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Ms. Natalia Zioła
Institute of Environmental Engineering of the Polish Academy of Sciences, 34 M. Skłodowska-Curie Str., 41-819 Zabrze, Poland

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0 Air Pollution
0 Pollution
0 Soot
0 environment
0 Black carbon

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Journal article
Published: 23 June 2021 in Atmosphere
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In recent years, black carbon (BC) has been gaining more attention due to the diversity of anthropogenic sources and the harmful effects on human health, environment, and climate. In this paper, for the first time in Poland, the results of long-term measurements of eBC concentrations (2009–2020) at the urban background station in Zabrze (southern Poland) are presented. A Multi-Angle Absorption Photometer (MAAP) was used, which enables the measurement of eBC concentration in fine particulate matter (PM2.5). The mean concentration of eBC over the 11-year period (3.82 μg·m−3) was higher compared to the values recorded at most European urban stations. Annual averaged eBC levels showed a downward trend and clear seasonal variations, which was caused mainly by changes in the intensity of anthropogenic emissions. The impact of meteorological parameters, in particular air temperature and wind speed, which determine the intensity of emissions and the conditions of pollutant dispersion, was not without significance. The work additionally attempts to assess the possible impact of remedial actions carried out in Zabrze over the last decade. The results showed that modernization in industry and heating and maintenance of green areas potentially had the most important impact on the decline in eBC concentrations.

ACS Style

Natalia Zioła; Barbara Błaszczak; Krzysztof Klejnowski. Long-Term eBC Measurements with the Use of MAAP in the Polluted Urban Atmosphere (Poland). Atmosphere 2021, 12, 808 .

AMA Style

Natalia Zioła, Barbara Błaszczak, Krzysztof Klejnowski. Long-Term eBC Measurements with the Use of MAAP in the Polluted Urban Atmosphere (Poland). Atmosphere. 2021; 12 (7):808.

Chicago/Turabian Style

Natalia Zioła; Barbara Błaszczak; Krzysztof Klejnowski. 2021. "Long-Term eBC Measurements with the Use of MAAP in the Polluted Urban Atmosphere (Poland)." Atmosphere 12, no. 7: 808.

Journal article
Published: 14 June 2021 in Atmosphere
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Raman microspectroscopy and thermo-optical-transmittance (TOT) method were used to study airborne ambient soot collected at the suburban air monitoring station in southern Poland during the residential heating (January-February) and non-heating (June–July) seasons of 2017. Carbonaceous material constituted on average 47.2 wt.% of PM2.5 during the heating season and 26.9 wt.% in the non-heating season. Average concentrations of OC (37.5 ± 11.0 μg/m3) and EC (5.3 ± 1.1 μg/m3) during the heating season were significantly higher than those in the non-heating season (OC = 2.65 ± 0.78 μg/m3, and EC = 0.39 ± 0.18 μg/m3). OC was a chief contributor to the TC mass concentration regardless of the season. All Raman parameters indicated coal combustion and biomass burning were the predominant sources of soot in the heating season. Diesel soot, which is structurally less ordered than soot from other sources, was dominant during the non-heating season. The D1 and G bands area ratio (D1A/GA) was the most sensitive Raman parameter that discriminated between various soot sources, with D1A/GA > 1 for diesel soot, and less than 1 for soot from coal and wood burning. Due to high daily variability of both TOT and Raman spectroscopy data, single-day measurements can be inconclusive regarding the soot source apportionment. Long-time measurement campaigns are recommended.

ACS Style

Natalia Zioła; Kamila Banasik; Mariola Jabłońska; Janusz Janeczek; Barbara Błaszczak; Krzysztof Klejnowski; Barbara Mathews. Seasonality of the Airborne Ambient Soot Predominant Emission Sources Determined by Raman Microspectroscopy and Thermo-Optical Method. Atmosphere 2021, 12, 768 .

AMA Style

Natalia Zioła, Kamila Banasik, Mariola Jabłońska, Janusz Janeczek, Barbara Błaszczak, Krzysztof Klejnowski, Barbara Mathews. Seasonality of the Airborne Ambient Soot Predominant Emission Sources Determined by Raman Microspectroscopy and Thermo-Optical Method. Atmosphere. 2021; 12 (6):768.

