Hongtao Sun

Dr. Hongtao Sun


Research Focus & Metrics

Academic Career Length

16Years (2011-Present)

(Calculated once Scilit publication data is synced: current year − year of first publication + 1)

Representative Publications

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8 January 2018 in Nature Catalysis
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Journal Article
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HFHuilong Fei
Huilong Fei
JDJuncai Dong
Juncai Dong
YFYexin Feng
Yexin Feng
CAChristopher S. Allen
Christopher S. Allen
CWChengzhang Wan
Chengzhang Wan
YHYu Huang
Yu Huang

12 May 2017 in Science
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Journal Article
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Hongtao SunHongtao Sun
Hongtao Sun
LMLin Mei
Lin Mei
JLJunfei Liang
Junfei Liang
ZZZipeng Zhao
Zipeng Zhao
CLChain Lee
Chain Lee
XDXiangfeng Duan
Xiangfeng Duan
As with donuts, the holes matter: Improving the density of stored charge and increasing the speed at which it can move through a material are usually opposing objectives. Sun et al. developed a Nb 2 O 5 /holey graphene framework composite with tailored porosity. The three-dimensional, hierarchically porous holey graphene acted as a conductive scaffold to support Nb 2 O 5 . A high mass loading and improved power capability were reached by tailoring the porosity in the holey graphene backbone with higher charge transport in the composite architecture. The interconnected graphene network provided excellent electron transport, and the hierarchical porous structure in the graphene sheets facilitated rapid ion transport and mitigated diffusion limitations. Science , this issue p. 599

17 December 2018 in Nature Reviews Materials
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Journal Article
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Hongtao SunHongtao Sun
Hongtao Sun
JZJian Zhu
Jian Zhu
DBDaniel Baumann
Daniel Baumann
LPLele Peng
Lele Peng
YXYuxi Xu
Yuxi Xu
XDXiangfeng Duan
Xiangfeng Duan

15 February 2019 in Science
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Journal Article
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Xiang XuXiang Xu
Xiang Xu
QZQiangqiang Zhang
Qiangqiang Zhang
MHMenglong Hao
Menglong Hao
YHYuan Hu
Yuan Hu
ZLZhaoyang Lin
Zhaoyang Lin
XDXiangfeng Duan
Xiangfeng Duan
Elastic ceramics: Aerogels hold promise as lightweight replacements for thermal insulation. However, poor mechanical stability has hampered progress in moving toward commercialization. Xu et al. designed a mechanical metamaterial that pinches in a small amount when you compress it (see the Perspective by Chhowalla and Jariwala). This is characteristic of materials with a negative Poisson's ratio and dramatically improves mechanical stability. The trick was using three-dimensional graphene structures to template the ceramic aerogels, thus producing a superinsulating material endowed with excellent mechanical properties. Science , this issue p. 723 ; see also p. 694

4 September 2015 in Science
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Journal Article
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GXGuoqing Xin
Guoqing Xin
TYTIANKAI YAO
TIANKAI YAO
Hongtao SunHongtao Sun
Hongtao Sun
SSSpencer Michael Scott
Spencer Michael Scott
DSDali Shao
Dali Shao
JLJie Lian
Jie Lian
A superior mix of big and small: Graphene is often described as an unrolled carbon nanotube. However, although nanotubes are known for their exceptional mechanical and conductivity properties, the same is not true of graphene-based fibers. Xin et al. intercalated small fragments of graphene into the gaps formed by larger graphene sheets that had been coiled into fibers. Once annealed, the large sheets provided pathways for conduction, while the smaller fragments helped reinforce the fibers. The result? Superior thermal and electrical conductivity and mechanical strength. Science , this issue p. 1083

31 July 2014 in Nature Communications
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Journal Article
Open access
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Hongtao SunHongtao Sun
Hongtao Sun
GXGuoqing Xin
Guoqing Xin
THTao Hu
Tao Hu
Mingpeng YuMingpeng Yu
Mingpeng Yu
DSDali Shao
Dali Shao
JLJie Lian
Jie Lian
Mechanical and chemical degradations of high-capacity anodes, resulting from lithiation-induced stress accumulation, volume expansion and pulverization, and unstable solid–electrolyte interface formation, represent major mechanisms of capacity fading, limiting the lifetime of electrodes for lithium-ion batteries. Here we report that the mechanical degradation on cycling can be deliberately controlled to finely tune mesoporous structure of the metal oxide sphere and optimize stable solid–electrolyte interface by high-rate lithiation-induced reactivation. The reactivated Co3O4 hollow sphere exhibits a reversible capacity above its theoretical value (924 mAh g−1 at 1.12 C), enhanced rate performance and a cycling stability without capacity fading after 7,000 cycles at a high rate of 5.62 C. In contrast to the conventional approach of mitigating mechanical degradation and capacity fading of anodes using nanostructured materials, high-rate lithiation-induced reactivation offers a new perspective in designing high-performance electrodes for long-lived lithium-ion batteries.