In this article, a mid-infrared all-fiber light-induced thermoelastic spectroscopy (LITES) sensor based on a hollow-core anti-resonant fiber (HC-ARF) was reported for the first time. The HC-ARF was applied as a light transmission medium and gas chamber. The constructed all-fiber structure has merits of low loss, easy optical alignment, good system stability, reduced sensor size and cost. The mid-infrared transmission structure can be utilized to target the strongest gas absorption lines. The reversely-tapered SM1950 fiber and the HC-ARF were spatially butt-coupled with a V-shaped groove between the two fibers to facilitate gas entry. Carbon monoxide (CO) with an absorption line at 4291.50 cm-1 (2.33 µm) was chosen as the target gas to verify the sensing performance. The experimental results showed that the all-fiber LITES sensor based on HC-ARF had an excellent linear response to CO concentration. Allan deviation analysis indicated that the system had excellent long-term stability. A minimum detection limit (MDL) of 3.85 ppm can be obtained when the average time was 100 s.
A novel quartz enhanced photoacoustic spectroscopy (QEPAS) trace gas detection scheme is reported in this paper. A cylindrical lens was employed for near-infrared laser focusing. The laser beam was shaped as a planar line laser between the gap of the quartz tuning fork (QTF) prongs. Compared with a spherical lens-based QEPAS sensor, the cylindrical lens-based QEPAS sensor has the advantages of easier laser beam alignment and a reduction of stringent stability requirements. Therefore, the reported approach is useful in long-term and continuous sensor operation.
In this paper, an all-fiber light-induced thermoelastic spectroscopy (LITES) sensor based on hollow-core anti-resonant fiber (HC-ARF) and self-designed low-frequency quartz tuning fork (QTF) is reported for the first time. By utilizing HC-ARF as both the transmission medium and gas chamber, the laser tail fiber was spatially coupled with the HC-ARF, and the end of the HC-ARF was directly guided onto the QTF surface, resulting in an all-fiber structure. This design eliminated the need for lens combinations, thereby enhancing system stability and reducing cost and size. Additionally, a self-designed rectangular-tip QTF with a low resonant frequency of 8.69 kHz was employed to improve the sensor’s detection performance. Acetylene (C2H2), with an absorption line at 6534.37 cm−1 (1.53 μm), was chosen as the target gas. Experimental results clearly demonstrated that the detection performance of the rectangular-tip QTF system was 2.9-fold higher than that of a standard commercial QTF system. Moreover, it exhibited an outstanding linear response to varying C2H2 concentrations, indicating its high sensitivity and reliability in detecting C2H2. The Allan deviation analysis was used to assess the system’s stability, and the results indicated that the system exhibits excellent long-term stability.
A tunable diode laser absorption spectroscopy (TDLAS) sensor with a highly sensitive dual-component for methane (CH4) and acetylene (C2H2) detection is reported in this paper for the first time. A multi-pass cell (MPC) design model was established employing a vector-based ray-tracing method. A dual-channel MPC with an interlaced dual hexagonal star pattern was designed to improve gas absorption and realize real-time synchronous detection of CH4 and C2H2. During the simultaneous continuous monitoring of CH4 and C2H2, the sensor exhibited an excellent linear response to concentration variations. The minimum detection limit (MDL) for CH4 reached 132.08 ppb, improving to 77.32 ppb when the average time was increased to 300 s. In the case of C2H2, the MDL was measured at 20.19 ppb and further reduced to 3.50 ppb under the same extended average time.
In this paper, a highly sensitive carbon monoxide (CO) light-induced thermoelastic spectroscopy (LITES) sensor based on tapered-fiber focusing and a fiber-coupled multipass cell (MPC) is demonstrated for the first time. An MPC with a fiber-coupled structure and an optical length of 40 m is employed to significantly increase the effective absorption path length, reduce the difficulty of optical alignment, and improve the robustness of the sensor system. By comparing five different beam shaping and focusing schemes at the MPC output, the influence of the excitation spot size on the generation of the LITES signal is thoroughly investigated. Experimental results demonstrate that the system response is significantly enhanced as the spot size is compressed. Owing to the micron-scale focused spot produced by the tapered fiber end face, the tapered-fiber configuration exhibits the strongest sensing response among the five schemes. This configuration achieves the highest signal-to-noise ratio (SNR) and exhibits a good linear response to CO concentration. The minimum detection limit (MDL) of the proposed CO-LITES sensor is 3.86 ppm. Based on Allan deviation analysis, when the system integration time reaches 300 s, the minimum detection limit can be further improved to 304 ppb, demonstrating excellent long-term stability.