Isolated terawatt (TW) attosecond (as) hard X-ray pulse is greatly desired for four-dimensional investigations of natural phenomena with picometer spatial and attosecond temporal resolutions. Since the demand for such sources is continuously increasing, the possibility of generating such pulse by a single current spike without the use of optical or electron delay units in an undulator line is addressed. The conditions of a current spike (width and height) and a modulation laser pulse (wavelength and power) is also discussed. We demonstrate that an isolated TW-level as a hard X-ray can be produced by a properly chosen single current spike in an electron bunch with simulation results. By using realistic specifications of an electron bunch of the Pohang Accelerator Laboratory X-ray Free-Electron Laser (PAL-XFEL), we show that an isolated, >1.0 TW and ~36 as X-ray pulse at 12.4 keV can be generated in an optimized-tapered undulator line. This result opens a new vista for current XFEL operation: the attosecond XFEL.

The X-ray free-electron laser of the Pohang Accelerator Laboratory (PAL-XFEL) was opened to users in 2017. Since then, significant progress has been made in PAL-XFEL operation and beamline experiments. This includes increasing the FEL pulse energy, increasing the FEL photon energy, generating self-seeding FEL, and trials of two-color operation. In the beamline, new instruments or endstations have been added or are being prepared. Overall, beamline operation has been stabilized since its initiation, which has enabled excellent scientific results through efficient user experiments. In this paper, we describe details of the recent progress of the PAL-XFEL.

The isolated terawatt (TW) attosecond (as) hard X-ray pulse will expand the scope of ultrafast science, including the examination of phenomena that have not been studied before, such as the dynamics of electron clouds in atoms, single-molecule imaging, and examining the dynamics of hollow atoms. Therefore, several schemes for the generation of an isolated TW-as X-ray pulse in X-ray free electron laser (XFEL) facilities have been proposed with the manipulation of electron properties such as emittance or current. In a multi-spike scheme, a series of current spikes were employed to amplify the X-ray pulse. A single-spike scheme in which a TW-as X-ray pulse can be generated by a single current spike was investigated for ideal parameters for the XFEL machine. This paper reviews the proposed schemes and assesses the feasibility of each scheme.

A Hanbury Brown and Twiss interferometry experiment based on second-order correlations was performed at the PAL-XFEL facility. The statistical properties of the X-ray radiation were studied within this experiment. Measurements were performed at the NCI beamline at 10 keV photon energy under various operation conditions: self-amplified spontaneous emission (SASE), SASE with a monochromator, and self-seeding regimes at 120 pC, 180 pC and 200 pC electron bunch charge. Statistical analysis showed short average pulse duration from 6 fs to 9 fs depending on the operational conditions. A high spatial degree of coherence of about 70–80% was determined in the spatial domain for the SASE beams with the monochromator and self-seeding regime of operation. The obtained values describe the statistical properties of the beams generated at the PAL-XFEL facility.

Attosecond (asec) X-ray free-electron laser (XFEL) has attracted considerable interest over the past years. Nowadays typical XFEL application experiments demand 10¹⁰–10¹¹ photons per pulse, which corresponds to a peak power of terawatts (TW) in case of asec hard X-ray pulse. To the realization of such TW asec-XFEL pulse, however, the unavoidable increase of slice energy spread (SES) due to laser heater, which is commonly used to mitigate the micro-bunching instability (MBI), would be a major obstacle. To deal with this problem, the effect of such a SES is investigated in this work. The results reveal that (1) SES of a current spike is linearly proportional to the peak current of a current spike in an electron beam, (2) surprisingly, this linearity is independent of the wavelength of an energy modulation driving laser which is used to make a current spike and (3) the gain length of current spike in the undulator is sensitive to the initial SES, so there is an optimal peak current of the current spike for successful FEL lasing process. Utilizing these characteristics, a series of simulations with parameters for Pohang Accelerator Laboratory X-ray Free Electron Laser was carried out to demonstrate that an isolated, TW asec-XFEL pulse can be generated even when the SES is increased due to the usage of laser heater to prevent the MBI in the XFEL. We show that an isolated X-ray pulse with >1 TW and a pulse duration of 73 as (~3 × 10¹⁰ photons/pulse at 12.4 keV or 0.1 nm) can be generated by using ten current spikes with optimal peak current. It becomes clear for the first time that the disadvantage from the increased SES can be indeed overcome.