The aim of this study was to characterise the microstructural organisation of staple carbon fibre-reinforced polymer composites and to investigate their mechanical properties. Conventionally, fibre-reinforced materials are manufactured using continuous fibres. However, discontinuous fibres are crucial for developing sustainable structural second-life applications. Specifically, aligning staple fibres into yarn or tape-like structures enables similar usage to continuous fibre-based products. Understanding the effects of fibre orientation, fibre length, and compaction on mechanical performance can facilitate the fibres’ use as standard engineering materials. This study employed methods ranging from microscale to macroscale, such as image analysis, X-ray computed tomography, and mechanical testing, to quantify the microstructural organisations resulting from different alignment processing methods. These results were compared with the results of mechanical tests to validate and comprehend the relationship between fibre alignment and strength. The results show a significant influence of alignment on fibre orientation distribution, fibre volume fraction, tortuosity, and mechanical properties. Furthermore, different characteristics of the staple fibre tapes were identified and attributed to kinematic effects during movement of the sliver alignment unit, resulting in varying tape thicknesses and fuzzy surfaces.

Carbon staple fiber composites are materials reinforced with discrete-length carbon fibers processed using traditional textile technologies, offering moderate mechanical properties and flexibility in manufacturing. These composites can be produced from recycled carbon staple fibers, aligned into yarn and tape-like structures, providing a more sustainable alternative while balancing performance, cost-effectiveness, and environmental impact. Aligning staple fibers into tape-like structures enables similar applications to those of continuous-fiber-based products, while allowing control over fiber orientation distribution, fiber volume fraction, and length distribution, which are all critical factors influencing both mechanical and thermo-mechanical properties. This study focuses on the experimental characterization and numerical investigation of Coefficients of Thermal Expansion (CTEs) in aligned carbon staple fiber composites. The effects of fiber orientation and volume fraction on coefficients of thermal expansion under different fiber alignment parameters are analyzed, revealing distinct thermal expansion behavior compared to typical aligned unidirectional continuous carbon fiber composite laminates. Unlike continuous unidirectional laminates, which typically exhibit transversely isotropic behavior without tensile–shear coupling, staple fiber composites demonstrate different in-plane axial, transverse, and out-of-plane CTE characteristics. To explain these deviations, a modeling approach is introduced, incorporating detailed experimental information on fiber distributions and microstructural features rather than averaged fiber orientation values. This involves a multi-scale analysis based on a laminate analogy through which all composite thermo-elastic properties can be predicted, accounting for variations in fiber orientations, volume fractions, and tape thicknesses. It is shown that while the local variation of fiber volume fraction has a small effect on the homogenized value of the coefficients of thermal expansion, fiber misalignment, tape thickness, and asymmetry in fiber orientation distribution will significantly affect the measurements of CTEs. For the case of carbon staple fiber composites, the asymmetry in fiber orientation distribution significantly influences the measurements of axial CTE. Fiber orientation asymmetry causes tensile–shear coupling under mechanical and thermal loading, leading to an unbalanced laminate with in-plane shear–tensile deformation. This coupling disrupts uniform displacement, complicating strain measurements and the determination of composite properties.

Short carbon fiber-reinforced bio-based polyamide 11 (PA11) composites were developed in filament form for Additive Fusion Technology (AFT) 3D printing and benchmarked against injection-molded samples. Composites containing 15 and 25 weight percent (wt%) recycled carbon fibers (rCFs) were successfully extruded into 1.75 mm diameter filaments, whereas higher fiber contents (35 wt%) led to brittle filament failure. AFT printing with subsequent consolidation produced short fiber composites with highly aligned fibers, while injection molding generated more randomly oriented microstructures. Mechanical testing revealed that AFT-printed composites in the fiber direction achieved significantly higher stiffness and comparable tensile strength to injection-molded counterparts. At 25 wt% fiber content, AFT 0° specimens reached an axial tensile modulus of 14.5 GPa, about 32% higher than injection-molded samples (11.0 GPa), with similar axial tensile strength (~123 vs. 126 MPa). However, AFT specimens displayed pronounced anisotropy: transverse (90°) properties dropped to ~2.3 GPa for transverse modulus and ~46–50 MPa transverse tensile strength, near matrix-dominated levels. Impact testing showed orientation-dependent toughness, with AFT 90° samples at 15% fiber content achieving the highest impact energy (76 kJ·m⁻²), while AFT 0° samples were ~30% lower than injection-molded equivalents. Dynamic mechanical analysis confirmed that AFT 0° composites maintained higher stiffness up to ~80 °C. Overall, these results demonstrate that aligned short fiber filaments enable high stiffness and strength performance comparable to injection molding, with the trade-off of anisotropy that must be carefully considered in design. This study is the first to demonstrate the feasibility of combining bio-based PA11 with recycled short carbon fibers in AFT printing, thereby extending additive manufacturing to sustainable and high-stiffness short fiber composites.

