Ecologically friendly wood electronics will help alleviating the shortcomings of state-of-art cellulose-based “green electronics”. Here we introduce iron-catalyzed laser-induced graphitization (IC-LIG) as an innovative approach for engraving large-scale electrically conductive structures on wood with very high quality and efficiency, overcoming the limitations of conventional LIG including high ablation, thermal damages, need for multiple lasing steps, use of fire retardants and inert atmospheres. An aqueous bio-based coating, inspired by historical iron-gall ink, protects wood from laser ablation and thermal damage while promoting efficient graphitization and smoothening substrate irregularities. Large-scale (100 cm²), highly conductive (≥2500 S m⁻¹) and homogeneous surface areas are engraved single-step in ambient atmosphere with a conventional CO₂ laser, even on very thin (∼450 µm) wood veneers. We demonstrate the validity of our approach by turning wood into highly durable strain sensors, flexible electrodes, capacitive touch panels and an electroluminescent LIG-based device.

Structural color is frequently exploited by living organisms for biological functions and has also been translated into synthetic materials as a more durable and less hazardous alternative to conventional pigments. Additive manufacturing approaches were recently exploited for the fabrication of exquisite photonic objects, but the angle-dependence observed limits a broader application of structural color in synthetic systems. Here, we propose a manufacturing platform for the 3D printing of complex-shaped objects that display isotropic structural color generated from photonic colloidal glasses. Structurally colored objects are printed from aqueous colloidal inks containing monodisperse silica particles, carbon black, and a gel-forming copolymer. Rheology and Small-Angle-X-Ray-Scattering measurements are performed to identify the processing conditions leading to printed objects with tunable structural colors. Multimaterial printing is eventually used to create complex-shaped objects with multiple structural colors using silica and carbon as abundant and sustainable building blocks.

Significance: A set of magnetically responsive, soft hairs, which form a soft magnetic carpet, can be infused with a liquid to achieve switchable wetting. Applying a pattern of magnetic field results in a reconfigurable wetting pattern on the soft magnetic carpet. Combining this switchable wetting with a travelling magnetic field wave can allow us to spatially manipulate droplets. The efficiency of the droplet manipulation depends on the size and the contact angle of the droplet, which allows a pathway to sort and separate different droplets. Temporal and spatial control over multiple droplets allows us to conduct droplet reactions, which has a potential to be used for automated analytical testing and screening.

Biological materials such as nacre have evolved microstructural design principles that result in outstanding mechanical properties. While nacre’s design concepts have led to bio-inspired materials with enhanced fracture toughness, the microstructural features underlying the remarkable damping properties of this biological material have not yet been fully explored in synthetic composites. Here, we study the damping behavior of nacre-like composites containing mineral bridges and platelet asperities as nanoscale structural features within its brick-and-mortar architecture. Dynamic mechanical analysis was performed to experimentally elucidate the role of these features on the damping response of the nacre-like composites. By enhancing stress transfer between platelets and at the brick/mortar interface, mineral bridges and nano-asperities were found to improve the damping performance of the composite to levels that surpass many biological and man-made materials. Surprisingly, the improved properties are achieved without reaching the perfect organization of the biological counterparts. Our nacre-like composites display a loss modulus 2.4-fold higher than natural nacre and 1.4-fold more than highly dissipative natural fiber composites. These findings shed light on the role of nanoscale structural features on the dynamic mechanical properties of nacre and offer design concepts for the manufacturing of bio-inspired composites for high-performance damping applications.

Colors enable interaction and communication between living species in a myriad of biological and artificial environments. While living organisms feature low‐power mechanisms to dynamically control color in soft tissues, man‐made color‐changing devices remain predominantly rigid and energy intensive. Here, architectured composites that display striking color changes when stretched in selective directions under ambient light with minimum power input are reported. The orientation‐dependent color change results from the rotation of reflective coated platelets that are embedded in a soft polymer matrix and pre‐aligned in a well‐defined architecture. The light reflected by the platelets generates structural color defined by the oxide coating on the platelet surface. By magnetically programming the initial orientation and spatial distribution of selected platelets within the soft matrix, composites with strain‐modulated color‐changing effects that cannot be achieved using state‐of‐the‐art technologies are created. The proposed concept of strain‐induced architectured color can be harnessed to develop low‐power smart stretchable displays, tactile synthetic skins, and autonomous soft robotic devices that undergo fast and reversible color changes through the mechano‐optic coupling programmed within their soft composite architecture.