Plasma jets are sources of repetitive and stable ionization waves, meant for applications where they interact with surfaces of different characteristics. As such, plasma jets provide an ideal testbed for the study of transient reproducible streamer discharge dynamics, particularly in inhomogeneous gaseous mixtures, and of plasma–surface interactions. This topical review addresses the physics of plasma jets and their interactions with surfaces through a pedagogical approach. The state-of-the-art of numerical models and diagnostic techniques to describe helium jets is presented, along with the benchmarking of different experimental measurements in literature and recent efforts for direct comparisons between simulations and measurements. This exposure is focussed on the most fundamental physical quantities determining discharge dynamics, such as the electric field, the mean electron energy and the electron number density, as well as the charging of targets. The physics of plasma jets is described for jet systems of increasing complexity, showing the effect of the different components (tube, electrodes, gas mixing in the plume, target) of the jet system on discharge dynamics. Focussing on coaxial helium kHz plasma jets powered by rectangular pulses of applied voltage, physical phenomena imposed by different targets on the discharge, such as discharge acceleration, surface spreading, the return stroke and the charge relaxation event, are explained and reviewed. Finally, open questions and perspectives for the physics of plasma jets and interactions with surfaces are outlined.

The ratio of the spectral band intensities of the first negative and second positive spectral systems of molecular nitrogen is a well recognized method for indirect determination of the electric field. It is applied for various plasmas, e.g. barrier and corona discharges for industrial applications or geophysical plasmas occurring in the Earth’s atmosphere. The method relies on the dependence of the intensity ratio R ( E / N ) of selected bands on the reduced electric field strength. Both experimental and theoretical approaches have been used to determine this dependence, yet there still is a rather large spread in the data available in literature. The primary aim of this work is to quantify the overall uncertainty of the theoretical R ( E / N ) dependence and identify the main sources of this uncertainty. As the first step we perform sensitivity analysis on a full N ₂ /O ₂ plasma kinetics model to find a minimal set of processes that are influential for the R ( E / N ) dependence. It is found to be in agreement with simplified kinetic models generally used. Subsequently, we utilize Monte Carlo-based uncertainty quantification to provide a confidence band for the electric field obtained from the theoretical R ( E / N ) dependence. Finally, subsequent steps are proposed to significantly reduce the uncertainty of the method.

Numerical simulations and experiments are performed to better understand the interaction between a pulsed helium plasma jet and a dielectric target. The focus of this work lies on the volume and surface charge influence on the electric field distribution. Experimentally, the electric field due to surface charges is measured inside an electro-optic target under exposure of a plasma jet, using the optical technique called Mueller polarimetry. For the first time, the time-resolved spatial distributions of both the axial and radial components of electric field inside the target are obtained simultaneously. A 2D fluid model is used in a complementary way to the experiments in order to study separately the contribution of volume charges and surface charges to the spatio-temporal evolutions of the electric field during the plasma–surface interaction. The experimental investigation shows that the average axial and radial components of electric field inside the dielectric target, only due to surface charges, are lower than generally reported for electric field values in the plasma plume. Thanks to the phenomenological comparison with experiments, simulations show that during the plasma–surface interaction two effects sequentially determine the electric field inside the target: firstly, a relatively high electric field is observed due to the proximity of the ionization front; afterwards, in longer timescales, lower electric fields are induced due to the contribution of both leftover volume charges close to the target and surface charges deposited on its surface. The experimental technique provides a unique way to examine this second phase of the plasma–surface interaction.

The interaction of kHz μs-pulsed atmospheric pressure He jets with metallic targets is studied through simulations and experiments, focusing on the differences between floating and grounded targets. It is shown that the electric potential of the floating target is close to grounded in the instants after the impact of the discharge, but rises to a high voltage, potentially more than half of the applied voltage, at the end of the 1 μs pulse. As a result, a return stroke takes place after the discharge impact with both grounded and floating targets, as a redistribution between the high voltage electrode and the low voltage target. Electric field, electron temperature and electron density in the plasma plume are higher during the pulse with grounded target than with floating target, as gradients of electric potential progressively dissipate in the latter case. Finally, at the fall of the pulse, another electrical redistribution takes place, with higher intensity with the highly-charged floating target than with the grounded target. It is shown that this phenomenon can lead to an increase in electric field, electron temperature and electron density in the plume with floating target.

The review provides an up-to-date overview and discussion of phenomena related to positive streamer breakdowns in short uniform and non-uniform field (corona) gaps. The terminology used to specify different types of streamer phenomena is critically discussed in light of a unified theory of high-pressure gas discharges describing the sequence of ionization events from initial electron avalanches up to a partial or complete breakdown. The emphasis is given to the understanding of the formation of an active cathode spot by the streamer arrival to the cathode, which is the critical but still obscure phase of the breakdown development. Based on the analysis including a computer simulation model a hypothesis is advanced that also such widely studied and practically important gas discharge phenomena as negative corona Trichel pulses and fast ionization instabilities in cathode regions of high-pressure gas discharges are due to the formation of positive streamers in the immediate cathode vicinity. The proposed hypothesis offers attractive feature of the unification of a wide scale of high-pressure gas discharges within the general class of positive streamer initiated breakdown phenomena. Moreover, it provides indications for further study in the field both by experiment and computer simulations.

This work investigates the dynamical charging of a surface under exposure of a non-equilibrium plasma jet at atmospheric pressure through a quantitative comparison between modeling and experiments. We show using mono-polar pulses with variable pulse duration and amplitude that the charging time (i.e. the time from impact of the ionization wave till the fall of the high voltage pulse) is a crucial element determining the plasma-surface interaction. This is done through direct measurements of the electric field induced inside the target using the optical diagnostic technique called Mueller polarimetry and comparison with the electric field calculated using a 2D fluid model of the plasma jet interaction with the target in the same conditions as in the experiments. When the charging time is kept relatively short (less than 100 ns), the surface spreading of the discharge and consequent surface charge deposition are limited. When it is relatively long (up to microseconds), the increased surface spreading and charge deposition significantly change the electric field to which the target is exposed during the charging time and when the applied voltage returns to zero.