Electromagnetic field confinement is crucial for nanophotonic technologies, since it allows for enhancing light–matter interactions, thus enabling light manipulation in deep sub‐wavelength scales. In the terahertz (THz) spectral range, radiation confinement is conventionally achieved with specially designed metallic structures—such as antennas or nanoslits—with large footprints due to the rather long wavelengths of THz radiation. In this context, phonon polaritons—light coupled to lattice vibrations—in van der Waals (vdW) crystals have emerged as a promising solution for controlling light beyond the diffraction limit, as they feature extreme field confinements and low optical losses. However, experimental demonstration of nanoscale‐confined phonon polaritons at THz frequencies has so far remained elusive. Here, it is provided by employing scattering‐type scanning near‐field optical microscopy combined with a free‐electron laser to reveal a range of low‐loss polaritonic excitations at frequencies from 8 to 12 THz in the vdW semiconductor α‐MoO₃. In this study, THz polaritons are visualized with: i) in‐plane hyperbolic dispersion, ii) extreme nanoscale field confinement (below λ_o ⁄75), and iii) long polariton lifetimes, with a lower limit of >2 ps.

Structural anisotropy in crystals is crucial for controlling light propagation, particularly in the infrared spectral regime where optical frequencies overlap with crystalline lattice resonances, enabling light-matter coupled quasiparticles called phonon polaritons (PhPs). Exploring PhPs in anisotropic materials like hBN and MoO₃ has led to advancements in light confinement and manipulation. In a recent study, PhPs in the monoclinic crystal β-Ga₂O₃ (bGO) were shown to exhibit strongly asymmetric propagation with a frequency dispersive optical axis. Here, using scanning near-field optical microscopy (s-SNOM), we directly image the symmetry-broken propagation of hyperbolic shear polaritons in bGO. Further, we demonstrate the control and enhancement of shear-induced propagation asymmetry by varying the incident laser orientation and polariton momentum using different sizes of nano-antennas. Finally, we observe significant rotation of the hyperbola axis by changing the frequency of incident light. Our findings lay the groundwork for the widespread utilization and implementation of polaritons in low-symmetry crystals.

We present the characterization of a Zero-bias Schottky diode-based Terahertz (THz) detector up to 5.56 THz. The detector was operated with both a table-top system until 1.2 THz and at a Free-Electron Laser (FEL) facility at singular frequencies from 1.9 to 5.56 THz. We used two measurement techniques in order to discriminate the sub-ns-scale (via a 20 GHz oscilloscope) and the ms-scale (using the lock-in technique) responsivity. While the lock-in measurements basically contain all rectification effects, the sub-ns-scale detection with the oscilloscope is not sensitive to slow bolometric effects caused by changes of the IV characteristic due to temperature. The noise equivalent power (NEP) is 10 pW/$\sqrt{\mathrm{Hz}}$ in the frequency range from 0.2 to 0.6 THz and 17 pW/$\sqrt{\mathrm{Hz}}$ at 1.2 THz and increases to 0.9 $\mathsf{\mu }$W/$\sqrt{\mathrm{Hz}}$ at 5.56 THz, which is at the state of the art for room temperature zero-bias Schottky diode-based THz detectors with non-resonant antennas. The voltage and current responsivity of ∼500 kV/W and ∼100 mA/W, respectively, is demonstrated over a frequency range of 0.2 to 1.2 THz with the table-top system.

At the electron linac for beams with high brilliance and low emittance (ELBE) center for high-power radiation sources, the second version of a superconducting radio-frequency (SRF) photoinjector has been put into operation and has been routinely applied for user operation at the ELBE electron accelerator. SRF guns are suitable for generating a continuous wave electron beam with high average currents and high beam brightness. The SRF gun at ELBE has the goal to generate short electron pulses with bunch charges of 200–300 pC at typical repetition rates of 100 kHz for the production of superradiant, coherent terahertz radiation. The SRF gun includes a 3.5-cell, 1.3-GHz niobium cavity and a superconducting solenoid. A support system with liquid nitrogen (${\mathrm{LN}}_2$) cooling allows the operation of normal-conducting, high quantum efficiency photocathodes. We present the design and performance of the SRF gun as well as beam measurement results of the operation with Mg photocathodes at an acceleration gradient of $8\mathrm{MV}/\mathrm{m}$ (4 MeV kinetic energy). In the last section, we discuss the SRF gun application for production of coherent terahertz radiation at the ELBE facility.

The vast repository of van der Waals (vdW) materials supporting polaritons offers numerous possibilities to tailor electromagnetic waves at the nanoscale. The development of twistoptics—the modulation of the optical properties by twisting stacks of vdW materials—enables directional propagation of phonon polaritons (PhPs) along a single spatial direction, known as canalization. Here we demonstrate a complementary type of directional propagation of polaritons by reporting the visualization of unidirectional ray polaritons (URPs). They arise naturally in twisted hyperbolic stacks with very different thicknesses of their constituents, demonstrated for homostructures of $$\alpha$$α -MoO₃ and heterostructures of $$\alpha$$α -MoO₃ and $$\beta$$β -Ga₂O₃. Importantly, their ray-like propagation, characterized by large momenta and constant phase, is tunable by both the twist angle and the illumination frequency. Apart from their fundamental importance, our findings introduce twisted asymmetric stacks as efficient platforms for nanoscale directional polariton propagation, opening the door for applications in nanoimaging, (bio)-sensing, or polaritonic thermal management.

We study the photoinduced metallization process in niobium dioxide ${\mathrm{NbO}}_2$. This compound undergoes the thermal insulator-to-metal transition at the remarkably high temperature of 1080 K. Our optical pump-terahertz probe measurements reveal the ultrafast switching of the film on a subpicosecond timescale and the formation of a metastable metallic phase when the incident pump fluence exceeds the threshold of $\sim 10\mathrm{mJ}/\mathrm{c}{\mathrm{m}}^2$. Remarkably, this threshold value corresponds to the deposited energy which is capable of heating ${\mathrm{NbO}}_2$ only up to 790 K, thus, evidencing the nonthermal character of the photoinduced insulator-to-metal transition. We also observe an enhanced formation of the metallic phase above the second threshold of $\sim 17.5\mathrm{mJ}/\mathrm{c}{\mathrm{m}}^2$ which corresponds to the onset of the thermal switching. The transient optical conductivity in the metastable phase can be modeled using the Drude-Smith model confirming its metallic character. The present observation of nonthermal transition evidences a leading role played by electronic correlations in ${\mathrm{NbO}}_2$ and can serve as an important test bed for understanding photoinduced phenomena in strongly correlated oxides.