Xiaoshuai Han

Dr. Xiaoshuai Han


Research Focus & Metrics

Academic Career Length

6Years (2021-Present)

(Calculated once Scilit publication data is synced: current year − year of first publication + 1)

Representative Publications

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12 September 2022 in Nanomaterials
Verified
Journal Article
Open access
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JWJingwen Wang
Jingwen Wang
XHXiaoshuai Han
Xiaoshuai Han
CZChunmei Zhang
Chunmei Zhang
Kunming LiuKunming Liu
Kunming Liu
Gaigai DuanGaigai Duan
Gaigai Duan
Food packaging nowadays is not only essential to preserve food from being contaminated and damaged, but also to comply with science develop and technology advances. New functional packaging materials with degradable features will become a hot spot in the future. By far, plastic is the most common packaging material, but plastic waste has caused immeasurable damage to the environment. Cellulose known as a kind of material with large output, wide range sources, and biodegradable features has gotten more and more attention. Cellulose-based materials possess better degradability compared with traditional packaging materials. With such advantages above, cellulose was gradually introduced into packaging field. It is vital to make packaging materials achieve protection, storage, transportation, market, and other functions in the circulation process. In addition, it satisfied the practical value such as convenient sale and environmental protection, reduced cost and maximized sales profit. This review introduces the cellulose resource and its application in composite packaging materials, antibacterial active packaging materials, and intelligent packaging materials. Subsequently, sustainable packaging and its improvement for packaging applications were introduced. Finally, the future challenges and possible solution were provided for future development of cellulose-based composite packaging materials.

11 December 2022 in Polymers
Verified
Journal Article
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SJShaoju Jian
Shaoju Jian
YCYuhuang Chen
Yuhuang Chen
FSFengshuo Shi
Fengshuo Shi
YLYifei Liu
Yifei Liu
WJWenlong Jiang
Wenlong Jiang
AYAnd Weisen Yang
And Weisen Yang
The occurrence of fluoride contamination in drinking water has gained substantial concern owing to its serious threat to human health. Traditional adsorbents have shortcomings such as low adsorption capacity and poor selectivity, so it is urgent to develop new adsorbents with high adsorption capacity, renewable and no secondary pollution. In this work, magnetic electrospun La-Mn-Fe tri-metal oxide nanofibers (LMF NFs) for fluoride recovery were developed via electrospinning and heat treatment, and its defluoridation property was evaluated in batch trials. Modern analytical tools (SEM, BET, XRD, FTIR) were adopted to characterize the properties of the optimized adsorbent, i.e., LMF11 NFs with a La:Mn molar ratio of 1:1. The surface area calculated via BET method and pHpzc assessed using pH drift method of LMF11 NFs were 55.81 m2 g−1 and 6.47, respectively. The results indicated that the adsorption amount was highly dependent on the pH of the solution, and reached the highest value at pH = 3. The kinetic behavior of defluoridation on LMF11 NFs was dominated by the PSO model with the highest fitted determination coefficients of 0.9999. Compared with the other three isotherm models, the Langmuir model described defluoridation characteristics well with larger correlation coefficients of 0.9997, 0.9990, 0.9987 and 0.9976 at 15 °C, 25 °C, 35 °C and 45 °C, respectively. The optimized LMF11 NFs exhibited superior monolayer defluoridation capacities for 173.30–199.60 mg F−/g at pH 3 at 15–45 °C according to the Langmuir isotherm model. A thermodynamic study proved that the defluoridation by LMF11 NFs is a spontaneous, endothermic along with entropy increase process. In addition, the LMF11 NFs still showed high defluoridation performance after three reused cycles. These findings unveil that the synthesized LMF11 NFs adsorbent is a good adsorbent for fluoride remediation from wastewater owing to its low cost, high defluoridation performance and easy operation.

