We review the progress in the investigation of the Verdet constant of new magneto-active materials for the Faraday-effect-based devices used in high-power laser systems. A practical methodology for advanced characterization of the Verdet constant of these materials is presented, providing a useful tool for benchmarking the new materials. The experimental setup used for the characterization is a flexible and robust tool for evaluating the Faraday rotation angle induced in the magneto-active material, from which the Verdet constant is calculated based on the knowledge of the magnetic field and the material sample parameters. A general model for describing the measured Verdet constant data as a function of wavelength and temperature is given. In the final part of this review, we present a brief overview of several magneto-active materials, which have been to-date reported as promising candidates for utilization in the Faraday devices. This overview covers room-temperature investigations of the Verdet constant of several materials, which could be used for the ultraviolet, visible, near-infrared and mid-infrared wavelengths.

A high-contrast high-intensity petawatt-class Ti:sapphire chirped-pulse amplification laser has been developed for research on high field science. A saturable absorber and a low-gain optical parametric chirped-pulse amplification preamplifier in the front-end have improved the temporal contrast in the system to ∼ $2 \times 10^{12}$ on the subnanosecond time scale at the ∼70 TW power level. In addition to the high-contrast broadband high-energy output from the final amplifier has been achieved with a flat-top spatial profile with a filling factor of ∼70%. This is the result of pump beam spatial profile homogenization with diffractive optical elements. The system produces the uncompressed output pulse energy of 29 J, indicating the capability for reaching a peak power of ∼600 TW. We discuss in detail the design, performance, and characterization of the laser including output power, pulse duration, and spatiotemporal beam quality. We also describe the on-going upgrade of the laser system and some applications for the laser in relativistic dominated laser–matter interactions.

An overview of the latest developments of kilowatt-level diode pumped solid state lasers for advanced applications at the HiLASE Centre is presented. An overview of subcontracted and in-house-developed laser beamlines is presented. The aim of development is to build kW-class beamlines delivering picosecond pulses between 1- and 100-kHz repetition rates and high-energy nanosecond pulses at 10 Hz. The picosecond beamlines are based on Yb:YAG thin-disk amplifiers and chirped pulse amplification. The current status of the beamlines’ performance is reported. The advantages of zero-phonon line and pulsed pumping are demonstrated with respect to efficiency, thin disk temperature and beam quality. New diagnostics methods supporting the high average power lasers’ development, such as the high-resolution spectroscopy of Yb-doped materials, in situ thin disk deformation measurements, single-shot M² measurement, realization of wavefront correction by a deformable mirror and the laser performance of a new mixed garnet ceramics, are described. The energetic, thermal and fluid-mechanical numerical modeling for the optimization of the multi-slab amplifiers is also described.

The relatively narrow choice of magneto-active materials that could be used to construct Faraday devices (such as rotators or isolators) for the mid-infrared wavelengths arguably represents a pressing issue that is currently limiting the development of the mid-infrared lasers. Furthermore, the knowledge of the magneto-optical properties of the yet-reported mid-infrared magneto-active materials is usually restricted to a single wavelength only. To address this issue, we have dedicated this work to a comprehensive investigation of the magneto-optical properties of both the emerging (Dy${}_2$O${}_3$ ceramics and CeF${}_3$ crystal) and established (Y${}_3$Fe${}_5$O${}_{12}$ crystal) mid-infrared magneto-active materials. A broadband radiation source was used in a combination with an advanced polarization-stepping method, enabling an in-depth analysis of the wavelength dependence of the investigated materials’ Faraday rotation. We were able to derive approximate models for the examined dependence, which, as we believe, may be conveniently used for designing the needed mid-infrared Faraday devices for lasers with the emission wavelengths in the 2-$\mathsf{\mu }\mathrm{m}$ spectral region. In the case of Y${}_3$Fe${}_5$O${}_{12}$ crystal, the derived model may be used as a rough approximation of the material’s saturated Faraday rotation even beyond the 2-$\mathsf{\mu }\mathrm{m}$ wavelengths.

Temperature and wavelength dependence of the Verdet constant of dysprosium sesquioxide ($\mathrm{{{Dy}_2}{{O}_3}}$) transparent ceramics has been measured for the temperatures ranging from cryogenic $20\,\mathrm {K}$ up to room temperature $297\,\mathrm {K}$ and for the wavelength range starting from visible $0.6\,\mathrm {{\mu }m}$ up to mid-infrared $2.3\,\mathrm {{\mu }m}$. Several absorption bands corresponding to the electronic transitions in $\mathrm{{{Dy}_2}{{O}_3}}$ have been identified and removed from the data analysis due to high absorption of the matching wavelengths within these absorption bands. The Verdet constant data has been fitted by the multi-transition model function covering the whole temperature and wavelength range. Such fitted function could be used for the detailed design of magneto-optical devices as well as for the analysis of physical properties of the material itself.

Potassium terbium fluoride K T b 3 F 10 (KTF) crystal is a promising magneto-active material for creating multi-kilowatt average-power Faraday isolators operating at the visible and near-infrared wavelengths. Nevertheless, the key material’s parameter needed for the design of any Faraday isolator—the Verdet constant, has not been comprehensively investigated yet. In this Letter, we report on measurement of the Verdet constant of the KTF crystal for wavelengths between 600 and 1500 nm and for temperatures ranging from 15 to 295 K. A suitable model for the Verdet constant as a function of wavelength and temperature has been developed and may be conveniently used for optimal design of KTF-based high-average-power Faraday isolators.