Practical applications of next-generation stretchable electronics hinge on the development of sustained power supplies to drive highly sensitive on-skin sensors and wireless transmission modules. Although the manufacture of stretchable self-charging power units has been demonstrated by integrating stretchable energy harvesters and power management circuits with energy storage units, they often suffer from low and unstable output power especially under mechanical deformation and human movements, as well as complex and expensive fabrication processes. This work presents a low-cost, scalable, and facile manufacturing approach based on laser-induced graphene foams to yield a self-powered wireless sensing platform. 3D porous foams with high specific surface area and excellent charge transport provide an efficient flow of triboelectric electrons in triboelectric nanogenerators. The surface coating or doping with second laser irradiation on these foams can also form a 3D composite to provide high energy density in micro-supercapacitor arrays. The integration of a triboelectric nanogenerator and power management circuits with micro-supercapacitor arrays can efficiently harvest intermittent mechanical energy from body movements into stable power output. 3D foams and their composites patterned into various geometries conveniently create various deformable sensors on large scale at low cost. The generated stable, yet high, power with adjustable voltage and current outputs drives various stretchable sensors and wireless transmission modules to wirelessly measure pulse, strain, temperature, electrocardiogram, blood pressure, and blood oxygen. The self-powered, wireless, wearable sensing platform paves the way to wirelessly detect clinically relevant biophysical and biochemical signals for early disease diagnostics and healthy aging.
Multi‐functional actuation systems involve the mechanical integration of multiple actuation and sensor devices with external energy sources. The intricate combination makes it difficult to meet the requirements of lightweight. Hence, polypyrrole@graphene‐bacterial cellulose (PPy@G‐BC) films are proposed to construct multi‐responsive and bilayer actuators integrated with multi‐mode self‐powered sensing function. The PPy@G‐BC film not only exhibits good photo‐thermoelectric (PTE) properties but also possesses good hydrophilicity and high Young's modulus. Thus, the PPy@G‐BC films are used as active layers in multi‐responsive bilayer actuators integrated with self‐powered sensing functions. Here, two types of multi‐functional actuators integrated with self‐powered sensing functions is designed. One is a light‐driven actuator that realizes the self‐powered temperature sensing function through the PTE effect. Assisted by a machine learning algorithm, the self‐powered bionic hand can realize intelligent gesture recognition with an accuracy rate of 96.8%. The other is humidity‐driven actuators integrated a zinc‐air battery, which can realize self‐powered humidity sensing. Based on the above advantages, these two multi‐functional actuators are ingeniously integrated into a single device, which can simultaneously perform self‐powered temperature/humidity sensing while grasping objects. The highly integrated design enables the efficient utilization of environmental energy sources and complementary synergistic monitoring of multiple physical properties without increasing system complexity.