Chicago/Turabian Style

Natalia Zioła; Kamila Banasik; Mariola Jabłońska; Janusz Janeczek; Barbara Błaszczak; Krzysztof Klejnowski; Barbara Mathews. 2021. "Seasonality of the Airborne Ambient Soot Predominant Emission Sources Determined by Raman Microspectroscopy and Thermo-Optical Method." Atmosphere 12, no. 6: 768.

Journal article
Published: 30 April 2021 in Atmospheric Measurement Techniques
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Aerosolized black carbon is monitored worldwide to quantify its impact on air quality and climate. Given its importance, measurements of black carbon mass concentrations must be conducted with instruments operating in quality-checked and ensured conditions to generate data which are reliable and comparable temporally and geographically. In this study, we report the results from the largest characterization and intercomparison of filter-based absorption photometers, the Aethalometer model AE33, belonging to several European monitoring networks. Under controlled laboratory conditions, a total of 23 instruments measured mass concentrations of black carbon from three well-characterized aerosol sources: synthetic soot, nigrosin particles, and ambient air from the urban background of Leipzig, Germany. The objective was to investigate the individual performance of the instruments and their comparability; we analyzed the response of the instruments to the different aerosol sources and the impact caused by the use of obsolete filter materials and the application of maintenance activities. Differences in the instrument-to-instrument variabilities from equivalent black carbon (eBC) concentrations reported at 880 nm were determined before maintenance activities (for soot measurements, average deviation from total least square regression was −2.0 % and the range −16 % to 7 %; for nigrosin measurements, average deviation was 0.4 % and the range −15 % to 17 %), and after they were carried out (for soot measurements, average deviation was −1.0 % and the range −14 % to 8 %; for nigrosin measurements, the average deviation was 0.5 % and the range −12 % to 15 %). The deviations are in most of the cases explained by the type of filter material employed by the instruments, the total particle load on the filter, and the flow calibration. The results of this intercomparison activity show that relatively small unit-to-unit variability of AE33-based particle light absorbing measurements is possible with well-maintained instruments. It is crucial to follow the guidelines for maintenance activities and the use of the proper filter tape in the AE33 to ensure high quality and comparable black carbon (BC) measurements among international observational networks.

ACS Style

Andrea Cuesta-Mosquera; Griša Močnik; Luka Drinovec; Thomas Müller; Sascha Pfeifer; María Cruz Minguillón; Björn Briel; Paul Buckley; Vadimas Dudoitis; Javier Fernández-García; María Fernández-Amado; Joel Ferreira De Brito; Veronique Riffault; Harald Flentje; Eimear Heffernan; Nikolaos Kalivitis; Athina-Cerise Kalogridis; Hannes Keernik; Luminita Marmureanu; Krista Luoma; Angela Marinoni; Michael Pikridas; Gerhard Schauer; Norbert Serfozo; Henri Servomaa; Gloria Titos; Jesús Yus-Díez; Natalia Zioła; Alfred Wiedensohler. Intercomparison and characterization of 23 Aethalometers under laboratory and ambient air conditions: procedures and unit-to-unit variabilities. Atmospheric Measurement Techniques 2021, 14, 3195 -3216.

AMA Style

Andrea Cuesta-Mosquera, Griša Močnik, Luka Drinovec, Thomas Müller, Sascha Pfeifer, María Cruz Minguillón, Björn Briel, Paul Buckley, Vadimas Dudoitis, Javier Fernández-García, María Fernández-Amado, Joel Ferreira De Brito, Veronique Riffault, Harald Flentje, Eimear Heffernan, Nikolaos Kalivitis, Athina-Cerise Kalogridis, Hannes Keernik, Luminita Marmureanu, Krista Luoma, Angela Marinoni, Michael Pikridas, Gerhard Schauer, Norbert Serfozo, Henri Servomaa, Gloria Titos, Jesús Yus-Díez, Natalia Zioła, Alfred Wiedensohler. Intercomparison and characterization of 23 Aethalometers under laboratory and ambient air conditions: procedures and unit-to-unit variabilities. Atmospheric Measurement Techniques. 2021; 14 (4):3195-3216.

