Long fiber-reinforced thermoplastics (LFTs) are an attractive design option for many engineering applications due to their excellent mechanical properties and processability. When processing these materials, the length of the fibers inevitably decreases, which ultimately affects the mechanical performance of the finished part. Since none of the existing modeling techniques can accurately predict fiber damage of LFTs during injection molding, a new phenomenological approach for modeling fiber attrition is presented. First, multiple controlled studies employing a Couette rheometer are performed to determine correlations between processing conditions, material properties, and fiber length reduction. The results show shear stress and fiber concentration impact fiber damage. Based on these findings, a phenomenological model to predict breaking rate and unbreakable length of a fiber under giving conditions is developed. The model is based on the beam theory with distributed hydrodynamic stresses acting on a fiber. Fiber–fiber interactions are accounted for and correlated with the fiber volume fraction via a fitting parameter. The model tracks both the number-average and weight-average fiber length during processing, which can in turn be used to extract the fiber length distribution.
Long fiber-reinforced thermoplastics are an attractive design option for many industries due to their excellent mechanical properties and processability. Processing of these materials has a significant influence on their microstructure, which controls the properties of the final part. The microstructure is characterized by the fibers’ orientation, length, and concentration. Many characterization methods can capture the fiber orientation and concentration changes through the thickness in injection molded parts, but not the changes in fiber length. In this study, a technique for measuring fiber length in the core and shell regions of molded parts was proposed, experimentally verified, and used on injection molded 20 wt.% glass fiber-reinforced polypropylene plaques. The measured fiber length in the core was 50% higher than in the shell region. Comparison with simulation results shows disagreement in the shape of the through-thickness fiber length profile. Stiffness predictions show that the through-thickness changes in fiber length have little impact on the longitudinal and transverse Young’s modulus.
Predicting the fiber orientation of reinforced molded components is required to improve their performance and safety. Continuum-based models for fiber orientation are computationally very efficient; however, they lack in a linked theory between fiber attrition, fiber–matrix separation and fiber alignment. This work, therefore, employs a particle level simulation which was used to simulate the fiber orientation evolution within a sliding plate rheometer. In the model, each fiber is accounted for and represented as a chain of linked rigid segments. Fibers experience hydrodynamic forces, elastic forces, and interaction forces. To validate this fundamental modeling approach, injection and compression molded reinforced polypropylene samples were subjected to a simple shear flow using a sliding plate rheometer. Microcomputed tomography was used to measure the orientation tensor up to 60 shear strain units. The fully characterized microstructure at zero shear strain was used to reproduce the initial conditions in the particle level simulation. Fibers were placed in a periodic boundary cell, and an idealized simple shear flow field was applied. The model showed a faster orientation evolution at the start of the shearing process. However, agreement with the steady-state aligned orientation for compression molded samples was found.
This study aims to use particle level simulation to simulate the breakage behavior of glass fibers subjected to simple shear flow. Each fiber is represented as a chain of rods that experience hydrodynamic, interaction, and elastic effects. In order to validate the approach of the model, the simulation results were compared to simple shear flow experiments conducted in a Couette Rheometer. The excluded volume force constants and critical fiber breakage curvature were tuned in the simulation to gain a better understanding of the system. Relaxation of the fiber clusters and a failure probability theory were introduced into the model to solve the fiber entanglement and thus, better fit the experimental behavior. The model showed agreement with the prediction on fiber length reduction in both number average length and weight average length. In addition, the simulation had a similar trend of breakage distribution compared to a loop test using glass fibers.
The simulative prediction of fiber orientation for injection-molded short fiber-reinforced thermoplastics is an important step in prediction warpage and failure of injection molded parts. There exists a variety of phenomenological macroscopic fiber orientation models, which are computationally very efficient but strongly dependent on phenomenological parameters. This research focuses on a mechanistic fiber orientation model for concentrated short fiber-reinforced thermoplastics. A fully coupled computational fluid dynamics particle simulation is used to estimate the lubrication forces between two fibers in different configurations (angles between fibers, velocities) with varying fiber length and surrounding fluid viscosity. Based on these data, a calibrated lubrication model is developed and implemented in a mechanistic fiber orientation simulation. In addition, the fiber orientation estimated by the enhanced mechanistic fiber model is compared to experimental fiber orientation data obtained with a glass fiber-reinforced thermoplastic industrial grade, which showed an improvement over a simulation that did not include the lubrication force.
Understanding the mechanics of fiber attrition during the extrusion process is highly important in predicting the strength of long fiber-reinforced thermoplastic composites. However, little work has been done to investigate the mechanics of fiber dispersion and its effects on fiber attrition. This study aims at investigating fiber dispersion in simple shear flows for long fiber-reinforced thermoplastic pellets. Depending on the fabrication process, fiber bundles display distinct levels of compaction within the pellets. Studies have shown that morphological differences can lead to differences in dispersion mechanics; therefore, using a Couette rheometer and a sliding plate rheometer, coated and pultruded pellets were subjected to simple shear deformation, and the amount of dispersion was quantified. Additionally, a new image-based analysis method is presented in this study to measure fiber dispersion for a multi-pellet-filled system. Results from the single-pellet dispersion study showed a small amount of correlation between the dimensionless morphological parameter and the dispersion measurement. Pultruded and coated pellets were both found to have similar dispersion rates in a multi-pellet system. However, pultruded pellets were found to have a higher dispersion value at all levels when compared with coated pellets in both dispersion studies.