High lumen-density laser lighting has become an advanced lighting technology. However, as an important component, transparent light-conversion materials exhibit low efficiency and luminescence declining behaviors, especially under high power density lasers, seriously restricting their potential applications. Herein, high quality YAG:Ce transparent ceramics (TCs) with different Ce concentrations and sizes were designed and fabricated for comparison with YAG:Ce single crystals to reveal the nature behind the above phenomena under the assistance of different encapsulated models of LED/LD devices. The highest luminous efficiency for the TCs of over 248 lm W−1 was achieved in the LED device, while only 170 lm W−1 could be reached for the LD devices. The strong thermal quenching and concentration quenching worked synergistically to result in the luminescence declining behavior in the 0.5 at% YAG:Ce ceramics, which have 80% and 20% responsibility after smart experimental comparison, respectively. Besides, the potential factors for the low efficiency in TC-based LD lighting were also revealed. Therefore, this work not only shows the optical performance of TCs in LED and LD applications, but also presents how the deep influence factors and excitation models lead to differences in their performance. It significantly reinforces the understanding of fundamental problems for TC-based high power laser lighting. These results are crucial for advancing TC-supported technologies in illumination, projection and scintillation.
How topological defects, unavoidable at symmetry-breaking phase transitions in a wide range of systems, evolve through consecutive phase transitions with different broken symmetries remains unexplored. , a bilayer ferrite, exhibits two intriguing structural phase transitions and dense networks of the so-called type II structural vortices at room temperature, so it is an ideal system to explore the topological defect evolution. From our extensive experimental investigation, we demonstrate that the cooling rate at the second-order transition (1290°C) plays a decisive role in determining the vortex density at room temperature, following the universal Kibble-Zurek mechanism. In addition, we discovered a transformation between topologically distinct vortices ( to vortices) at the first-order transition (550°C), which conserves the number of vortex cores. Remarkably, the vortices consist of two phases with an identical symmetry but two distinct magnitudes of an order parameter. Furthermore, when lattice distortion is enhanced by chemical doping, an alternative type of topological defects emerges: loop domain walls with orthorhombic distortions in the tetragonal background, resulting in unique pseudo-orthorhombic twins. Our findings open an avenue to explore the evolution of topological defects through multiple phase transitions.