Chicago/Turabian Style

Andrea Cuesta-Mosquera; Griša Močnik; Luka Drinovec; Thomas Müller; Sascha Pfeifer; María Cruz Minguillón; Björn Briel; Paul Buckley; Vadimas Dudoitis; Javier Fernández-García; María Fernández-Amado; Joel Ferreira De Brito; Veronique Riffault; Harald Flentje; Eimear Heffernan; Nikolaos Kalivitis; Athina-Cerise Kalogridis; Hannes Keernik; Luminita Marmureanu; Krista Luoma; Angela Marinoni; Michael Pikridas; Gerhard Schauer; Norbert Serfozo; Henri Servomaa; Gloria Titos; Jesús Yus-Díez; Natalia Zioła; Alfred Wiedensohler. 2021. "Intercomparison and characterization of 23 Aethalometers under laboratory and ambient air conditions: procedures and unit-to-unit variabilities." Atmospheric Measurement Techniques 14, no. 4: 3195-3216.

Journal article
Published: 15 January 2021 in Atmosphere
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This study assesses the air quality in Zabrze (southern Poland) based on the ambient concentrations of equivalent black carbon (eBC). eBC measurement campaigns were carried out from April 2019 to March 2020 using a modern AE33 Aethalometer, accompanied by parallel measurements of gaseous pollutants, PM10 and meteorological parameters. The use of the two-component AE33 model allows for the determination of the eBC from fossil fuel combustion (eBCff) and biomass burning (eBCbb). The obtained results showed a clear seasonal variability of eBC concentrations, with higher average levels in the heating season (4.70 µg·m−3) compared to the non-heating one (1.79 µg·m−3). In both seasons, the eBCff component had a dominant share in total eBC, which indicates significant emissions from the combustion of fossil fuels for heating purposes and from local traffic sources. The obtained results showed high correlation coefficients with gaseous and particulate pollutants, with the strongest relationship for eBC and carbon monoxide (CO). During the non-heating and heating period, both anticyclone and cyclone systems played an important role in shaping eBC, eBCff and eBCbb concentrations. High concentrations of all components occurred with a significant decrease in air temperature and solar radiation in winter.

ACS Style

Natalia Zioła; Barbara Błaszczak; Krzysztof Klejnowski. Temporal Variability of Equivalent Black Carbon Components in Atmospheric Air in Southern Poland. Atmosphere 2021, 12, 119 .

AMA Style

Natalia Zioła, Barbara Błaszczak, Krzysztof Klejnowski. Temporal Variability of Equivalent Black Carbon Components in Atmospheric Air in Southern Poland. Atmosphere. 2021; 12 (1):119.

Chicago/Turabian Style

Natalia Zioła; Barbara Błaszczak; Krzysztof Klejnowski. 2021. "Temporal Variability of Equivalent Black Carbon Components in Atmospheric Air in Southern Poland." Atmosphere 12, no. 1: 119.

Preprint content
Published: 28 August 2020
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Airborne black carbon particles are monitored in many networks to quantify its impact on air quality and climate. Given its importance, measurements of black carbon mass concentrations must be conducted with instruments operating in a quality checked and assured conditions to generate reliable and comparable data. According to WMO (World Meteorological Organization) and GAW (Global Atmosphere Watch), intercomparisons against a reference instrument are a crucial part of quality controls in measurement activities (WMO, 2016). The WMO-GAW World Calibration Centre for Aerosol Physics (WCCAP) carried out several instrumental comparison and calibration workshops of absorption photometers in the frame of ACTRIS (European Research Infrastructure for the observation of Aerosol, Clouds and Trace Gases) and the COST Action COLOSSAL (Chemical On-Line cOmpoSition and Source Apportionment of fine aerosoL) in January and June 2019. The experiments were conducted to intercompare filter-based particle light absorption photometers, specifically aethalometers AE33 (Magee Scientific), which are operated by research institutions, universities or governmental entities across Europe. The objective was to investigate the individual performance of 23 instruments and their comparability, using synthetic aerosols in a controlled environment and ambient air from the Leipzig urban background. The methodology and results of the intercomparison are presented in this work. The observed instrument-to-instrument variabilities showed differences that were evaluated, before maintenance activities (average deviation from total least square regression: 1.1 %, range: −6 % to 16 %, for soot measurements; average deviation: 0.3 %, range: −14 % to 19 %, for nigrosin measurements), and after they were carried out (average deviation: 0.4 %, range: −8 % to 14 %, for soot measurements; average deviation: 1.1 %, range: −15 % to 11 %, for nigrosin measurements). The deviations are in most of the cases explained by the filter material, the total particles load on the filter, the performance of the flow systems and previous flow check and calibrations carried out with non-calibrated devices. The results of this intensive intercomparison activity show that relatively small unit-to-unit uncertainties of AE33-based particle light absorbing measurements are possible with functioning instruments. It is crucial to follow the guidelines for maintenance activities and the use of the proper filter tape in the AE33 to assure high quality and comparable BC measurements among international observational networks.

