A method for measuring the interactions of charged dust particles within a three-dimensional dust cloud in a plasma is presented. The measurements have been performed with the help of gravity-driven heavy charged probe particles, which moved through a dust cloud levitating at the diffuse edge of an inductively coupled rf discharge plasma. Assuming a screened Coulomb potential surrounding each particle, both the particle charge and the effective screening length were calculated from an analysis of the elastic particle interactions for 20, 30, and 50 Pa of neon pressure. The basic parameters of the bulk discharge plasma have been diagnosed with a Langmuir probe to compare the experimental data with those deriving from different theoretical approaches. The observed discrepancies are discussed.
Experimental data on the active Brownian motion of single particles in the RF (radio-frequency) discharge plasma under the influence of thermophoretic force, induced by laser radiation, depending on the material and type of surface of the particle, are presented. Unlike passive Brownian particles, active Brownian particles, also known as micro-swimmers, move directionally. It was shown that different dust particles in gas discharge plasma can convert the energy of a surrounding medium (laser radiation) into the kinetic energy of motion. The movement of the active particle is a superposition of chaotic motion and self-propulsion.
Various self-excited motions in dusty plasmas involving spatial variations of macroparticle charge are considered. Two basic types of instabilities in these systems are examined numerically and analytically. The main attention is given to the vortex motions of macroparticles. Conditions suitable for creating the instabilities examined are discussed. Experimental observations of self-excited oscillations in dc-glow, and capacitive rf, discharges are presented. It is shown that spatial variation of dust charge can account for many phenomena observed in inhomogeneous laboratory dusty plasmas.
Three-dimensional structure of complex (dusty) plasmas was investigated under long-term microgravity conditions in the Plasmakristall-4 facility on the International Space Station. The microparticle suspensions were confined in a polarity-switched dc discharge. The experimental results were compared to the results of the molecular dynamics simulations with the interparticle interaction potential represented as a superposition of isotropic Yukawa and anisotropic quadrupole terms. Both simulated and experimental data exhibited qualitatively similar structural features, indicating the bulk liquid-like order with the inclusion of solid-like strings aligned with the axial electric field. Individual strings were identified and their size spectrum was calculated. The decay rate of the size spectrum was found to decrease with the enhancement of string-like structural features.
1 June 2022 in Physical Chemistry Chemical Physics
Overdamped active Brownian motion of self-propelled particles in a liquid has been fairly well studied. However, there are a variety of situations in which the overdamped approximation is not justified, for instance, when self-propelled particles move in a low-viscosity medium or when their rotational diffusivity is enhanced by internal active processes or external control. Examples of various origins include biofilaments driven by molecular motors, living and artificial microflyers and interfacial surfers, field-controlled and superfluid microswimmers, vibration-driven granular particles and autonomous mini-robots with sensorial delays, etc. All of them extend active Brownian motion to the underdamped case, i.e., to active Langevin motion, which takes into account inertia. Despite a rich experimental background, there is a gap in the theory in the field where rotational inertia significantly affects the random walk of active particles on all time scales. In particular, although the well-known models of active Brownian and Ornstein–Uhlenbeck particles include a memory effect of the direction of motion, they are not applicable in the underdamped case, because the rotational inertia, which they do not account for, can partially prevent “memory loss” with increasing rotational diffusion. We describe the two-dimensional motion of a self-propelled particle with both translational and rotational inertia and velocity fluctuations. The proposed generalized analytical equations for the mean kinetic energy, mean-square displacement and noise-averaged trajectory of the self-propelled particle are confirmed by numerical simulations in a wide range of self-propulsion velocities, moments of inertia, rotational diffusivities, medium viscosities and observation times.