The durability of piezoresistive sensor materials is a core prerequisite for their implementation in structural health monitoring systems. In this work, three piezoresistive materials were subjected to extensive cyclic tensile loadings, and their behaviour was analysed before, after, and during testing. To this end, aluminium specimens were coated with three different industry-grade lacquers, and then piezoresistive materials were applied onto each specimen. Sensors made from carbon black displayed excellent linearity even after tensile loading cycles ($R^2>0.88$). A decline in linearity of all sensors based on carbon allotropes was discovered, whereas the polymer-based sensors improved. Furthermore, their adhesion to the substrate is of great importance. Good adhesion ensures the strains in the underlying structure are correctly transmitted into the sensor materials. Based on contact angle measurements of liquids on sensor materials and on lacquers, their work of adhesion was determined. The findings were verified by tape adhesion tests.