15 April 2023 in Molecules
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Journal Article
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JSJiangyan Song
Jiangyan Song
AYAnd Weisen Yang
And Weisen Yang
XHXiaoshuai Han
Xiaoshuai Han
Shaohua JiangShaohua Jiang
Shaohua Jiang
CZChunmei Zhang
Chunmei Zhang
JHJiapeng Hu
Jiapeng Hu
The performance of a Ce(III)-4,4′,4″-((1,3,5-triazine-2,4,6-triyl) tris (azanediyl)) tribenzoic acid–organic framework (Ce-H3TATAB-MOFs) for capturing excess fluoride in aqueous solutions and its subsequent defluoridation was investigated in depth. The optimal sorption capacity was obtained with a metal/organic ligand molar ratio of 1:1. The morphological characteristics, crystalline shape, functional groups, and pore structure of the material were analyzed via SEM, XRD, FTIR, XPS, and N2 adsorption–desorption experiments, and the thermodynamics, kinetics, and adsorption mechanism were elucidated. The influence of pH and co-existing ions for defluoridation performance were also sought. The results show that Ce-H3TATAB-MOFs is a mesoporous material with good crystallinity, and that quasi-second kinetic and Langmuir models can describe the sorption kinetics and thermodynamics well, demonstrating that the entire sorption process is a monolayer-governed chemisorption. The Langmuir maximum sorption capacity was 129.7 mg g−1 at 318 K (pH = 4). The adsorption mechanism involves ligand exchange, electrostatic interaction, and surface complexation. The best removal effect was reached at pH 4, and a removal effectiveness of 76.57% was obtained under strongly alkaline conditions (pH 10), indicating that the adsorbent has a wide range of applications. Ionic interference experiments showed that the presence of PO43− and H2PO4− in water have an inhibitory effect on defluoridation, whereas SO42−, Cl−, CO32−, and NO3− are conducive to the adsorption of fluoride due to the ionic effect.

20 January 2023 in International Journal of Biological Macromolecules
Verified
Journal Article
Closed access
JWJingwen Wang
Jingwen Wang
XHXiaoshuai Han
Xiaoshuai Han
WWWeijie Wu
Weijie Wu
XWXiaoyi Wang
Xiaoyi Wang
LDLinhu Ding
Linhu Ding
Shaohua JiangShaohua Jiang
Shaohua Jiang

8 March 2023 in Molecules
Verified
Journal Article
Open access
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XMXiaofan Ma
Xiaofan Ma
XHXiaoshuai Han
Xiaoshuai Han
JHJiapeng Hu
Jiapeng Hu
AYAnd Weisen Yang
And Weisen Yang
JHJingquan Han
Jingquan Han
Shaohua JiangShaohua Jiang
Shaohua Jiang
With the increasing pollution of electromagnetic (EM) radiation, it is necessary to develop low-cost, renewable electromagnetic interference (EMI) shielding materials. Herein, wood-derived carbon (WC) materials for EMI shielding are prepared by one-step carbonization of renewable wood. With the increase in carbonization temperature, the conductivity and EMI performance of WC increase gradually. At the same carbonization temperature, the denser WC has better conductivity and higher EMI performance. In addition, due to the layered superimposed conductive channel structure, the WC in the vertical-section shows better EMI shielding performance than that in the cross-section. After excluding the influence of thickness and density, the specific EMI shielding effectiveness (SSE/t) value can be calculated to further optimize tree species. We further discuss the mechanism of the influence of the microstructure of WC on its EMI shielding properties. In addition, the lightweight WC EMI material also has good hydrophobicity and heat insulation properties, as well as good mechanical properties.

10 May 2021 in Research Square
Verified
Preprint
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LDLinhu Ding
Linhu Ding
XHXiaoshuai Han
Xiaoshuai Han
HLHuiling Li
Huiling Li
JHJingquan Han
Jingquan Han
LCLihua Cao
Lihua Cao
Shaohua JiangShaohua Jiang
Shaohua Jiang
The study on novel natural fibers in polymer-based composites will help promote the invention of novel reinforcement and expand their possible applications. Herein, novel cellulosic fibers were extracted from the stem of manau rattan (Calamus manan) by mechanical separation. It is the first time to comprehensively analyze and study the chemical, thermal, mechanical and morphological properties of manau rattan fibers by Fourier Transform Infrared Spectroscopy (FTIR), X-Ray Photoelectron Spectroscopy (XPS), X-Ray Diffraction Analysis (XRD), Thermogravimetric Analysis (TGA), single fiber tensile test and Scanning Electron Microscopy (SEM). Component analysis results showed the cellulose, hemicellulose and lignin contents of manau rattan fibers were 42, 20, and 27%, respectively. The surface of the rattan fiber was hydrophilic according to the oxygen/carbon ratio of 0.49. Manau rattan has a high crystalline index of 48.28%, inducing a high maximum degradation temperature of 332.8°C. This reveals that it can be used as a reinforcement for thermoplastic composites whose operating temperature is below 300°C. The average tensile strength can reach 273.28 MPa, which is beneficial to improve the mechanical properties of rattan fiber reinforced composites. SEM images displayed the rough surface of the fiber, which helps to enhance the interfacial adhesion between the fibers and matrices in composites. This work was also in comparison with some other natural fibers. The above analysis and research showed the great potential of manau rattan fibers as the reinforcement in polymer-based composites.