ACS Style

Andrea Cuesta-Mosquera; Griša Močnik; Luka Drinovec; Thomas Müller; Sascha Pfeifer; María Cruz Minguillón; Briel Björn; Paul Buckley; Vadimas Dudoitis; Javier Fernández-García; María Fernández-Amado; Joel Ferreira De Brito; Harald Flentje; Eimear Heffernan; Nikolaos Kalivitis; Athina-Cerise Kalogridis; Hannes Keernik; Luminita Marmureanu; Krista Luoma; Angela Marinoni; Michael Pikridas; Gerhard Schauer; Norbert Serfozo; Henri Servomaa; Gloria Titos; Jesús Yus-Díez; Natalia Zioła; Alfred Wiedensohler. Intercomparison and characterization of 23 Aethalometers under laboratory and ambient air conditions: Procedures and unit-to-unit variabilities. 2020, 1 .

AMA Style

Andrea Cuesta-Mosquera, Griša Močnik, Luka Drinovec, Thomas Müller, Sascha Pfeifer, María Cruz Minguillón, Briel Björn, Paul Buckley, Vadimas Dudoitis, Javier Fernández-García, María Fernández-Amado, Joel Ferreira De Brito, Harald Flentje, Eimear Heffernan, Nikolaos Kalivitis, Athina-Cerise Kalogridis, Hannes Keernik, Luminita Marmureanu, Krista Luoma, Angela Marinoni, Michael Pikridas, Gerhard Schauer, Norbert Serfozo, Henri Servomaa, Gloria Titos, Jesús Yus-Díez, Natalia Zioła, Alfred Wiedensohler. Intercomparison and characterization of 23 Aethalometers under laboratory and ambient air conditions: Procedures and unit-to-unit variabilities. . 2020; ():1.

Chicago/Turabian Style

Andrea Cuesta-Mosquera; Griša Močnik; Luka Drinovec; Thomas Müller; Sascha Pfeifer; María Cruz Minguillón; Briel Björn; Paul Buckley; Vadimas Dudoitis; Javier Fernández-García; María Fernández-Amado; Joel Ferreira De Brito; Harald Flentje; Eimear Heffernan; Nikolaos Kalivitis; Athina-Cerise Kalogridis; Hannes Keernik; Luminita Marmureanu; Krista Luoma; Angela Marinoni; Michael Pikridas; Gerhard Schauer; Norbert Serfozo; Henri Servomaa; Gloria Titos; Jesús Yus-Díez; Natalia Zioła; Alfred Wiedensohler. 2020. "Intercomparison and characterization of 23 Aethalometers under laboratory and ambient air conditions: Procedures and unit-to-unit variabilities." , no. : 1.

Preprint content
Published: 28 August 2020
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ACS Style

Andrea Cuesta-Mosquera; Griša Močnik; Luka Drinovec; Thomas Müller; Sascha Pfeifer; María Cruz Minguillón; Briel Björn; Paul Buckley; Vadimas Dudoitis; Javier Fernández-García; María Fernández-Amado; Joel Ferreira De Brito; Harald Flentje; Eimear Heffernan; Nikolaos Kalivitis; Athina-Cerise Kalogridis; Hannes Keernik; Luminita Marmureanu; Krista Luoma; Angela Marinoni; Michael Pikridas; Gerhard Schauer; Norbert Serfozo; Henri Servomaa; Gloria Titos; Jesús Yus-Díez; Natalia Zioła; Alfred Wiedensohler. Supplementary material to "Intercomparison and characterization of 23 Aethalometers under laboratory and ambient air conditions: Procedures and unit-to-unit variabilities". 2020, 1 .