The aim of this study was to explore the compactibility of unidirectional staple carbon fibre laminates in comparison with their uni- and biaxial continuous fibre counterparts. Resin-preimpregnated plies were inserted into a heated compression mould at an elevated mould temperature of 110 °C. By applying stepwise loading, the correlation between consolidation pressure and fibre volume content was derived and related to fibre orientation distribution. The fibre orientation distribution is obtained from photographic image analyses of 2D ply sections of the same samples using the structure tensor approach. For commonly used autoclave prepreg pressure of 6.8 bar results indicate that lower-oriented staple carbon fibre unidirectional laminates with a fibre orientation distribution factor η₀ = 0.74 can potentially reach a maximum of 39% fibre volume fraction, while higher-oriented laminates with η₀ = 0.78 end up at 43%. An exponential extrapolation suggests that a consolidation pressure of ≥90 bar is required to achieve 60% fibre volume content with highly oriented unidirectional staple carbon fibre laminates.

The increasing availability of recycled carbon fibres (rCFs) from manufacturing waste and end-of-life composite structures offers new opportunities for sustainable, high-performance composites. However, the discontinuous nature of recycled fibres requires efficient alignment and consolidation. In this study, highly aligned discontinuous carbon fibre tapes were manufactured from recycled carbon staple fibres and bio-based polyamide 11 (PA11) fibres using a textile-based processing route and compression moulding. Two material systems containing nominal fibre mass fractions of 50 wt.% and 70 wt.% rCF were investigated. The resulting laminates were characterised in terms of fibre volume content (FVC), fibre orientation distribution, and mechanical performance. FVC of up to 56.72 vol.% were achieved for the 70 wt.% rCF material. Tensile testing revealed a significant increase in stiffness and strength with increasing fibre content, reaching values of 48.1 GPa and 866 MPa. The longitudinal compression modulus and the in-plane shear modulus showed similar trends, while the transverse tensile strength and compressive strength remained strongly influenced by local defects and fibre–matrix interactions. A 2D mesoscopic image analysis demonstrated a pronounced preferential fibre orientation, with approximately 69% of the analysed fibre regions aligned within ±10° of the dominant fibre direction. The derived alignment coefficient η₀ correlated well with the tensile modulus, confirming the strong influence of mesoscopic fibre architecture on mechanical performance. The results demonstrate that the combination of bio-based PA11 and oriented rCF, enabled through textile-based alignment technologies, provides a promising pathway towards sustainable lightweight composite structures.

Aligned recycled carbon fiber (rCF)/polyetherimide (PEI) tapes are a promising material for lightweight aerospace thermoplastic composite structures with reduced environmental impact, provided that their directional properties can be translated into robust components. To assess the viability of rCF/PEI for aircraft interior applications, this study tracks the development of the “Eco Bracket” across four key stages: sustainability screening, coupon characterization, microstructural interpretation, and application-level structural assessment. A project-level life-cycle assessment compared an Additive Fusion Technology (AFT) rCF/PEI bracket with cast and milled aluminum routes and yielded a short-term climate impact of 0.678 kg CO₂-eq for rCF/PEI, representing a significant reduction compared to 5.1 kg CO₂-eq for cast aluminum and 20.9 kg CO₂-eq for milled aluminum. Coupon testing characterized the anisotropic mechanical response of the rCF/PEI tape, including the elastic moduli and strengths under axial and transverse tension, in-plane shear, and axial and transverse compression. Scanning electron microscopy of a representative fracture surface showed a rough, fiber-dominated morphology with exposed fiber bundles, pull-out, and local variations in matrix coverage, supporting the interpretation that consolidation and local wet-out quality govern the transfer from coupon capability to component performance. At the application level, the manufactured rCF/PEI bracket achieved a peak load of 3517.6 N, corresponding to 93% of the strength of an industry-standard polyetherketoneketone (PEKK) reference bracket, and failed in the fastener-hole region predicted as critical by the finite element model. The combined results indicate that aligned rCF/PEI tapes can deliver mechanical properties consistent with the design requirements of aircraft interior brackets, while process robustness, fiber-path fidelity, and local consolidation quality remain the key barriers to repeatable component performance.