Sedimentation can cause numerous problems in rivers, estuaries, harbors, and coastal areas. It is therefore important to trace and model the movement of sediments. The natural physical, chemical, and biological components of the aquatic sediment generally relate to these features in its terrestrial catchment area. It consequently contains the naturally occurring radionuclides of thorium, uranium, and potassium, which can be used as tracers. To achieve this aim, a delta underwater gamma system (DUGS) was developed to map the radionuclides in aquatic sediments. Though the system has been tested for radiometric accuracy, the low concentrations of natural radionuclides in aquatic sediments and the attenuation by the water and detector enclosure necessitated an evaluation to determine the detection efficiency of the detector along with optimal operational parameters. These included spectra accumulation time and underwater speed. The DUGS was consequently used to determine and optimize these parameters for mobile measurement of aquatic sediments. The acquired gamma spectra were also analyzed using full spectrum and energy window analysis to determine the optimal method for extracting the activity concentrations of the nuclides in the sediments.
10 December 2022 in Journal of Radioanalytical and Nuclear Chemistry
This study reports on natural radioactivity levels and radiation risk estimates from soil samples collected in five villages near the Manyoni Uranium Deposit in central Tanzania. The mean activity concentrations of 40K, 232Th, and 238U were 207 Bq kg−1, 78 Bq kg−1, and 302 Bq kg−1, respectively. While 40K levels were below the world average, the levels of 232Th and 238U were more than 1.7 and 9.2 times higher than world average values. The average absorbed dose rate for the area was 196 nSv h−1. Annual effective dose estimate values for outdoor and indoor exposure were 0.24 mSv and 0.96 mSv, respectively, exceeding global averages by 3.4 and 2.3 times. Based on the average external hazard index (Hex = 1.19) and excess lifetime cancer risk (ELCR = 0.46%), there is a potential risk of radiological effects from radiation exposure, with Mwanzi Village identified as a high background radiation area.
This study was realized in the frame of an IAEA Coordinated Research Project for the evaluation of sediment dynamics, applying in-situ radiometric methods accompanied with a theoretical model. The in-situ methods were validated using lab-based high-resolution gamma-ray spectrometry. Sediment dynamics assessments were performed based on the measured and mapped activity concentrations of specific 238U progenies (214Bi or 214Pb), 232Th progenies (208Tl and 228Ac), and 40K along the shoreline of the beach. The maps of the activity concentrations of natural radionuclides were produced rapidly using software tools (R language v4.5). The sediment dynamics of the studied area were also investigated through numerical simulations, applying an open source model considering land–sea interactions and meteorological conditions and the corresponding sediment processes. The assessments, which were conducted utilizing the detailed data from the natural radioactivity maps, were validated by the simulation results, since both were found to be in agreement. Generally, it was confirmed that the distribution of radionuclides reflects the selective transport processes of sediments, which are related to the corresponding processes that occur in the study area. Legrena Beach in Attica, Greece, served as a pilot area for the comparative analysis of methods and demonstration of their relevance and applicability for studying coastal processes.
5 December 2025 in Journal of Radioanalytical and Nuclear Chemistry