Coal gangue accounts for the bulk of the solid waste produced during coal mining. Conventional gangue disposal methods often fail to meet the requirements of environmental protection regulations, making it necessary to broaden the approach used in the disposal of coal gangue. The research aims to explore the feasibility of using gangue to displace coarse aggregates to prepare underground roadway shotcrete. Key performance indicators, including the slump, compressive strength, and tensile strength of the gangue‐based shotcrete with different mixing proportions, were tested. Influences of factors including the cement content, water‐cement ratio, and accelerator content on the performance of gangue‐based shotcrete were analyzed, the optimal mixing proportion of the shotcrete was determined, and a nonlinear prediction model for the strength of the shotcrete was established. Results show that Group O‐4 has the optimal mixing proportion of gangue‐based shotcrete, that is, the cement content, water–cement ratio, and accelerator content are separately 450 kg·m −3 , 0.55, and 4%. Under that mix design, the slump, compressive strength, and tensile strength are 116 mm, 25.8 MPa, and 2.09 MPa, respectively. A multifactor coupling model was built based on orthogonal test data, and a predictive model for the compressive and tensile strengths of gangue‐based shotcrete was obtained through nonlinear regression and fitting. The research provides a theoretical basis and technical support for the use of solid‐waste coal gangue. Finally, the influences of the particle size of gangue on the performance of the shotcrete were analyzed, and the optimal particle size range of gangue was determined to be 0–10 mm.