Air quality is concerned with pollutants in both the gas phase and solid or liquid phases. The latter are referred to as aerosols, which are multifaceted agents affecting air quality, weather and climate through many mechanisms. Unlike gas pollutants, aerosols interact strongly with meteorological variables with the strongest interactions taking place in the planetary boundary layer (PBL). The PBL hosting the bulk of aerosols in the lower atmosphere is affected by aerosol radiative effects. Both aerosol scattering and absorption reduce the amount of solar radiation reaching the ground and thus reduce the sensible heat fluxes that drive the diurnal evolution of the PBL. Moreover, aerosols can increase atmospheric stability by inducing a temperature inversion as a result of both scattering and absorption of solar radiation, which suppresses dispersion of pollutants and leads to further increases in aerosol concentration in the lower PBL. Such positive feedback is especially strong during severe pollution events. Knowledge of the PBL is thus crucial for understanding the interactions between air pollution and meteorology. A key question is how the diurnal evolution of the PBL interacts with aerosols, especially in vertical directions, and affects air quality. We review the major advances in aerosol measurements, PBL processes and their interactions with each other through complex feedback mechanisms, and highlight the priorities for future studies.

Fine particulate matter with aerodynamic diameters ≤2.5 µm (PM_2.5) has adverse effects on human health and the atmospheric environment. The estimation of surface PM_2.5 concentrations has made intensive use of satellite-derived aerosol products. However, it has been a great challenge to obtain high-quality and high-resolution PM_2.5 data from both ground and satellite observations, which is essential to monitor air pollution over small-scale areas such as metropolitan regions. Here, the space–time extremely randomized trees (STET) model was enhanced by integrating updated spatiotemporal information and additional auxiliary data to improve the spatial resolution and overall accuracy of PM_2.5 estimates across China. To this end, the newly released Moderate Resolution Imaging Spectroradiometer Multi-Angle Implementation of Atmospheric Correction AOD product, along with meteorological, topographical and land-use data and pollution emissions, was input to the STET model, and daily 1 km PM_2.5 maps for 2018 covering mainland China were produced. The STET model performed well, with a high out-of-sample (out-of-station) cross-validation coefficient of determination (R²) of 0.89 (0.88), a low root-mean-square error of 10.33 (10.93) µg m⁻³, a small mean absolute error of 6.69 (7.15) µg m⁻³ and a small mean relative error of 21.28 % (23.69 %). In particular, the model captured well the PM_2.5 concentrations at both regional and individual site scales. The North China Plain, the Sichuan Basin and Xinjiang Province always featured high PM_2.5 pollution levels, especially in winter. The STET model outperformed most models presented in previous related studies, with a strong predictive power (e.g., monthly R²=0.80), which can be used to estimate historical PM_2.5 records. More importantly, this study provides a new approach for obtaining high-resolution and high-quality PM_2.5 dataset across mainland China (i.e., ChinaHighPM_2.5), important for air pollution studies focused on urban areas.

The important roles of the planetary boundary layer (PBL) in climate, weather and air quality have long been recognized, but little is known about the PBL climatology in China. Using the fine-resolution sounding observations made across China and reanalysis data, we conducted a comprehensive investigation of the PBL in China from January 2011 to July 2015. The boundary layer height (BLH) is found to be generally higher in spring and summer than that in fall and winter. The comparison of seasonally averaged BLHs derived from observations and reanalysis, on average, shows good agreement, despite the pronounced inconsistence in some regions. The BLH, derived from soundings conducted three or four times daily in summer, tends to peak in the early afternoon, and the diurnal amplitude of BLH is higher in the northern and western subregions of China than other subregions. The meteorological influence on the annual cycle of BLH is investigated as well, showing that BLH at most sounding sites is negatively associated with the surface pressure and lower tropospheric stability, but positively associated with the near-surface wind speed and temperature. In addition, cloud tends to suppress the development of PBL, particularly in the early afternoon. This indicates that meteorology plays a significant role in the PBL processes. Overall, the key findings obtained from this study lay a solid foundation for us to gain a deep insight into the fundamentals of PBL in China, which helps to understand the roles that the PBL plays in the air pollution, weather and climate of China.

A new methodology is developed to construct a global (60°S–60°N) long‐term (2000–2019) high‐resolution (∼10‐km h) mesoscale convective system (MCS) database by tracking MCS jointly using geostationary satellite infrared brightness temperature (T_b) and precipitation feature (PF) characteristics from the Integrated Multi‐satellitE Retrievals for GPM precipitation data sets. Independent validation shows that the satellite‐based MCS data set is able to reproduce important MCS statistics derived from ground‐based radar network observations in the United States and China. We show that by carefully considering key PF characteristics in addition to T_b signatures, the new method significantly improves upon previous T_b‐only methods in detecting MCSs in the midlatitudes for all seasons. Results show that MCSs account for over 50% of annual total rainfall across most of the tropical belt and in selected regions of the midlatitudes, with a strong seasonality over many regions of the globe. The tracking database allows Lagrangian aspects such as MCS lifetime and translational speed and direction to be analyzed. The longest‐lived MCSs preferentially occur over the subtropical oceans. The land MCSs have higher cloud‐tops associated with more intense convection, and oceanic MCSs have much higher rainfall production. While MCSs are observed in many regions of the globe, there are fundamental differences in their dynamic and thermodynamic structures that warrant a better understanding of processes that control their evolution. This global database provides significant opportunities for observational and modeling studies of MCSs, their characteristics, and roles in regional and global water and energy cycles, as well as their hydrologic and other impacts.