The aerosol hygroscopic growth (HG) characteristics in coastal areas are very complex, which is one of the main influences on the simulation accuracy of radiation transfer modeling for coastal environments. Previous studies have shown that aerosol HG characteristics are very different in open oceans and inland regions. However, the aerosol HG features in coastal areas are strongly affected by its type. In this work, an aerosol backward trajectory tracing model was used to classify the local aerosol type. Using long-term field campaign data in Qingdao (25 September 2019 to 25 October 2020), the HG characteristics of different types of aerosols (i.e., land source, sea source, and mixed aerosol) under different seasons and different atmospheric environments (i.e., pollution background and clean background) were studied. Quantitative models of aerosol HG factor were established for aerosols from different sources in different seasons and under different pollution background conditions. The major type of local aerosol is terrestrial aerosol, as the marine source only accounts for 10–20%. Seasonal HG characteristics (deliquescence point, DP) of mixed and land source aerosol vary significantly, from around RH = 60% to RH = 85%, while that of the marine aerosol is rather consistent (RH = 80%). When the atmospheric background is relatively clean, the DPs of aerosols from different sources are almost the same (about RH = 80%), but when the pollution is heavy, the DPs of terrestrial aerosols are almost 20% lower than those of marine sources. These models can be directly used to characterize the hygroscopic characteristics of atmospheric aerosols in Qingdao at specific seasons or pollution levels for radiative transfer modeling, remote sensing, and so forth.

Above-low-level-cloud aerosols (ACAs) have gradually gained more interest in recent years; however, the combined aerosol–cloud radiation effects are not well understood. The uncertainty about the radiative effects of aerosols above cloud mainly stems from the lack of comprehensive and accurate retrieval of aerosols and clouds for ACA scenes. In this study, an improved ACA identification and retrieval methodology was developed to provide a new global view of the ACA distribution by combining three-channel CALIOP (The Cloud–Aerosol Lidar with Orthogonal Polarization) observations. The new method can reliably identify and retrieve both thin and dense ACA layers, providing consistent results between the day- and night-time retrieval of ACAs. Then, new four-year (2007 to 2010) global ACA datasets were built, and new seasonal mean views of global ACA occurrence, optical depth, and geometrical thickness were presented and analyzed. Further discussion on the relative position of ACAs to low clouds showed that the mean distance between the ACA layer and the low cloud deck over the tropical Atlantic region is less than 0.2 km. This indicates that the ACAs over this region are more likely to be mixed with low-level clouds, thereby possibly influencing the cloud microphysics over this region, contrary to findings reported from previous studies. The results not only help us better understand global aerosol transportation and aerosol–cloud interactions but also provide useful information for model evaluation and improvements.

In order to investigate the equivalent complex refractive index of atmospheric aerosols near the Earth’s surface, we conducted measurements in the Hefei region from March to April 2022. These measurements utilized a micro-pulse lidar, an Aethalometer, and a Portable Optical Particle Profiler. These measurements encompassed aerosol particle size distribution as well as standard meteorological parameters including temperature, humidity, atmospheric pressure, and wind speed. Subsequently, this dataset was employed to develop an optimization algorithm for retrieving the equivalent complex refractive indices of near-surface aerosols. The methodology relies on lookup tables containing data for extinction efficiency and absorption efficiency factors. It operates on the premise of aerosol property stability within a defined time frame, utilizing measured extinction and absorption coefficients as simultaneous constraints during this period to inversely derive both the real and imaginary parts of the aerosol complex refractive index. Results from the simulation analysis reveal that the newly optimized retrieval algorithm, which relies on lookup tables, exhibits reduced sensitivity to instrument errors when compared to single-point constraint algorithms. This enhancement results in a more efficient and dependable approach for retrieving the aerosol complex refractive index. Empirical inversion and simulation studies were carried out to determine the aerosol equivalent complex refractive index in the Hefei region, utilizing measured data. This inversion process yielded an average complex refractive index of 1.48-i0.017 for aerosols in the Hefei region throughout the experimental period. Correlation analysis unveiled a positive association between the real part of the aerosol complex refractive index and the single-scattering albedo (SSA), whereas the imaginary part displayed a linear negative correlation with the SSA. The mathematical relationship between the real part and the SSA is $y=0.19x+0.62$, and the corresponding relationship between the imaginary part and the SSA is $y=-5.3x+0.99$. This research offers a novel method for the retrieval of the aerosol equivalent complex refractive index.

A regional aerosol model can complement globally averaged models and improve the accuracy of atmospheric numerical models in local applications. This study established a seasonal aerosol model based on data from the Aerosol Robotic Network (AERONET) of the sea area around eastern China, and its performance in calculating the aerosol optical depth (AOD) was evaluated. The seasonal columnar volume particle size distributions (VPSDs) illustrated a bimodal structure consisting of fine and coarse modes. The VPSDs of spring, autumn, and winter roughly agreed with each other, with their amplitudes of fine and coarse modes being almost equal; however, the fine mode of the summer VPSD was approximately twice as high as that of the coarse mode. Lognormal mode decomposition analysis revealed that fine and coarse modes comprised two sub-modes. Fitting the seasonal VPSDs to the four-mode lognormal distribution yielded a parameterized aerosol size distribution model. Furthermore, seasonal variations in complex refractive indices (CRIs) indicated unignorable changes in aerosol compositions. Overall, error analysis validated that the proposed model could meet accuracy requirements for optical engineering applications, with median AOD calculation errors of less than 0.01.