This study presents an inkjet-printed, single-step double layer electrode with an acrylate adhesion layer on PES to enhance Ag adhesion. The electrode offers strong mechanical stability and a simplified solution for flexible device applications.

Digital printing technologies—including inkjet printing, aerosol jet printing, and electrohydrodynamic jet printing—have emerged as promising strategies for next-generation electronic devices. However, the weak adhesion between printed electrodes and substrates can lead to electrode delamination, thereby compromising device reliability and lifetime. In this study, a dielectric interlayer was introduced to improve the adhesion of silver (Ag) mesh electrodes on glass, polyethersulfone film, and polyimide film substrates. The optimized electrode on PES film achieved an optical transmittance of 83% at 550 nm and line resistance of 0.3 Ω, confirming its suitability as a transparent electrode. The incorporation of the interlayer also enhanced the adhesion and mechanical flexibility across all substrates. Moreover, the printed electrodes exhibited uniform surface heating under an applied bias (≤DC 3 V), and their feasibility as low-power flexible transparent heaters was experimentally demonstrated. These findings present a simple and effective printing strategy for fabricating robust and multifunctional electrodes, offering enormous potential for the realization of future flexible and transparent electronic systems.