The frequent occurrence of severe air pollution episodes in China has been a great concern and thus the focus of intensive studies. Planetary boundary layer height (PBLH) is a key factor in the vertical mixing and dilution of near-surface pollutants. However, the relationship between PBLH and surface pollutants, especially particulate matter (PM) concentration across China, is not yet well understood. We investigate this issue at ∼1600 surface stations using PBLH derived from space-borne and ground-based lidar, and discuss the influence of topography and meteorological variables on the PBLH–PM relationship. Albeit the PBLH–PM correlations are roughly negative for most cases, their magnitude, significance, and even sign vary considerably with location, season, and meteorological conditions. Weak or even uncorrelated PBLH–PM relationships are found over clean regions (e.g., Pearl River Delta), whereas nonlinearly negative responses of PM to PBLH evolution are found over polluted regions (e.g., North China Plain). Relatively strong PBLH–PM interactions are found when the PBLH is shallow and PM concentration is high, which typically corresponds to wintertime cases. Correlations are much weaker over the highlands than the plains regions, which may be associated with lighter pollution loading at higher elevations and contributions from mountain breezes. The influence of horizontal transport on surface PM is considered as well, manifested as a negative correlation between surface PM and wind speed over the whole nation. Strong wind with clean upwind air plays a dominant role in removing pollutants, and leads to obscure PBLH–PM relationships. A ventilation rate is used to jointly consider horizontal and vertical dispersion, which has the largest impact on surface pollutant accumulation over the North China Plain. As such, this study contributes to improved understanding of aerosol–planetary boundary layer (PBL) interactions and thus our ability to forecast surface air pollution.

The planetary boundary layer (PBL) governs the vertical transport of mass, momentum, and moisture between the surface and the free atmosphere, and thus the determination of PBL height (BLH) is recognized as crucial for air quality, weather, and climate analysis. Although reanalysis products can provide important insight into the global view of BLH in a seamless way, the BLH observed in situ on a global scale remains poorly understood due to the lack of high-resolution (1 or 2 s) radiosonde measurements. The present study attempts to establish a near-global BLH climatology at synoptic times (00:00 and 12:00 UTC) and in the daytime using high-resolution radiosonde measurements over 300 radiosonde sites worldwide for the period 2012 to 2019, which is then compared against the BLHs obtained from four reanalysis datasets, including ERA5, MERRA-2, JRA-55, and NCEP-2. The variations in daytime BLH exhibit large spatial and temporal dependence, and as a result the BLH maxima are generally discerned over the regions such as the western United States and western China, in which the balloon launch times mostly correspond to the afternoon. The diurnal variations in BLH are revealed with a peak at 17:00 local solar time (LST). The most promising reanalysis product is ERA5, which underestimates BLH by around 130 m as compared to radiosondes released during daytime. In addition, MERRA-2 is a well-established product and has an underestimation of around 160 m. JRA-55 and NCEP-2 might produce considerable additional uncertainties, with a much larger underestimation of up to 400 m. The largest bias in the reanalysis data appears over the western United States and western China, and it might be attributed to the maximal BLH in the afternoon when the PBL has risen. Statistical analyses further indicate that the biases of reanalysis BLH products are positively associated with orographic complexity, as well as the occurrence of static instability. To our best knowledge, this study presents the first near-global view of high-resolution radiosonde-derived boundary layer height and provides a quantitative assessment of the four frequently used reanalysis products.

Summer precipitation plays critical roles in the energy balance and the availability of fresh water over eastern China. However, little is known regarding the trend in local‐scale precipitation (LSP). Here we developed a novel method to determine LSP events in the summer afternoon throughout eastern China from 1970 to 2010 based on hourly gauge measurements. The LSP occurrence hours decrease at an annual rate of 0.25%, which varies considerably by region, ranging from 0.14% over the Yangtze River Delta to 0.56% over the Pearl River Delta. This declining frequency of LSP is generally accompanied by an increase in rain rate of LSP but a decrease in visibility, whose linkage to LSP events was investigated. In particular, more LSP events tended to form when the atmosphere was slightly polluted. Afterward, LSP was suppressed. These findings have important implications for improving our understanding of the climatology of daytime precipitation at local scales.

The aerosol–planetary boundary layer (PBL) interaction was proposed as an important mechanism to stabilize the atmosphere and exacerbate surface air pollution. Despite the tremendous progress made in understanding this process, its magnitude and significance still have large uncertainties and vary largely with aerosol distribution and meteorological conditions. In this study, we focus on the role of aerosol vertical distribution in thermodynamic stability and PBL development by jointly using micropulse lidar, sun photometer, and radiosonde measurements taken in Beijing. Despite the complexity of aerosol vertical distributions, cloud-free aerosol structures can be largely classified into three types: well-mixed, decreasing with height, and inverse structures. The aerosol–PBL relationship and diurnal cycles of the PBL height and PM_2.5 associated with these different aerosol vertical structures show distinct characteristics. The vertical distribution of aerosol radiative forcing differs drastically among the three types, with strong heating in the lower, middle, and upper PBL, respectively. Such a discrepancy in the heating rate affects the atmospheric buoyancy and stability differently in the three distinct aerosol structures. Absorbing aerosols have a weaker effect of stabilizing the lower atmosphere under the decreasing structure than under the inverse structure. As a result, the aerosol–PBL interaction can be strengthened by the inverse aerosol structure and can be potentially neutralized by the decreasing structure. Moreover, aerosols can both enhance and suppress PBL stability, leading to both positive and negative feedback loops. This study attempts to improve our understanding of the aerosol–PBL interaction, showing the importance of the observational constraint of aerosol vertical distribution for simulating this interaction and consequent feedbacks.