Microfluidic devices and micro-pumps are increasingly necessitated in many fields ranging from untethered soft robots, to pharmaceutical and biomedical technology. While realization of such devices is limited by miniaturization constraints of conventional actuators, these restrictions can be resolved by using smart material transducers instead. This paper proposes and investigates the first ionic polymer metal composite (IPMC) actuator-driven linear peristaltic pump. With the aim of designing a monolithic device, our concept is based on a single IPMC actuator that is etched on both sides and cut with kirigami-inspired slits by laser ablation. Our pump has a planar configuration, operates with low activation voltages (< 5 V) and is simple to manufacture and thus miniaturize. We build proof-of-principle prototypes of an open and closed design of our proposed pump concept, model the closed design, and evaluate both configurations experimentally. Results show the feasibility of the proposed IPMC-driven pump. Without any optimization, the open pump achieved pumping rates of 669 pL/s, while the closed pump configuration attained a 4.57 Pa pressure buildup and 9.18 nL/s pumping rate. These results indicate feasibility of the concept, and future work will focus on design optimization.

Excellent conductivity makes silver (Ag) an attractive electrode and current collector material for a variety of devices, also promising faster soft actuators. However, high reactivity challenges the use of Ag in electrochemical systems, as dendritic growth can create undesired conduction pathways and short‐circuit the oppositely polarized electrodes. The challenge of rapid Ag electrochemical migration is addressed using a mixed mixed‐room temperature ionic liquid (RTIL) system (l‐ethyl‐3‐methylimidazolium bis‐(trifluoromethylsulfonyl)‐imide and trihexyl(tetradecyl)phosphonium chloride) that prevents short‐circuiting by engaging the produced Ag⁺ ions with Cl⁻ anions. The stability of the system is demonstrated on an ionic actuator using Ag–silver chloride (AgCl) electrodes and a mixed‐RTIL electrolyte. The work demonstrates fast (in 5 s) transfer of a large (0.2 C cm⁻²) charge to high‐specific‐surface‐area carbon without observable dendritic growth in cycling and good electromechanical performance: 4° s⁻¹ deflection rate at 0.8 V s⁻¹ scan rate. Simple spray‐deposition of the Ag–AgCl electrodes promises scalable and cost‐effective fabrication. The combination of high stability and vast charge capacity encourages the engagement of Ag‐based electrodes for many electrochemical applications involving organic electrolytes also beyond robotics.

Solid-state electromechanical smart material actuators are versatile as they permit diverse shapes and designs and can exhibit different actuation modes. An important advantage of these actuators compared to conventional ones is that they can be easily miniaturized to a sub-millimeter scale. In recent years, there has been a great surge in novel liquid pumps operated by these smart material actuators. These devices create opportunities for applications in fields ranging from aerospace and robotics to the biomedical and drug delivery industries. Although these have mainly been prototypes, a few products have already entered the market. To assist in the further development of this research track, we provide a taxonomy of the electromechanical smart material actuators available, and subsequently focus on the ones that have been utilized for operating pumps. The latter includes unidirectional shape memory alloy-, piezoelectric ceramic-, ferroelectric polymer-, dielectric elastomer-, ionic polymer metal composite- and conducting polymer-based actuators. Their properties are reviewed in the context of engineering pumps and summarized in comprehensive tables. Given the diverse requirements of pumps, these varied smart materials and their actuators offer exciting possibilities for designing and constructing devices for a wide array of applications.