Using NASA's A‐Train satellite measurements, we evaluate the accuracy of cloud water content (CWC) and water vapor mixing ratio (H₂O) outputs from 19 climate models submitted to the Phase 5 of Coupled Model Intercomparison Project (CMIP5), and assess improvements relative to their counterparts for the earlier CMIP3. We find more than half of the models show improvements from CMIP3 to CMIP5 in simulating column‐integrated cloud amount, while changes in water vapor simulation are insignificant. For the 19 CMIP5 models, the model spreads and their differences from the observations are larger in the upper troposphere (UT) than in the lower or middle troposphere (L/MT). The modeled mean CWCs over tropical oceans range from ∼3% to ∼15× of the observations in the UT and 40% to 2× of the observations in the L/MT. For modeled H₂Os, the mean values over tropical oceans range from ∼1% to 2× of the observations in the UT and within 10% of the observations in the L/MT. The spatial distributions of clouds at 215 hPa are relatively well‐correlated with observations, noticeably better than those for the L/MT clouds. Although both water vapor and clouds are better simulated in the L/MT than in the UT, there is no apparent correlation between the model biases in clouds and water vapor. Numerical scores are used to compare different model performances in regards to spatial mean, variance and distribution of CWC and H₂O over tropical oceans. Model performances at each pressure level are ranked according to the average of all the relevant scores for that level.

Convective clouds produce a significant proportion of the global precipitation and play an important role in the energy and water cycles. We quantify changes of the convective cloud ice mass-weighted altitude centroid (Z_IWC) as a function of aerosol optical thickness (AOT). Analyses are conducted in smoke, dust and polluted continental aerosol environments over South America, Central Africa and Southeast Asia, using the latest measurements from the CloudSat and CALIPSO satellites. We find aerosols can inhibit or invigorate convection, depending on aerosol type and concentration. On average, smoke tends to suppress convection and results in lower Z_IWC than clean clouds. Polluted continental aerosol tends to invigorate convection and promote higher Z_IWC. The dust aerosol effects are regionally dependent and their signs differ from place to place. Moreover, we find that the aerosol inhibition or invigoration effects do not vary monotonically with AOT and the variations depend strongly on aerosol type. Our observational findings indicate that aerosol type is one of the key factors in determining the aerosol effects on convective clouds.

Our knowledge is still poor regarding the response of the precipitation vertical structure to aerosols, partly due to the ignorance of precipitation occurring at different spatial scales. A total of 6 years of collocated ground-based PM₁₀ and satellite-based (Tropical Rainfall Measuring Mission, TRMM) radar data, along with ERA-Interim reanalysis, are used in this study to investigate the aerosol effects on three localized rain regimes (shallow, stratiform, and convective rain) over the Pearl River Delta region of China. A subjective analysis method is proposed to discriminate between the localized and synoptic-scale precipitations based on weather composite charts where daily averaged wind field at 850 hPa is overlaid with the geopotential height at 500 hPa. In general, average rain rate tends to be greater under polluted conditions than under clean conditions. But such potential aerosol effects are regime dependent: as the atmosphere becomes slightly polluted (PM₁₀≤38 µg m⁻³), the top 1 % radar reflectivity (Z) for all regimes initially increases, followed by continued increases and weak decreases for convective and stratiform/shallow rain regimes, respectively. As the atmosphere becomes much more polluted, such regime dependences of aerosol effects are more significant. From a perspective of the vertical Z structure, comparisons between polluted conditions (days with the highest third of PM₁₀ concentration) and clean conditions (days with the lowest third of PM₁₀ concentration) show that the convective rain regime exhibits a deeper and stronger Z pattern, whereas a much shallower and weaker Z pattern is observed for stratiform and shallow precipitation regimes. In particular, the top height of the 30 dBZ rain echo increases by ∼29 % (∼1.27 km) for the convective regime, but decreases by ∼10.8 % (∼0.47 km) for the stratiform regime. However, no noticeable changes are observed for the shallow precipitation regime. Impacts of meteorological factors are further studied on both rain top height (RTH) and the center of gravity of Z, including vertical velocity, vertical wind shear, convection available potential energy, and vertically integrated moisture flux divergence (MFD). The possible invigoration effect on convective precipitation seems dependent on wind shear, in good agreement with previous findings. Overall, the observed dependence of the precipitation vertical structure on ground-based PM₁₀ supports the notion of aerosol invigoration or suppression effect on cold or warm rain and adds new insights into the nature of the complex interactions between aerosol and various localized precipitation regimes.

The seasonal and regional variations of cloud fractions are compared across two generations of global climate model ensembles, specifically, the Coupled Model Intercomparison Project‐5 (CMIP5) and CMIP6, through the historical period in terms of skills and multimodel agreement. We find a wider spread of historical cloud fraction changes in the CMIP6 than was simulated by the CMIP5. The global mean cloud fractions of CMIP6 increased by about 4.5% from the CMIP5, which attributed to greater changes in the northern hemisphere than in the southern hemisphere. The CMIP6 cloud fractions in recent years are validated with the CALIPSO_CLOUSAT observations to understand the cloud fraction uncertainties in CMIP6 models. The CMIP6 ensemble mean of cloud fractions compares well with the observations with a mean difference of 0.5% in lower altitudes. The CMIP6 cloud fractions are higher than the observations at higher latitudes in both hemispheres in the upper troposphere, and the biases vary from one model to another. The spatial difference between the ensemble and observations is further revealed over the tropics: where the model displays a 3% higher bias. In addition, we observed a significant trend occuring in the northern hemisphere since the mid‐20th century using calculations of cloud fraction trends based on the robust regression technique. Finally, we reduce the differences between the model and observations by applying a simple regression technique. The results exemplify that the model and modified observations compare well, with the root mean square value decreased by nearly 28%, and the correlation increased significantly.

The geographical shift of global anthropogenic aerosols from the developed countries to the Asian continent since the 1980s could potentially perturb the regional and global climate due to aerosol‐cloud‐radiation interactions. We use an atmospheric general circulation model with different aerosol scenarios to investigate the radiative and microphysical effects of anthropogenic aerosols from different regions on the radiation budget, precipitation, and large‐scale circulations. An experiment contrasting anthropogenic aerosol scenarios in 1970 and 2010 shows that the altered cloud reflectivity and solar extinction by aerosols results in regional surface temperature cooling in East and South Asia, and warming in the US and Europe, respectively. These aerosol‐induced temperature changes are consistent with the relative temperature trends from 1980 to 2010 over different regions in the reanalysis data. A reduced meridional streamfunction and zonal winds over the tropics as well as a poleward shift of the jet stream suggest weakened and expanded tropical circulations, which are induced by the redistributed aerosols through a relaxing of the meridional temperature gradient. Consequently, precipitation is suppressed in the deep tropics and enhanced in the subtropics. Our assessments of the aerosol effects over the different regions suggest that the increasing Asian pollution accounts for the weakening of the tropics circulation, while the decreasing pollution in Europe and US tends to shift the circulation systems southward. Moreover, the aerosol indirect forcing is predominant over the total aerosol forcing in magnitude, while aerosol radiative and microphysical effects jointly shape the meridional energy distributions and modulate the circulation systems.