Fig. 1. Illustraion of the experimental setups of neutron tomography.

This study developed a high-temperature and high-pressure (HTHP) cell for in situ neutron imaging of hydrothermal reactions. The cell’s maximum temperature and pressure were 500 °C and 50 MPa, respectively, and its vessel for observing reactions comprised SUS316 stainless steel. Neutron transmission images were obtained to observe the behavior of sub- and supercritical water and the decomposition of two plastics (polypropylene and polyethylene) at HTHP. The images showed that water’s density and phase changed with temperature and pressure, affecting neutron transmission (and thus image brightness). The plastics began to melt and change shape at 150–200 °C, and they decomposed at 500 °C and 20 MPa. This study provides a basis for future research using the HTHP cell to examine various reactions such as the decomposition of biomass samples, the reforming of heavy oil, and the synthesis of nano-materials using sub- and supercritical water.

This study presents a significant development in the Energy-Resolved Neutron Imaging System RADEN, in the Japan Proton Accelerator Research Complex, Japan. Through a systematic study, the collimation power of the facility was reevaluated. What was initially considered to be values of 230, 420, and 760 have been proven to be much higher. To perform the calculation of the L/D factor of the beam, a state-of-the-art method has been used, along with a standard reference sample to measure the resolution of neutron images. To add robustness to the results, the study compares five different scintillators of different composition and thickness [6LiF:ZnS(Ag) of 50, 100, 200, and 300 μm and Gd2O2S of 50 μm]. The calculated collimating power of the beam ranges between 470 and 1520. These results place a spotlight on an existing discrepancy between the geometrically calculated L/D and the actual measurable quantity, as well as highlight the superior performance of the RADEN beamline.

Japanese swords have a history of more than one thousand years and are recognized as metallic art objects. The sword-making process is not clearly understood, especially for old swords made before about 1600 A.D. Knowledge of structural information such as crystallite sizes and anisotropy is important to understand the sword characteristics and the sword-making process. Bragg-edge transmission imaging is a useful noninvasive method that can extract this structural information continuously over a wide area of the sword. Neutron CT is powerful enough to detect quenched areas, voids, and precipitates. Using both methods, we measured more than 10 swords and obtained information on the two-dimensional crystallite size distribution, anisotropy parameter, lattice plane spacing, and quenched regions. Comparison of the results indicated the following features: the crystallite size distributions showed two patterns: an almost uniform distribution of small-sized crystallites, and mixed distributions of large- and small-sized crystallites. The patterns were observed in different eras and places. The preferred orientation showed different patterns, and strain areas due to quenching were observed in many swords. The quenched area showed a trend that the quenching was weaker for old swords than newer ones. CT images showed the boundaries of the quenched regions and a void in the layered structure for one sword, for which a layered structure was confirmed.