AMA Style

Andrea Cuesta-Mosquera, Griša Močnik, Luka Drinovec, Thomas Müller, Sascha Pfeifer, María Cruz Minguillón, Briel Björn, Paul Buckley, Vadimas Dudoitis, Javier Fernández-García, María Fernández-Amado, Joel Ferreira De Brito, Harald Flentje, Eimear Heffernan, Nikolaos Kalivitis, Athina-Cerise Kalogridis, Hannes Keernik, Luminita Marmureanu, Krista Luoma, Angela Marinoni, Michael Pikridas, Gerhard Schauer, Norbert Serfozo, Henri Servomaa, Gloria Titos, Jesús Yus-Díez, Natalia Zioła, Alfred Wiedensohler. Supplementary material to "Intercomparison and characterization of 23 Aethalometers under laboratory and ambient air conditions: Procedures and unit-to-unit variabilities". . 2020; ():1.

Chicago/Turabian Style

Andrea Cuesta-Mosquera; Griša Močnik; Luka Drinovec; Thomas Müller; Sascha Pfeifer; María Cruz Minguillón; Briel Björn; Paul Buckley; Vadimas Dudoitis; Javier Fernández-García; María Fernández-Amado; Joel Ferreira De Brito; Harald Flentje; Eimear Heffernan; Nikolaos Kalivitis; Athina-Cerise Kalogridis; Hannes Keernik; Luminita Marmureanu; Krista Luoma; Angela Marinoni; Michael Pikridas; Gerhard Schauer; Norbert Serfozo; Henri Servomaa; Gloria Titos; Jesús Yus-Díez; Natalia Zioła; Alfred Wiedensohler. 2020. "Supplementary material to "Intercomparison and characterization of 23 Aethalometers under laboratory and ambient air conditions: Procedures and unit-to-unit variabilities"." , no. : 1.

Journal article
Published: 30 June 2020 in Sustainability
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This research concerns the measurement of daily PM10 concentrations and the assessment of heavy metals and polycyclic aromatic hydrocarbons (PAHs). The measurements were carried out in the urban-industrial area in southern Poland in the period from February to December 2019 (covering heating and non-heating seasons). The metal content of As, Cd, Pb, Ni, Co, Cr, Cu, Zn, V, was estimated using mass spectrometry with inductively excited plasma (ICP-MS), and that of Au and Mg using atomic emission spectrometry with induced plasma (ICP-OES). Analysis of selected PAHs (Naph, Acy, Ace, Fl, Phen, An, Fluo, Pyr, BaA, Chry, BbF, BkF, BaP, IcdP, DahA, BghiP) was performed using a gas chromatograph coupled with mass spectrometry (GC-MS). The share of the analyzed metals in PM10 concentrations was ~ 1.37% in the entire measurement period, ~ 1.09% in the heating season and ~ 1.55% in the non-heating one. High concentrations of aluminum and chromium, observed over the measurement period, indicate the presence of strong anthropogenic sources of both metals. In the case of PAHs in PM10, the average total share of the analyzed was ~ 1.25%, while this share slightly increased in the heating season (average: ~ 2.19%) compared to non-heating (average: ~ 0.63%).

ACS Style

Natalia Zioła; Krzysztof Słaby. The Content of Selected Heavy Metals and Polycyclic Aromatic Hydrocarbons (PAHs) in PM10 in Urban-Industrial Area. Sustainability 2020, 12, 5284 .

AMA Style

Natalia Zioła, Krzysztof Słaby. The Content of Selected Heavy Metals and Polycyclic Aromatic Hydrocarbons (PAHs) in PM10 in Urban-Industrial Area. Sustainability. 2020; 12 (13):5284.

Chicago/Turabian Style

Natalia Zioła; Krzysztof Słaby. 2020. "The Content of Selected Heavy Metals and Polycyclic Aromatic Hydrocarbons (PAHs) in PM10 in Urban-Industrial Area." Sustainability 12, no. 13: 5284.

