High Voltage and Discharge Plasma Laboratory, Beijing International S&T Cooperation Base for Plasma Science and Energy Conversion, Institute of Electrical Engineering, Chinese Academy of Sciences, Beijing 100190, China
Dr. Cheng Zhang
High Voltage and Discharge Plasma Laboratory, Beijing International S&T Cooperation Base for Plasma Science and Energy Conversion, Institute of Electrical Engineering, Chinese Academy of Sciences, Beijing 100190, China
Persistent pharmaceutical pollutants (PPPs) have been identified as potential endocrine disruptors that mimic growth hormones when consumed at nanogram per litre to microgram per litre concentrations. Their occurrence in potable water remains a great threat to human health. Different conventional technologies developed for their removal from wastewater have failed to achieve complete mineralisation. Advanced oxidation technologies such as dielectric barrier discharges (DBDs) based on free radical mechanisms have been identified to completely decompose PPPs. Due to the existence of pharmaceuticals as mixtures in wastewater and the recalcitrance of their degradation intermediate by-products, no single advanced oxidation technology has been able to eliminate pharmaceutical xenobiotics. This review paper provides an update on the sources, occurrence, and types of pharmaceuticals in wastewater by emphasising different DBD configurations previously and currently utilised for pharmaceuticals degradation under different experimental conditions. The performance of the DBD geometries was evaluated considering various factors including treatment time, initial concentration, half-life time, degradation efficiency and the energy yield (G50) required to degrade half of the pollutant concentration. The review showed that the efficacy of the DBD systems on the removal of pharmaceutical compounds depends not only on these parameters but also on the nature/type of the pollutant.
26 March 2020 in Plasma Sources Science and Technology
In this work, the propagation of the surface ionization wave (SIW) in the nanosecond pulsed surface dielectric barrier discharge with different dielectric materials and pulse repetition rates is investigated. The current waveforms at different locations along the route of the SIW propagation are obtained, based on a specially designed ground strip array geometry. The temporal evolution and spatial distribution of the electric field during the SIW propagation are measured by using the electric field induced second harmonic generation method. The distribution of the residual surface potential after the discharge is mapped with a Kelvin electrostatic probe, which verifies both the existence of the residual electric field and its opposite direction to that during the SIW propagation. It is found that with the dielectric material on which the surface charges decay faster, there are the well-pronounced primary and secondary SIWs with a higher velocity on the voltage rising edge and both the peak current and the peak electric field are also higher, with a less spatial attenuation along the SIW propagation route. It is demonstrated that the residual surface charges with the same polarity as the high-voltage pulse suppress the development of the SIW.
29 May 2019 in Plasma Sources Science and Technology
Pulsed plasma actuators are used for an active flow control application since the 2000s. In this paper, we discuss shock wave and vortex characteristics in pulsed plasma actuators after an introduction of research progress on atmospheric-pressure discharge plasma actuators. First, the shock wave characteristics in surface dielectric barrier discharge (SDBD) actuator operating in diffuse-like and multi-streamer modes are discussed. In the most general case, a shock wave in a diffuse-like SDBD actuator is stronger and faster than in a multi-streamer SDBD actuator. Improved plasma actuators, such as the three-electrode SDBD actuator and the plasma synthetic jet actuator have the enhanced shock wave characteristics. Second, in order to investigate the effects of pulse parameters on the shock wave characteristics in nanosecond-pulse SDBD actuator, a particle image velocimetry system is used to capture the formation of starting vortexes at different pulse rise times, pulse durations, and pulse repetition frequencies (PRFs). It is shown that the velocity of a starting vortex significantly increases when the pulse rise time decreases from 400 ns to 50 ns due to a more significant hydrodynamic effect generated during a shorter rise time. This phenomenon is confirmed by calculating a reduced electric field E/N at a short rise time, which turns out to be higher at a shorter rise time than that at a relatively longer rise time. It is also shown that the velocity of a starting vortex increases and its active area enlarges when the PRF increases.
Triboelectric nanogenerator (TENG) operates on the principle of utilizing contact electrification and electrostatic induction. However, visualization and standardized quantification of surface charges for triboelectric materials remain challenging. Here, we report a surface charge visualization and standardized quantification method using electrostatic surface potential measured by Kevin probe and the iterative regularization strategy. Moreover, a tuning strategy on surface charge is demonstrated based on the corona discharge with a three-electrode design. The long-term stability and dissipation mechanisms of the injected negative or positive charges demonstrate high dependence on deep carrier traps in triboelectric materials. Typically, we achieved a 70-fold enhancement on the output voltage (~135.7 V) for the identical polytetrafluoroethylene (PTFE) based TENG (neg-PTFE/PTFE or posi-PTFE/PTFE triboelectric pair) with stable surface charge density (5% decay after 140 days). The charged PTFE was demonstrated as a robot e-skins for non-contact perception of object geometrics. This work provides valuable tools for surface charge visualization and quantification, giving a new strategy for a deeper understanding of contact electrification.
Typical ionization waves (IWs) are observed during the propagation of nanosecond pulsed atmospheric pressure plasma jets (APPJs) with argon flow, combining both the measurement of the axial electric field ( Ez ) and the temporal resolved optical imaging. The movement of the luminous APPJ head is recognized as the development of the IW front, accompanied with the propagation of the peak electric field. Especially, the radial distribution of Ez transits from a central peak profile before the IW front arrives to a hollow profile after the pass of the IW front. As for the temporal Ez trend, there is a mode transition from the single‐peak feature under a low peak voltage to the double‐peak feature under a higher peak voltage, indicating the existence of both primary and secondary IWs. The effect of target conditions on the IWs in APPJs is also explored. With a metal target, no residual electric field is observed before imposing the high‐voltage pulses. However, with a dielectric target, the residual surface charges generate a background electric field in the opposite direction to that during IW propagation. In the free APPJ (with no target), on the voltage falling edge, a negative electric field drives the electron flow to compensate the positive ions left over during the forward IW propagation on the voltage rising edge.