenically cooled Ge:Ga photoconductive detector.

Efficient and compact frequency converters are essential for frequency stabilization of terahertz sources. In this article, we present a ${3.5}$ -THz, ${\times 6}$ -harmonic, integrated Schottky diode mixer operating at room temperature. The designed frequency converter is based on a single-ended, planar Schottky diode with a submicron anode contact area defined on a suspended 2- ${\mu }$ m ultra-thin gallium arsenide substrate. The dc-grounded anode pad was combined with the radio frequency E-plane probe, which resulted in an electrically compact circuit. At $\text{200}$ -MHz intermediate frequency, a mixer conversion loss of about $\text{59}$ dB is measured resulting in a ${40}$ -dB signal-to-noise ratio for phase locking a ${3.5}$ -THz quantum-cascade laser. Using a quasi-static diode model combined with electromagnetic simulations, good agreement with the measured results was obtained. Harmonic frequency converters without the need of cryogenic cooling will help in the realization of highly sensitive space and air-borne heterodyne receivers.