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Yanqiu Shao
Advanced Materials Institute, Qilu University of Technology (Shandong Academy of Sciences), Jinan 250014, China

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Journal article
Published: 22 December 2020 in Polymers
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In this study, a type of alkaline solid polyelectrolyte (ASPE) membrane was developed via the introduction of microcrystalline cellulose (MCC) and its modified product (QMCC) into the polyvinyl alcohol (PVA) matrix. In this process, green NaOH/urea-based solvent was used to achieve a good dispersion of MCC in the PVA matrix; meanwhile, the OH− groups in the NaOH/urea-based solvent provided an alkaline environment for good ion conductivity. Compared to the MCC-incorporated ASPE, further improved conductivity was achieved when the MCC was modified with quantitative quaternary ammonium salt. TGA showed that the addition of QMCC improved the water retention of the matrix, which was beneficial to the OH− conduction in the system. Compared to the control (50 mS cm−1), a maximum conductivity of 238 mS cm−1 was obtained after the incorporation of QMCC in the PVA matrix. Moreover, the tensile strength of the polymer electrolyte were also significantly increased with the addition of QMCC. Finally, this developed ASPE membrane was used in assembling a flexible Zn–air battery and showed a promising potential in the development of flexible electronic devices.

ACS Style

Xiang You; Congde Qiao; Dan Peng; Weiliang Liu; Cong Li; Hui Zhao; Hao Qi; Xiaoxia Cai; Yanqiu Shao; Xinhua Shi. Preparation of Alkaline Polyelectrolyte Membrane Based on Quaternary Ammonium Salt–Modified Cellulose and Its Application in Zn–Air Flexible Battery. Polymers 2020, 13, 9 .

AMA Style

Xiang You, Congde Qiao, Dan Peng, Weiliang Liu, Cong Li, Hui Zhao, Hao Qi, Xiaoxia Cai, Yanqiu Shao, Xinhua Shi. Preparation of Alkaline Polyelectrolyte Membrane Based on Quaternary Ammonium Salt–Modified Cellulose and Its Application in Zn–Air Flexible Battery. Polymers. 2020; 13 (1):9.

Chicago/Turabian Style

Xiang You; Congde Qiao; Dan Peng; Weiliang Liu; Cong Li; Hui Zhao; Hao Qi; Xiaoxia Cai; Yanqiu Shao; Xinhua Shi. 2020. "Preparation of Alkaline Polyelectrolyte Membrane Based on Quaternary Ammonium Salt–Modified Cellulose and Its Application in Zn–Air Flexible Battery." Polymers 13, no. 1: 9.

Journal article
Published: 14 November 2018 in International Journal of Environmental Research and Public Health
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Composted sewage sludge (CSS) has been extensively used in agriculture and landscaping, offering a practical solution for waste disposal. However, some pharmaceutical and personal care products (PPCPs) like triclosan (TCS) and carbamazepine (CBZ) have restricted its land application. In this study, CSS was added to agricultural soil and garden soil at 0%, 5%, 10%, and 25% (w/w soil), and 4 mL of TCS and CBZ stock solution (1000 mg/L in methanol) was spiked into soil amended with CSS of each bottle to arrive at the concentration of 10 mg/kg. Samples were then collected after incubation for 120 days and analyzed for concentrations and half-life (t1/2) of TCS and CBZ, and soil physicochemical properties, together with enzyme activities. The results showed that TCS was degraded completely during the incubation period. In contrast, only about 5.82–21.43% CBZ was degraded. CSS amendment inhibited TCS and CBZ degradation and prolonged t1/2 compared to the control, and the t1/2 of TCS and CBZ increased with CSS addition amount in all treatments except for CBZ in the garden soil amended with 10% CSS. Correlation studies showed a significantly positive relationship between t1/2 of TCS and CBZ and total organic carbon (TOC), while a significantly negative relationship between t1/2 of the two PPCPs and pH was observed. Alkaline phosphatase showed a significantly negative relationship with the Ct/C0 of TCS in garden soil amended with 25% CSS and CBZ in the control. The urease activity was negatively correlated with the Ct/C0 of TCS in 10% and 25% CSS treatments and CBZ in 10% CSS treatment for garden soil.

ACS Style

Yanqiu Shao; Kai Yang; Rongchang Jia; Chao Tian; Ying Zhu. Degradation of Triclosan and Carbamazepine in Two Agricultural and Garden Soils with Different Textures Amended with Composted Sewage Sludge. International Journal of Environmental Research and Public Health 2018, 15, 2557 .

AMA Style

Yanqiu Shao, Kai Yang, Rongchang Jia, Chao Tian, Ying Zhu. Degradation of Triclosan and Carbamazepine in Two Agricultural and Garden Soils with Different Textures Amended with Composted Sewage Sludge. International Journal of Environmental Research and Public Health. 2018; 15 (11):2557.

Chicago/Turabian Style

Yanqiu Shao; Kai Yang; Rongchang Jia; Chao Tian; Ying Zhu. 2018. "Degradation of Triclosan and Carbamazepine in Two Agricultural and Garden Soils with Different Textures Amended with Composted Sewage Sludge." International Journal of Environmental Research and Public Health 15, no. 11: 2557.

