Biomimetic pectoral fin propulsion offers a low-noise, highly maneuverable alternative to conventional propellers for next-generation underwater robotic systems. This study develops a manta ray-inspired dual-servo pectoral fin module with a CPG-based controller and employs it as a single-fin test article in a recirculating water tunnel to quantify its hydrodynamic performance. Controlled experiments demonstrate that the fin generates stable thrust over a range of flapping amplitudes, with mean thrust increasing markedly as the amplitude rises, while also revealing an optimal frequency band in which thrust and thrust work are maximized and beyond which efficiency saturates. To interpret these trends, a quasi-steady CFD analysis using the k–ω SST turbulence model is conducted for a series of static angles of attack representative of the instantaneous effective angles experienced during flapping. The simulations show a transition from attached flow with favorable lift-to-drag ratios at moderate angles of attack to massive separation, deep stall, and high drag at extreme angles, corresponding to high-amplitude fin motion. By linking the experimentally observed thrust saturation to the onset of deep stall in the numerical flow fields, this work establishes a unified experimental–numerical framework that clarifies the hydrodynamic limits of pectoral fin propulsion and provides guidance for the design and operation of low-noise, highly maneuverable biomimetic underwater robots.