Multi-pass cells, known for their efficient spectral broadening, currently face a challenge in their peak power scalability. To address this, we implemented a strategy where the input pulse was split into 8 replicas, resulting in an increased pulse energy following nonlinear compression. The used laser delivered 208 fs pulses at 1030 nm, with pulse energies reaching up to 140μJ. Using 3 calcite crystals, the input pulse was divided and passed through the MPC, achieving a spectral broadening down to a 40 fs bandwidth limit. Subsequently, the replicas were recombined using an identical set of crystals and compressed via chirped mirrors. FROG measurements revealed a duration of 43 fs. The recombination losses amounted to less than 5 % of the output energy. This method is particularly attractive and cost-effective for spectral broadening of ultrafast lasers with adjustable repetition rate.
The saturable absorption of 2D Bi2Te3 layers is studied by using the Z-scan technique employing infrared 400 fs laser pulses. Optimization of the nonlinearities has been carried out by measuring the third-order nonlinear susceptibilities as a function of the film thickness. A thorough optimization of the thin film annealing conditions has been performed and is presented. For each thickness, the annealing parameters have been separately investigated. Scanning electron microscopy, X-ray diffraction, and UV-Vis spectrophotometry studies have also been performed on the as-deposited and crystallized 2D layers.
We present a hybrid two-stage multipass cell for spectral broadening. We demonstrate the compression of 1mJ, 1 ps pulses from a Yb:YAG amplifier down to 17 fs and report generating a 10-fs transform limited spectrum.
Q-switched lasers are compact, cost-effective, and highly pulse energy-scalable sources for nanosecond-scale laser pulses. The technology has been developed for many decades and is widely used in scientific, industrial and medical applications. However, their inherently narrow bandwidth imposes a lower limit on pulse duration—typically in the few-hundred-picosecond range—limiting the applicability of Q-switched technology in fields that require ultrafast laser pulses in the few-picosecond or femtosecond regime. In contrast, mode-locked lasers can produce broad-band, ultrafast ( 1 ps) pulses, but are complex, expensive, and typically require a large footprint. To bridge the parameter gap between these two laser platforms—in terms of pulse duration and achievable peak power—we here propose a Herriott-type multi-pass cell (MPC) based post-compression scheme for shortening the pulse durations of Q-switched lasers down to the ultrafast, picosecond regime. We experimentally demonstrate post-compression of 0.5 ns, 1 mJ pulses from a Q-switched laser to 24 ps using a compact glass-rod MPC for spectral broadening. We verify this result numerically and show that compression down to a few picoseconds is possible using the nanosecond MPC (nMPC). Through spectral filtering approaches, the nMPC suppresses detrimental nonlinear processes such as stimulated Raman scattering, which have set severe limitations for fiber-based post-compression of Q-switched lasers until today. Our results pave the way to cost-efficient and compact ultrafast laser platforms based on Q-switched laser technology.
A proof-of-concept demonstration of divided pulse spectral broadening in a multipass cell with common-path Mach-Zehnder-interferometers is reported. The used virtually dispersion-free, flexible delay lines offer unique peak power scaling potential in nonlinear pulse compression.