The extremely neutron-rich nucleus has been studied by Coulomb dissociation into at . A large strength of has been observed at low excitation energies. An analysis of the angular distribution of center of mass has led to a determination of the neutron separation energy of to be . The strength distribution can be well reproduced for a ground state structure with a dominant -wave valence neutron, providing a consistent picture of the neutron halo structure of .
Absolute cross sections for isotopically identified products formed in multinucleon transfer in the system at are reported. The isotopic distributions obtained using a large acceptance spectrometer demonstrated the production of the “hard-to-reach” neutron-rich isotopes for around the shell closure far from stability. The main contribution to the formation of these exotic nuclei is shown to arise in collisions with a small kinetic energy dissipation. The present experimental finding corroborates for the first time recent predictions that multinucleon transfer reactions would be the optimum method to populate and characterize neutron-rich isotopes around which are crucial for understanding both astrophysically relevant processes and the evolution of “magic” numbers far from stability.
The masses of , , and the transfermium nuclei and , produced by hot- and cold-fusion reactions, in the vicinity of the deformed neutron shell closure, have been directly measured using a multireflection time-of-flight mass spectrograph. The masses of and were measured for the first time. Using the masses of as anchor points for decay chains, the masses of heavier nuclei, up to and , were determined. These new masses were compared with theoretical global mass models and demonstrated to be in good agreement with macroscopic-microscopic models in this region. The empirical shell gap parameter derived from three isotopic masses was updated with the new masses and corroborates the existence of the deformed neutron shell closure for Md and Lr.
The new isotope was synthesized and systematic atomic mass measurements of nineteen neutron-rich Pa-Pu isotopes were performed in the multinucleon transfer reactions of the system at the KISS facility. The present experimental results demonstrate the crucial role of the multinucleon transfer reactions for accessing unexplored neutron-rich actinide isotopes toward the shell gap in this region of nuclides.