Journal article
Published: 01 January 2020 in Aerosol and Air Quality Research
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In the present study the results from annual measurement campaign (2018) conducted in Racibórz are presented. Daily PM2.5 samples were analyzed for carbonaceous matter (elemental and organic carbon) and water-soluble ions (Cl-, NO3-, SO42-, Na+, NH4+, K+, Ca2+, Mg2+). The content of secondary inorganic aerosol (SIA) as well as secondary and primary organic carbon (SOC and POC, respectively) was estimated. The contributions of aerosol chemical species along with meteorological parameters were further investigated to reveal the causes of the elevated PM2.5 concentrations. Considering the entire measurement period, PM2.5 concentrations exceeding 50 µg·m-3 were recorded in 38 cases, of which 7 episodes were identified. Such events were only observed in the heating season, due to stable meteorological conditions (low air temperatures, weak winds, high relative humidity, no precipitation) and increased emission of PM and its precursors from anthropogenic sources. The carbonaceous aerosol was the dominant component of PM2.5, especially POC, although the SOC content increased significantly during high pollution periods. The share of SIA clearly decreased with increasing PM2.5 concentration, and its variability was affected to a large extent by regional and/or long-range transport events. The results of the study could provide insights on the development of effective control strategies related to air pollution with fine particulate matter. This is particularly important in Poland, where PM2.5 concentrations remain high compared to many European countries.

ACS Style

Barbara Błaszczak; Natalia Zioła; Barbara Mathews; Krzysztof Klejnowski; Krzysztof Słaby. The Role of PM2.5 Chemical Composition and Meteorology during High Pollution Periods at a Suburban Background Station in Southern Poland. Aerosol and Air Quality Research 2020, 20, 2433 -2447.

AMA Style

Barbara Błaszczak, Natalia Zioła, Barbara Mathews, Krzysztof Klejnowski, Krzysztof Słaby. The Role of PM2.5 Chemical Composition and Meteorology during High Pollution Periods at a Suburban Background Station in Southern Poland. Aerosol and Air Quality Research. 2020; 20 (11):2433-2447.

Chicago/Turabian Style

Barbara Błaszczak; Natalia Zioła; Barbara Mathews; Krzysztof Klejnowski; Krzysztof Słaby. 2020. "The Role of PM2.5 Chemical Composition and Meteorology during High Pollution Periods at a Suburban Background Station in Southern Poland." Aerosol and Air Quality Research 20, no. 11: 2433-2447.

Review
Published: 28 December 2018 in Applied Sciences
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Air pollution by particulate matter (PM) is recognized as a one of the most important environmental issue. A particular attention is being paid to fine PM fraction (PM2.5, PM1.0) due to its detrimental impact on human health and long-term persistence in the air. Presented work is an in-depth bibliometric study on the concentrations and chemical composition of PM2.5 among 27 rural and 38 urban/urban background stations dispersed across the Europe. Obtained results indicate that the chemical composition of PM2.5, in terms of mass concentrations and percentage contribution of main chemical constituents, is relatively different in various parts of Europe. Urban and urban background stations are typically characterized by higher share of total carbon (TC) in PM2.5, compared to rural background sites, mostly pronounced during the heating periods. The share of the secondary inorganic aerosol (SIA) is typically higher at rural background stations, especially in North-Western Europe. In general, the relative contribution of SIA in PM2.5 mass, both at rural and urban background stations, showed more or less pronounced seasonal variation, opposite to Polish measurement sites. Moreover, Poland stands out from the majority of the European stations by strong dominance of total carbon over secondary inorganic aerosol.

ACS Style

Barbara Błaszczak; Kamila Widziewicz-Rzońca; Natalia Zioła; Krzysztof Klejnowski; Katarzyna Juda-Rezler. Chemical Characteristics of Fine Particulate Matter in Poland in Relation with Data from Selected Rural and Urban Background Stations in Europe. Applied Sciences 2018, 9, 98 .

AMA Style

Barbara Błaszczak, Kamila Widziewicz-Rzońca, Natalia Zioła, Krzysztof Klejnowski, Katarzyna Juda-Rezler. Chemical Characteristics of Fine Particulate Matter in Poland in Relation with Data from Selected Rural and Urban Background Stations in Europe. Applied Sciences. 2018; 9 (1):98.

Chicago/Turabian Style

Barbara Błaszczak; Kamila Widziewicz-Rzońca; Natalia Zioła; Krzysztof Klejnowski; Katarzyna Juda-Rezler. 2018. "Chemical Characteristics of Fine Particulate Matter in Poland in Relation with Data from Selected Rural and Urban Background Stations in Europe." Applied Sciences 9, no. 1: 98.