Journal article
Published: 28 March 2018 in International Journal of Environmental Research and Public Health
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A composted sewage sludge (CSS) was added to the soil of an urban garden at 5%, 10%, and 25% (w/w soil) and stabilised for 180 days. Samples were then collected and analysed for total heavy metal concentrations, chemical fractions, and bioaccessibility, together with some physicochemical properties. The results showed that the total chromium (Cr), copper (Cu), lead (Pb), and zinc (Zn) concentrations were increased with CSS addition rate. The CSS addition decreased the residual fractions of these four elements. The exchangeable Cr, Cu, and Pb fractions were very small or not detected, while Zn exhibited an increasing trend in its exchangeable fraction with CSS addition rate. The bioaccessibility of these four elements was increased with the CSS addition rate. Moreover, the Cr, Cu, and Zn bioaccessibility correlated positively with the total concentration, while the bioaccessibility of these four elements exhibited a negative correlation with the residual fraction. The fractionation and bioaccessibility of heavy metals may have also been influenced by pH, cation exchange capacity, and organic matter. The risk assessment code reflected the amended soil showed no or low environmental risks for Cr, Cu, and Pb and a medium risk for Zn. The hazardous index values and cancer risk levels indicated that the heavy metals in the soil amended with 25% CSS posed negligible potential noncarcinogenic and carcinogenic risks to children and adults via incidental ingestion.

ACS Style

Kai Yang; Tao Zhang; Yanqiu Shao; Chao Tian; Stephen R. Cattle; Ying Zhu; Jinjuan Song. Fractionation, Bioaccessibility, and Risk Assessment of Heavy Metals in the Soil of an Urban Recreational Area Amended with Composted Sewage Sludge. International Journal of Environmental Research and Public Health 2018, 15, 613 .

AMA Style

Kai Yang, Tao Zhang, Yanqiu Shao, Chao Tian, Stephen R. Cattle, Ying Zhu, Jinjuan Song. Fractionation, Bioaccessibility, and Risk Assessment of Heavy Metals in the Soil of an Urban Recreational Area Amended with Composted Sewage Sludge. International Journal of Environmental Research and Public Health. 2018; 15 (4):613.

Chicago/Turabian Style

Kai Yang; Tao Zhang; Yanqiu Shao; Chao Tian; Stephen R. Cattle; Ying Zhu; Jinjuan Song. 2018. "Fractionation, Bioaccessibility, and Risk Assessment of Heavy Metals in the Soil of an Urban Recreational Area Amended with Composted Sewage Sludge." International Journal of Environmental Research and Public Health 15, no. 4: 613.

Journal article
Published: 01 March 2017 in Journal of Environmental Management
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Sanitary landfill persists as a predominant sludge disposal method in particular in China. In this study, successive subsurface sludge samples (0.3 m deep) were collected from a bioreactor landfill unit where an anaerobic process took place during a 500 d period. The sludge samples were analyzed for total concentrations of cadmium (Cd), chromium (Cr), copper (Cu), nickel (Ni), lead (Pb) and zinc (Zn) and their species distributions, together with selected sludge chemical properties. In addition, the sludge samples were subjected to phytotoxicity testing. The results showed that the mobilities of Cd and Ni were decreased with landfill time, while the mobilities of Cr, Cu, Pb and Zn remained consistently low over the landfill period. The residual amounts of all these heavy metals were increased with landfill time, suggesting that the anaerobic sanitary landfill is an effective sludge stabilization method to reduce the ecological risk of these heavy metals. The increase in the sludge pH value with landfill time tended to promote the precipitation of heavy metals. Moreover, the sludge stabilization was found to be indicated by the formation of humic substance (HS) and volatilization of volatile matter (VM). The germination index (GI) values of barley (Hordeum vulgare L.) and Chinese cabbage (Brassica rapa chinensis) seeds grown in the 500 d anaerobically stabilized sludge were approximately 5.2- and 4.1-times higher than the values of those grown in the fresh sludge. The final sludge extract did not cause any significant inhibitory effect on the germination of the two types of seeds.

ACS Style

Kai Yang; Ying Zhu; Ranran Shan; Yanqiu Shao; Chao Tian. Heavy metals in sludge during anaerobic sanitary landfill: Speciation transformation and phytotoxicity. Journal of Environmental Management 2017, 189, 58 -66.

AMA Style

Kai Yang, Ying Zhu, Ranran Shan, Yanqiu Shao, Chao Tian. Heavy metals in sludge during anaerobic sanitary landfill: Speciation transformation and phytotoxicity. Journal of Environmental Management. 2017; 189 ():58-66.

Chicago/Turabian Style

Kai Yang; Ying Zhu; Ranran Shan; Yanqiu Shao; Chao Tian. 2017. "Heavy metals in sludge during anaerobic sanitary landfill: Speciation transformation and phytotoxicity." Journal of Environmental Management 189, no. : 58-66.