Long-wavelength stimulated emission (SE) is studied in optically pumped HgCdTe quantum well heterostructures with dielectric waveguides. Continuous temperature tuning of the wavelength from 27 to 18 μm is achieved in structures with optimized waveguides. Above 27 μm, SE clamps at 31 μm wavelength, where mode leaking is reduced due to the Reststrahlen effect in the GaAs substrate. The operating temperature is mainly limited by the activation of Auger recombination in quasi-equilibrium conditions, while at low temperatures, we expect that lowering initial carrier heating would enhance the gain considerably. We conclude that exploiting the Reststrahlen effect should allow one to achieve continuous wavelength tuning around 30 μm and operating wavelengths up to 40 μm with technologically attainable epistructure thickness.
Amplified interband emission within the 14–24 μm range is investigated in HgCdTe-based quantum wells under optical pumping. Carrier lifetimes are shown to be marginally limited only by Shockley–Read–Hall recombination, fully realizing the advantage of relativistic energy spectra of 2D HgCdTe in terms of suppressing the Auger processes. By carefully optimizing the waveguides and mitigating carrier heating, we achieve amplification thresholds as low as 1.5–2 W/cm2 at a pulse duration of 20–500 μs. With last generation quantum cascade lasers used for optical pumping, we estimate that continuous-wave HgCdTe lasers can operate in the very long-wavelength range (15–30 μm) and beyond.
HgTe/CdHgTe quantum well (QW) heterostructures have attracted a lot of interest recently due to insights they provided towards the physics of topological insulators and massless Dirac fermions. Our work focuses on HgCdTe QWs with the energy spectrum close to the graphene-like relativistic dispersion that is supposed to suppress the non-radiative Auger recombination. We combine various methods such as photoconductivity, photoluminescence and magneto-optical measurements as well as transmission electron microscopy to retrofit growth parameters in multi-QW waveguide structures, designed for long wavelengths lasing in the range of 10–22 μm. The results reveal that the attainable operating temperatures and wavelengths are strongly dependent on Cd content in the QW, since it alters the dominating recombination mechanism of the carriers.
Due to their widely tunable bandgap, HgCdTe heterostructures with quantum wells are a promising material system for semiconductor lasers in the entire mid-infrared range. Recently, Auger-suppressed structures allowed interband stimulated emission (SE) in the atmospheric transparency window 3–5 μm well above 200 K, while previously it was limited to temperatures below 175 K. In contrast to earlier works focused on ridge or vertical emitting HgCdTe lasers, here we demonstrate a whispering gallery mode microdisk (d = 50 μm) laser operating under optical pumping at ∼4 μm in the temperature range attainable by the thermoelectric cooling. Above 200 K, the emission spectrum consists of multiple 0.37-meV-wide peaks associated with the modes of the disk resonator. Laser generation is achieved up to 230 K, which is 40 K lower than the quenching temperature of SE in the unprocessed macroscopic sample. We associate the difference with the optical losses introduced by the inclined walls of the disk.
Heterostructures with thin Hg(Cd)Te/CdHgTe quantum wells (QWs) are attractive for the development of mid-infrared interband lasers. Of particular interest are room-temperature operating emitters for the short-wavelength infrared range (SWIR, typically defined as 1.7–3 μm). In this work, we report on the observation of stimulated emission (SE) in the 2.65–2.75 µm wavelength range at room temperature in an optically pumped HgCdTe QW laser heterostructure. We study a series of three samples with lengths ranging from 2.5 to 7 mm and discuss the effects related to the non-uniformity of the excitation beam profile. SE threshold intensity and the magnitude of pump-induced carrier heating are found to be effectively dependent on the chip size, which should be accounted for in possible designs of HgCdTe-based optical converters. We also pay attention to the problem of active medium engineering in order to push the SE wavelength towards the 3–5 µm atmospheric window and to lower the SE threshold.
Mercury vacancies, acting as double acceptors, are the dominant point defects in ternary HgCdTe alloys. Though HgCdTe is one of the leading materials in infrared optoelectronics, the energy spectra of the vacancies are still a matter of some debate. This work investigated the rates at which holes are captured to a singly ionized mercury vacancy via acoustic phonon emission in narrow-gap Hg1−xCdxTe with technologically relevant x~0.22. Combined with the calculated rates of intracenter transitions, the data allow one to predict the most pronounced optical transitions in the emission spectrum of a double-charged acceptor. The results are sustained by the photoluminescence spectroscopy in the terahertz domain, allowing one to identify the emission band that is related to neutral vacancies.